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Colloidal quantum dot materials have been widely studied for their excellent narrow emission spectra,tunable emission wavelengths,high luminous efficiencies and excellent stability,and their simultaneous solution-pro-cessability has made quantum dot light-emitting diodes(QLEDs)widely applicable and used. However,the inherent substrate mode within the device leads to a large amount of photons in QLED devices being confined internally and not utilized. In this work,a solvent self-infiltration nanoimprinting process is developed based on the traditional nanoimprinting process while utilizing the surface binding energy of polydimethylsiloxane (PDMS) material itself,which has low pressure dependence and simplifies the traditional process flow,and based on which the micro-nanostructured patterns in three sizes of 1. 3,1,0. 5 μm with high periodicity are produced. Micro-nano-structured patterned layers of three sizes were fabricated based on which the red,green and blue QLED devices were out-coupled to realize light extraction. In this case,the brightness of the 1. 3 μm micro-nanostructured coupled green QLED device reaches 715 069 cd·m-2,and the maximum external quantum efficiency(EQE)and current efficiency are enhanced to 12. 5% and 57. 3 cd·A-1. The individual electrical performances of the 1 μm-size-coupled blue QLED device are nearly 200% improvement. The EQE of the 0. 5 μm size-coupled red QLED device is also improved from 17. 3% to 20. 5%. And through the angular distribution test,it is proved that the micro-nano structure does not affect the luminous intensity of QLED devices,which is still close to the Lambertian emission. The solvent self-infiltration nanoimprinting process and QLED light extraction method proposed in this work provide a simple and effective way to improve the performance of QLEDs. © 2024 Editorial Office of Chinese Optics. All rights reserved.
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Chinese Journal of Luminescence
ISSN: 1000-7032
CN: 22-1116/O4
Year: 2024
Issue: 4
Volume: 45
Page: 613-620
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ESI Highly Cited Papers on the List: 0 Unfold All
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30 Days PV: 1
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