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author:

Yang, Kaiyu (Yang, Kaiyu.) [1] (Scholars:杨开宇) | Xu, Baolin (Xu, Baolin.) [2] | Lin, Qiuxiang (Lin, Qiuxiang.) [3] | Yu, Yongshen (Yu, Yongshen.) [4] | Hu, Hailong (Hu, Hailong.) [5] (Scholars:胡海龙) | Li, Fushan (Li, Fushan.) [6] (Scholars:李福山)

Indexed by:

Scopus SCIE

Abstract:

Perovskite light-emitting diodes (PeLEDs) have attracted wide attention due to their excellent photoelectric properties. A variety of additives have been studied for perovskite emission layers to enhance the performance of PeLEDs. However, the buried interface, which also has significant influence on the crystallization kinetics and exciton recombination dynamics of the perovskite emission layer, remains to be explored. In this work, we introduced a new ionic liquid 1-Ethyl-3-methylimidazolium dicyanamide (EMIM DCA) with the characteristics of low viscosity and high conductivity into the interfacial layer between the hole transport layer (HTL) and the perovskite film. Due to the strong interaction between the EMIM DCA and perovskite, the crystallization of the perovskite film is obviously improved and the defects at the interface are well passivated. As a result, the nonradiative recombination in the interlayer is significantly reduced. In addition, the introduction of EMIM DCA promoted the injection of charge carriers, thus achieving a high luminance of 32310 cd m(-2) and enabling the maximum external quantum efficiency (EQE) of the PeLEDs increased from 10.2 % to 18.7 %.

Keyword:

Buried interface Ionic liquids Light-emitting diodes Perovskite Q-2D

Community:

  • [ 1 ] [Yang, Kaiyu]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou, Peoples R China
  • [ 2 ] [Xu, Baolin]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou, Peoples R China
  • [ 3 ] [Lin, Qiuxiang]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou, Peoples R China
  • [ 4 ] [Hu, Hailong]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou, Peoples R China
  • [ 5 ] [Li, Fushan]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou, Peoples R China
  • [ 6 ] [Yang, Kaiyu]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou, Peoples R China
  • [ 7 ] [Yu, Yongshen]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou, Peoples R China
  • [ 8 ] [Hu, Hailong]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou, Peoples R China
  • [ 9 ] [Li, Fushan]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou, Peoples R China

Reprint 's Address:

  • 李福山

    [Li, Fushan]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou, Peoples R China

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Source :

CHEMICAL ENGINEERING JOURNAL

ISSN: 1385-8947

Year: 2024

Volume: 483

1 3 . 4 0 0

JCR@2023

Cited Count:

WoS CC Cited Count: 1

SCOPUS Cited Count: 2

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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