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author:

Zhao, Zebang (Zhao, Zebang.) [1] | Liu, Heng (Liu, Heng.) [2] | Yao, Yanyue (Yao, Yanyue.) [3] | Song, Dandan (Song, Dandan.) [4] | Xu, Zheng (Xu, Zheng.) [5] | Qiao, Bo (Qiao, Bo.) [6] | Wu, Chaoxing (Wu, Chaoxing.) [7] (Scholars:吴朝兴) | Swelm, Wageh (Swelm, Wageh.) [8] | Al-Ghamdi, Ahmed (Al-Ghamdi, Ahmed.) [9] | Zhao, Suling (Zhao, Suling.) [10]

Indexed by:

EI Scopus SCIE

Abstract:

The luminescent properties and mechanisms of non-carrier injection (NCI) mode quantum dot light-emitting diodes (QLEDs) are explored in this work. The intermediate insulator electric layer, Poly(vinylidene fluoride-trifluoroethylene-chlorofluoroethylene) (P(VDF-TrFE-CFE)), effectively blocks carrier injection from the electrodes. Carriers for radiative recombination in the quantum dot (QD) layer are generated by the corresponding carrier generation complex layer under an AC electric field. In this investigation, the emission layer (EML), comprising distinct layers of Cd-based quantum dots, is precisely regulated using the spontaneous spreading (SS) method. The work reveals that the thickness of the QDs in NCI-QLEDs significantly influences the device's luminescent performance. In NCI-QLEDs with a double QD layer as the EML, the device exhibits a maximum brightness of 1003.6 cd m ⁻2 and a start-up voltage of 7 root mean square voltage (VRMS). This brightness level represents the highest reported for vertical emission NCI-QLEDs. All devices exhibit a broad range of driven voltages. Interestingly, luminescence is detected only during a half-cycle of the driven signal, as indicated by transient time-resolved spectrum test results. A system is established to analyze the luminescence mechanism comprehensively. Finally, a proposed carrier compounding mechanism sheds light on the behavior of NCI-QLED devices. This work investigates the luminescent properties and mechanisms of quantum dot light-emitting diodes (QLEDs) in non-carrier injection mode. The emission layer is precisely regulated using the spontaneous spreading method. In NCI-QLEDs, employing a double QD layer as the EML, the device achieves a groundbreaking maximum brightness of 1003.6 cd m ⁻2, marking a record for vertical emission NCI-QLEDs.image

Keyword:

high brightness non-carrier-injection spontaneous spreading

Community:

  • [ 1 ] [Zhao, Zebang]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
  • [ 2 ] [Liu, Heng]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
  • [ 3 ] [Yao, Yanyue]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
  • [ 4 ] [Song, Dandan]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
  • [ 5 ] [Xu, Zheng]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
  • [ 6 ] [Qiao, Bo]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
  • [ 7 ] [Zhao, Suling]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China
  • [ 8 ] [Wu, Chaoxing]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China
  • [ 9 ] [Swelm, Wageh]King Abdulaziz Univ, Fac Sci, Dept Phys, Jeddah 21589, Saudi Arabia
  • [ 10 ] [Al-Ghamdi, Ahmed]King Abdulaziz Univ, Fac Sci, Dept Phys, Jeddah 21589, Saudi Arabia

Reprint 's Address:

  • [Zhao, Suling]Beijing Jiaotong Univ, Inst Optoelect Technol, Key Lab Luminescence & Opt Informat, Beijing 100044, Peoples R China;;[Wu, Chaoxing]Fuzhou Univ, Coll Phys & Informat Engn, Fuzhou 350108, Peoples R China;;

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Source :

ADVANCED MATERIALS INTERFACES

ISSN: 2196-7350

Year: 2023

Issue: 7

Volume: 11

4 . 3

JCR@2023

4 . 3 0 0

JCR@2023

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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