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author:

Zhang, Jin (Zhang, Jin.) [1] (Scholars:张进) | Zeng, Liangdan (Zeng, Liangdan.) [2] | Qiao, Ziwen (Qiao, Ziwen.) [3] | Wang, Jun (Wang, Jun.) [4] | Jiang, Xiancai (Jiang, Xiancai.) [5] (Scholars:江献财) | Zhang, Yu Shrike (Zhang, Yu Shrike.) [6] | Yang, Huanghao (Yang, Huanghao.) [7] (Scholars:杨黄浩)

Indexed by:

EI Scopus SCIE

Abstract:

Multifunctional hydrogels have important applications in various fields such as artificial muscles, wearable devices, soft robotics, and tissue engineering, especially for those with favorable mechanical properties, good low-temperature resistance, and stimuli-responsive capabilities. In the current study, a type of polyacrylamide/sodium alginate/carbon nanotube (PAAm/SA/CNT) double-network (DN) hydrogel was fabricated, which exhibited a high tensile strength of 271.68 +/- 6.04 kPa, a favorable conductivity of 1.38 +/- 0.17 S.m(-1), and a good self-healing ability under heating conditions. In addition, the composite hydrogel exhibited controllable photomechanical deformations under near-infrared irradiation, such as bending, swelling, swimming, and object grasping. To further broaden the applications of the hydrogel in low-temperature environments, calcium chloride (CaCl2) was introduced into such a PAAm/SA/CNT DN hydrogel as an additive. Interestingly, the tensile/compressive strengths as well as elasticity were well-maintained at a temperature as low as -20 degrees C. In addition, the PAAm/SA/CNT/CaCl 2 hydrogel presented excellent conductivity, recoverability, and strain-sensing capability under such extreme conditions. Overall, the investigations conducted in this paper have provided potentially new methods and inspirations for the generation of multifunctional PAAm/SA/CNT/CaCl2 hybrid DN hydrogels toward extended applications.

Keyword:

double-network hydrogel low-temperature resistance mechanical performance photomechanical deformation strain sensing

Community:

  • [ 1 ] [Zhang, Yu Shrike]Harvard Med Sch, Brigham & Womens Hosp, Dept Med, Div Engn Med, Cambridge, MA 02139 USA
  • [ 2 ] [Zhang, Jin]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou 350108, Peoples R China
  • [ 3 ] [Zeng, Liangdan]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou 350108, Peoples R China
  • [ 4 ] [Qiao, Ziwen]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou 350108, Peoples R China
  • [ 5 ] [Wang, Jun]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou 350108, Peoples R China
  • [ 6 ] [Yang, Huanghao]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou 350108, Peoples R China
  • [ 7 ] [Zhang, Jin]Fuzhou Univ, Coll Chem Engn, Fuzhou 350108, Peoples R China
  • [ 8 ] [Zeng, Liangdan]Fuzhou Univ, Coll Chem Engn, Fuzhou 350108, Peoples R China
  • [ 9 ] [Qiao, Ziwen]Fuzhou Univ, Coll Chem Engn, Fuzhou 350108, Peoples R China
  • [ 10 ] [Jiang, Xiancai]Fuzhou Univ, Coll Chem Engn, Fuzhou 350108, Peoples R China

Reprint 's Address:

  • 杨黄浩

    [Zhang, Yu Shrike]Harvard Med Sch, Brigham & Womens Hosp, Dept Med, Div Engn Med, Cambridge, MA 02139 USA;;[Yang, Huanghao]Fuzhou Univ, Coll Chem, State Key Lab Photocatalysis Energy & Environm, MOE Key Lab Analyt Sci Food Safety & Biol, Fuzhou 350108, Peoples R China

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Source :

ACS APPLIED MATERIALS & INTERFACES

ISSN: 1944-8244

Year: 2020

Issue: 27

Volume: 12

Page: 30247-30258

9 . 2 2 9

JCR@2020

8 . 5 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:196

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 103

SCOPUS Cited Count: 102

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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