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author:

Qiu, Xuejun (Qiu, Xuejun.) [1] | Tang, Yu (Tang, Yu.) [2] | Shi, Shilong (Shi, Shilong.) [3] | Cai, Yang (Cai, Yang.) [4] | Zhang, Qiaoming (Zhang, Qiaoming.) [5] | Deng, Ping (Deng, Ping.) [6] | Lei, Yanlian (Lei, Yanlian.) [7]

Indexed by:

EI

Abstract:

High-mobility organic field-effect transistors (OFETs), particularly those based on donor-acceptor polymers, often exhibit nonideal transfer characteristics, limiting their practical applications. Doping these semiconductors with specifically designed organic molecular electron acceptors can effectively address these deficiencies. By employing isoindigo-based acceptors with appropriate electron-withdrawing groups as dopants in diketopyrrolopyrrole-thienothiophene-based OFETs, we achieve an outstanding transistor performance with ideal transfer characteristics. Comprehensive analyses using ultraviolet-visible absorption, X-ray diffraction, ultraviolet photoelectron spectroscopy, and electrical measurements demonstrate that p-dopants play crucial roles in enhancing electron transfer, reducing charge carrier traps, and lowering contact resistance, thereby eliminating the typical 'double slope' and hysteresis in OFET transfer characteristics. © 2025 American Chemical Society.

Keyword:

Chemically sensitive field effect transistors Electron mobility High electron mobility transistors Organic field effect transistors Ultraviolet photoelectron spectroscopy

Community:

  • [ 1 ] [Qiu, Xuejun]Guangdong Provincial Engineering and Technology Research Center for Light and Health, School of Health Science, Guangdong Pharmaceutical University, Guangzhou; 510000, China
  • [ 2 ] [Tang, Yu]School of Physical Science and Technology, Chongqing Key Lab of Micro & Nano Structure Optoelectronics, Southwest University, Chongqing; 400715, China
  • [ 3 ] [Shi, Shilong]Guangdong Provincial Engineering and Technology Research Center for Light and Health, School of Health Science, Guangdong Pharmaceutical University, Guangzhou; 510000, China
  • [ 4 ] [Cai, Yang]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 5 ] [Zhang, Qiaoming]School of Physical Science and Technology, Chongqing Key Lab of Micro & Nano Structure Optoelectronics, Southwest University, Chongqing; 400715, China
  • [ 6 ] [Deng, Ping]College of Materials Science and Engineering, Fuzhou University, Fuzhou; 350108, China
  • [ 7 ] [Lei, Yanlian]School of Physical Science and Technology, Chongqing Key Lab of Micro & Nano Structure Optoelectronics, Southwest University, Chongqing; 400715, China

Reprint 's Address:

  • [zhang, qiaoming]school of physical science and technology, chongqing key lab of micro & nano structure optoelectronics, southwest university, chongqing; 400715, china

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Source :

ACS Applied Polymer Materials

Year: 2025

Issue: 9

Volume: 7

Page: 5448-5455

4 . 5 0 0

JCR@2023

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 4

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