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author:

Qiu, Xuejun (Qiu, Xuejun.) [1] | Tang, Yu (Tang, Yu.) [2] | Shi, Shilong (Shi, Shilong.) [3] | Cai, Yang (Cai, Yang.) [4] | Zhang, Qiaoming (Zhang, Qiaoming.) [5] | Deng, Ping (Deng, Ping.) [6] (Scholars:邓平) | Lei, Yanlian (Lei, Yanlian.) [7]

Indexed by:

EI SCIE

Abstract:

High-mobility organic field-effect transistors (OFETs), particularly those based on donor-acceptor polymers, often exhibit nonideal transfer characteristics, limiting their practical applications. Doping these semiconductors with specifically designed organic molecular electron acceptors can effectively address these deficiencies. By employing isoindigo-based acceptors with appropriate electron-withdrawing groups as dopants in diketopyrrolopyrrole-thienothiophene-based OFETs, we achieve an outstanding transistor performance with ideal transfer characteristics. Comprehensive analyses using ultraviolet-visible absorption, X-ray diffraction, ultraviolet photoelectron spectroscopy, and electrical measurements demonstrate that p-dopants play crucial roles in enhancing electron transfer, reducing charge carrier traps, and lowering contact resistance, thereby eliminating the typical "double slope" and hysteresis in OFET transfer characteristics.

Keyword:

donor-acceptorpolymer double-slope isoindigo acceptor organic field-effect transistors transfer curve

Community:

  • [ 1 ] [Qiu, Xuejun]Guangdong Pharmaceut Univ, Guangdong Prov Engn & Technol Res Ctr Light & Hlth, Sch Hlth Sci, Guangzhou 510000, Peoples R China
  • [ 2 ] [Shi, Shilong]Guangdong Pharmaceut Univ, Guangdong Prov Engn & Technol Res Ctr Light & Hlth, Sch Hlth Sci, Guangzhou 510000, Peoples R China
  • [ 3 ] [Tang, Yu]Southwest Univ, Sch Phys Sci & Technol, Chongqing Key Lab Micro&Nano Struct Optoelect, Chongqing 400715, Peoples R China
  • [ 4 ] [Zhang, Qiaoming]Southwest Univ, Sch Phys Sci & Technol, Chongqing Key Lab Micro&Nano Struct Optoelect, Chongqing 400715, Peoples R China
  • [ 5 ] [Lei, Yanlian]Southwest Univ, Sch Phys Sci & Technol, Chongqing Key Lab Micro&Nano Struct Optoelect, Chongqing 400715, Peoples R China
  • [ 6 ] [Cai, Yang]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China
  • [ 7 ] [Deng, Ping]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China

Reprint 's Address:

  • 邓平

    [Zhang, Qiaoming]Southwest Univ, Sch Phys Sci & Technol, Chongqing Key Lab Micro&Nano Struct Optoelect, Chongqing 400715, Peoples R China;;[Lei, Yanlian]Southwest Univ, Sch Phys Sci & Technol, Chongqing Key Lab Micro&Nano Struct Optoelect, Chongqing 400715, Peoples R China;;[Deng, Ping]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Peoples R China

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Source :

ACS APPLIED POLYMER MATERIALS

ISSN: 2637-6105

Year: 2025

Issue: 9

Volume: 7

Page: 5448-5455

4 . 5 0 0

JCR@2023

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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