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author：

Wang, H. (Wang, H..) [1] | Liu, Y. (Liu, Y..) [2] | Zhu, M. (Zhu, M..) [3] | Chen, Y. (Chen, Y..) [4] | Chen, D. (Chen, D..) [5] | Lin, Z. (Lin, Z..) [6] | Wang, K. (Wang, K..) [7] | Xu, Z. (Xu, Z..) [8] | Chen, S. (Chen, S..) [9] | Xing, G. (Xing, G..) [10] | Malyi, O.I. (Malyi, O.I..) [11] | Tang, Y. (Tang, Y..) [12] | Zhang, Y. (Zhang, Y..) [13]

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Scopus

Abstract：

Uneven　Zn　deposition　and　unfavorable　side　reactions　have　prevented　the　reversibility　of　the　Zn　anode.　Herein,　we　design　a　rearranged　(002)　textured　Zn　anode　inspired　by　a　traditional　curvature-enhanced　adsorbate　coverage　(CEAC)　process　to　realize　the　highly　reversible　Zn　anode.　The　rearranged　(002)　textured　structure　directs　superconformal　Zn　deposition　by　controlling　the　spatial　deposition　rate　of　the　rearranged　crystal　planes,　thereby　promoting　bottom-up　“superfilling”　of　the　3D　Zn　skeletons.　Meanwhile,　our　designed　anode　also　induces　the　epitaxial　Zn　deposition,　alleviating　the　parasitic　reactions　owing　to　the　lowest　surface　energy　of　the　(002)　plane.　Attributed　to　these　superiorities,　uniform　and　oriented　Zn　deposition　can　be　obtained,　exhibiting　an　ultra-long　lifespan　over　479　hrs　at　an　ultrahigh　depth　of　discharge　(DOD)　of　82.12　%.　The　Zn|Na2V6O16　⋅　3H2O　battery　delivers　an　improved　cycling　performance,　even　at　a　high　area　capacity　of　5.15　mAh/cm2　with　a　low　negative/positive　(N/P)　capacity　ratio　of　1.63.　The　superconformal　deposition　approach　for　Zn　anodes　paves　the　way　for　the　practical　application　of　high-performance　zinc-ion　batteries.　©　2024　Wiley-VCH　GmbH.

Keyword：

3D Zn anode epitaxial deposition parasitic reactions plastic deformation superconformal electrodeposition

Community：

  • [ 1 ] [Wang H.]Qingyuan Innovation Laboratory, Quanzhou, 362801, China
  • [ 2 ] [Wang H.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 3 ] [Liu Y.]State Key Laboratory of Functional Materials and Devices for Special Environmental Conditions, Xinjiang Technical Institute of Physics & Chemistry, CAS, 40-1 South Beijing Road, Urumqi, 830011, China
  • [ 4 ] [Zhu M.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 5 ] [Chen Y.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 6 ] [Chen D.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 7 ] [Lin Z.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 8 ] [Wang K.]Institute of Applied Physics and Materials Engineering, University of Macau, 999078, Macao
  • [ 9 ] [Xu Z.]Institute of Applied Physics and Materials Engineering, University of Macau, 999078, Macao
  • [ 10 ] [Chen S.]Institute of Applied Physics and Materials Engineering, University of Macau, 999078, Macao
  • [ 11 ] [Xing G.]Institute of Applied Physics and Materials Engineering, University of Macau, 999078, Macao
  • [ 12 ] [Malyi O.I.]Qingyuan Innovation Laboratory, Quanzhou, 362801, China
  • [ 13 ] [Malyi O.I.]Centre of Excellence ENSEMBLE3 Sp. z o. o., Wolczynska Str. 133, Warsaw, 01-919, Poland
  • [ 14 ] [Tang Y.]Qingyuan Innovation Laboratory, Quanzhou, 362801, China
  • [ 15 ] [Tang Y.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 16 ] [Zhang Y.]College of Chemical Engineering, Fuzhou University, Fuzhou, 350116, China

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Angewandte Chemie - International Edition

ISSN： 1433-7851

Year： 2024

Issue： 2

Volume： 64

1 6 . 1 0 0

JCR@2023

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ESI Highly Cited Papers on the List： 0 Unfold All

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