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author:

Yang, Yu (Yang, Yu.) [1] | Zhang, Yan (Zhang, Yan.) [2] | Fang, Zhibin (Fang, Zhibin.) [3] | Zhang, Lulu (Zhang, Lulu.) [4] | Zheng, Zuyang (Zheng, Zuyang.) [5] | Wang, Zhenfeng (Wang, Zhenfeng.) [6] | Feng, Wenhui (Feng, Wenhui.) [7] | Weng, Sunxian (Weng, Sunxian.) [8] | Zhang, Shiying (Zhang, Shiying.) [9] | Liu, Ping (Liu, Ping.) [10] (Scholars:刘平)

Indexed by:

EI Scopus SCIE

Abstract:

CdS has been regarded as a promising photocatalytic water-splitting visible-light photocatalyst, but low catalytic activity and photocorrosion seriously limited its practical application. Here, inspired by core-shell principles, we try to fabricate CdS@MoS2 core-shell structures by utilizing unstable CdS nanowires as core and multilayered MoS2 as shell. Multilayered MoS2 not only serves as a protective shell to preserve CdS but also provides abundant reactive sites and forms a type I junction, giving rise to remarkable hydrogen production activities. The optimum hydrogen production rate based on CdS@MoS2 core-shell composite reaches 26.14 mmol center dot h(-1)center dot g(-1), which is about 54 times greater than that of pure CdS and about twice that of CdS nanowires with 1% Pt. Impressively, the presentation of MoS2 nanosheets can effectively avoid photocorrosion, which resulted in 12 h stable hydrogen production.

Keyword:

CdS nanowires core-shell structure multilayered MoS2 photocatalyst photocorrosion

Community:

  • [ 1 ] [Yang, Yu]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 2 ] [Zhang, Yan]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 3 ] [Fang, Zhibin]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 4 ] [Zhang, Lulu]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 5 ] [Zheng, Zuyang]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 6 ] [Wang, Zhenfeng]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 7 ] [Feng, Wenhui]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 8 ] [Liu, Ping]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China
  • [ 9 ] [Zhang, Shiying]Changsha Univ, Hunan Key Lab Appl Environm Photocatalysis, Changsha 410022, Hunan, Peoples R China
  • [ 10 ] [Weng, Sunxian]State Grid Fujian Elect Power Res Inst, Fuzhou 350002, Peoples R China

Reprint 's Address:

  • 刘平

    [Liu, Ping]Fuzhou Univ, Res Inst Photocatalysis, State Key Lab Breeding Base Photocatalysis, Fuzhou 350002, Peoples R China

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Source :

ACS APPLIED MATERIALS & INTERFACES

ISSN: 1944-8244

Year: 2017

Issue: 8

Volume: 9

Page: 6950-6958

8 . 0 9 7

JCR@2017

8 . 5 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:306

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 111

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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