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author:

Yang, Yu (Yang, Yu.) [1] | Ji, Tao (Ji, Tao.) [2] (Scholars:季韬) | Su, Wenyue (Su, Wenyue.) [3] (Scholars:苏文悦) | Yang, Bin (Yang, Bin.) [4] | Zhang, Yong (Zhang, Yong.) [5] (Scholars:张勇) | Yang, Zhengxian (Yang, Zhengxian.) [6] (Scholars:杨政险)

Indexed by:

EI Scopus SCIE

Abstract:

The combination of photocatalyst with cementitious materials for air pollution abatement and self-cleaning has gained considerable attention. However, the most popularly used photocatalytic cementitious composites based on TiO2 achieve the purification function under ultraviolet sunlight, significantly impeding a broader application of photocatalytic cementitious composites. Here, the photocatalytic cementitious composites were prepared by incorporating g-C3N4 nanosheets (CNNs) in Portland cement. With the increase of CNNs content, the photocatalytic NOx abatement and self-cleaning performance was notably improved, while the micro-hardness of cementitious composites increased first and then decreased. Among the three mixing dosages (0.5%, 1% and 2% by weight of cement), the cementitious composite admixed with 2% CNNs showed the highest photocatalytic NOx abatement efficiency of 227.3 mu mol m(-2) h(-1), and could degrade the rhodamine B within 40 min under visible light. Additionally, its microscopic hardness was 5.4% higher than the one without CNNs, suggesting that a moderate amount of CNNs (below 2%) in cementitious composites was effective in achieving an improved photocatalytic depollution performance. (C) 2019 Elsevier Ltd. All rights reserved.

Keyword:

Cement hydration g-C3N4 nanosheets Micro-hardness Photocatalytic depollution performance Self-cleaning

Community:

  • [ 1 ] [Yang, Yu]Fuzhou Univ, Fujian Prov Univ, Res Ctr Adv Civil Engn Mat, Fuzhou 350116, Fujian, Peoples R China
  • [ 2 ] [Zhang, Yong]Fuzhou Univ, Fujian Prov Univ, Res Ctr Adv Civil Engn Mat, Fuzhou 350116, Fujian, Peoples R China
  • [ 3 ] [Yang, Zhengxian]Fuzhou Univ, Fujian Prov Univ, Res Ctr Adv Civil Engn Mat, Fuzhou 350116, Fujian, Peoples R China
  • [ 4 ] [Yang, Yu]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 5 ] [Ji, Tao]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 6 ] [Yang, Zhengxian]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China
  • [ 7 ] [Su, Wenyue]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350116, Fujian, Peoples R China
  • [ 8 ] [Yang, Bin]Chengdu Design & Res Inst Bldg Mat Ind Co Ltd, Chengdu 610051, Sichuan, Peoples R China
  • [ 9 ] [Zhang, Yong]Delft Univ Technol, Fac Civil Engn & Geosci, Sect Mat & Environm, Microlab, Stevinweg 1, NL-2628 CN Delft, Netherlands
  • [ 10 ] [Yang, Zhengxian]Washington State Univ, Dept Civil & Environm Engn, Pullman, WA 99164 USA

Reprint 's Address:

  • 杨政险

    [Yang, Zhengxian]Fuzhou Univ, Coll Civil Engn, Fuzhou 350116, Fujian, Peoples R China

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Source :

CONSTRUCTION AND BUILDING MATERIALS

ISSN: 0950-0618

Year: 2019

Volume: 225

Page: 120-131

4 . 4 1 9

JCR@2019

7 . 4 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:236

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 26

SCOPUS Cited Count: 30

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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