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author:

Yang, Y. (Yang, Y..) [1] | Ji, T. (Ji, T..) [2] | Su, W. (Su, W..) [3] | Yang, B. (Yang, B..) [4] | Zhang, Y. (Zhang, Y..) [5] | Yang, Z. (Yang, Z..) [6]

Indexed by:

Scopus

Abstract:

The combination of photocatalyst with cementitious materials for air pollution abatement and self-cleaning has gained considerable attention. However, the most popularly used photocatalytic cementitious composites based on TiO2 achieve the purification function under ultraviolet sunlight, significantly impeding a broader application of photocatalytic cementitious composites. Here, the photocatalytic cementitious composites were prepared by incorporating g-C3N4 nanosheets (CNNs) in Portland cement. With the increase of CNNs content, the photocatalytic NOx abatement and self-cleaning performance was notably improved, while the micro-hardness of cementitious composites increased first and then decreased. Among the three mixing dosages (0.5%, 1% and 2% by weight of cement), the cementitious composite admixed with 2% CNNs showed the highest photocatalytic NOx abatement efficiency of 227.3 μmol m−2 h−1, and could degrade the rhodamine B within 40 min under visible light. Additionally, its microscopic hardness was 5.4% higher than the one without CNNs, suggesting that a moderate amount of CNNs (below 2%) in cementitious composites was effective in achieving an improved photocatalytic depollution performance. © 2019 Elsevier Ltd

Keyword:

Cement hydration; g-C3N4 nanosheets; Micro-hardness; Photocatalytic depollution performance; Self-cleaning

Community:

  • [ 1 ] [Yang, Y.]Fujian Provincial University Research Center for Advanced Civil Engineering Materials, Fuzhou University, Fuzhou, 350116, China
  • [ 2 ] [Yang, Y.]College of Civil Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 3 ] [Ji, T.]College of Civil Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 4 ] [Su, W.]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou, 350116, China
  • [ 5 ] [Yang, B.]Chengdu Design & Research Institute of Building Materials Industry Co., Ltd, Chengdu, 610051, China
  • [ 6 ] [Zhang, Y.]Fujian Provincial University Research Center for Advanced Civil Engineering Materials, Fuzhou University, Fuzhou, 350116, China
  • [ 7 ] [Zhang, Y.]Microlab, Section of Materials and Environment, Faculty of Civil Engineering and Geosciences, Delft University of Technology, Stevinweg 1, CN Delft, 2628, Netherlands
  • [ 8 ] [Yang, Z.]Fujian Provincial University Research Center for Advanced Civil Engineering Materials, Fuzhou University, Fuzhou, 350116, China
  • [ 9 ] [Yang, Z.]College of Civil Engineering, Fuzhou University, Fuzhou, 350116, China
  • [ 10 ] [Yang, Z.]Department of Civil & Environmental Engineering, Washington State University, Pullman, WA 99164-2910, United States

Reprint 's Address:

  • [Yang, Z.]College of Civil Engineering, Fuzhou UniversityChina

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Source :

Construction and Building Materials

ISSN: 0950-0618

Year: 2019

Volume: 225

Page: 120-131

4 . 4 1 9

JCR@2019

7 . 4 0 0

JCR@2023

ESI HC Threshold:236

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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