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学者姓名：苏文悦
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Abstract ：
Mimicking photosynthesis to convert CO2 and H2O into value-added chemicals represents an optimal approach to mitigate energy shortages and environmental pollution, and the development of highly efficient and selective photocatalysts for CO2 to CO conversion is essential for the effective utilization of CO2 resources. Herein, a novel 2D@0D InVO4@MnWO4 S-scheme heterojunction composite is successfully developed via an in situ hydrothermal method, achieving the conversion of CO2 into CO under visible light irradiation using H2O as a reducing agent, without any noble metal cocatalysts or sacrificial reagents. The CO generation rate over the optimal InVO4@MnWO4 composite reaches 6.20 mu mol g-1 h-1, which is approximately 4.50 times than that of InVO4. The enhanced photocatalytic performance is ascribed to the charge separation facilitated by the formation of an S-scheme heterojunction between InVO4 and MnWO4. This work is expected to provide a new insight for the design of highly selective photocatalysts for the conversion of CO2 to CO.
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| GB/T 7714 | Xiang, Wenzhuo , Xu, Guoyu , Xiao, Lujiang et al. Construction of a 2D@0D InVO4@MnWO4 S-scheme for efficient photocatalytic reduction of CO2 to CO [J]. | NEW JOURNAL OF CHEMISTRY , 2025 , 49 (9) : 3751-3758 . |
| MLA | Xiang, Wenzhuo et al. "Construction of a 2D@0D InVO4@MnWO4 S-scheme for efficient photocatalytic reduction of CO2 to CO" . | NEW JOURNAL OF CHEMISTRY 49 . 9 (2025) : 3751-3758 . |
| APA | Xiang, Wenzhuo , Xu, Guoyu , Xiao, Lujiang , Zhang, Zizhong , Ji, Tao , Su, Wenyue . Construction of a 2D@0D InVO4@MnWO4 S-scheme for efficient photocatalytic reduction of CO2 to CO . | NEW JOURNAL OF CHEMISTRY , 2025 , 49 (9) , 3751-3758 . |
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Employing photocatalytic technology to transform CO2 into valuable fuels is considered a promising solution for addressing the exacerbated greenhouse effect and energy crisis. The development of photocatalysts featuring superior charge separation efficiency is pivotal for the widespread implementation of photocatalytic CO2 reduction technologies. Herein, zero-dimensional (0D) NixP nanoparticles are anchored onto two-dimensional (2D) LaTiO2N nanosheets by a photo-deposition method, and a NixP/LaTiO2N Schottky junction composite with excellent photocatalytic CO2 reduction performance is constructed. The optimal NixP/LaTiO2N composite achieves CO and CH4 yields of 9.39 and 4.15 mu mol g-1 h-1, respectively, with the utilized photoelectron number (UPN) reaching 51.98 mu mol g-1, which is approximately 9.7 times higher than that of LaTiO2N alone. The improved photocatalytic performance of the composites can be attributed to the formation of Schottky junctions, which effectively suppress the recombination of photogenerated carriers. This study provides a new idea for the development of 0D/2D Schottky junction photocatalysts.
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| GB/T 7714 | Xu, Guoyu , Chen, Yanan , Lin, Peiling et al. Construction of a 0D/2D NixP/LaTiO2N Schottky junction photocatalyst for efficient visible-light-driven photocatalytic CO2 reduction [J]. | CATALYSIS SCIENCE & TECHNOLOGY , 2025 , 15 (6) : 2027-2033 . |
| MLA | Xu, Guoyu et al. "Construction of a 0D/2D NixP/LaTiO2N Schottky junction photocatalyst for efficient visible-light-driven photocatalytic CO2 reduction" . | CATALYSIS SCIENCE & TECHNOLOGY 15 . 6 (2025) : 2027-2033 . |
| APA | Xu, Guoyu , Chen, Yanan , Lin, Peiling , Zhang, Zizhong , Ji, Tao , Su, Wenyue . Construction of a 0D/2D NixP/LaTiO2N Schottky junction photocatalyst for efficient visible-light-driven photocatalytic CO2 reduction . | CATALYSIS SCIENCE & TECHNOLOGY , 2025 , 15 (6) , 2027-2033 . |
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The photocatalytic conversion of CO2 into hydrocarbon fuel holds immense potential for achieving a carbon closed loop and carbon neutrality. Developing efficient photocatalysts plays a pivotal role in enabling the widespread application of photocatalytic CO2 reduction on a large scale. Herein, a novel S-scheme MnWO4/LaTiO2N heterojunction composite is successfully synthesized by a hydrothermal method. This composite catalyst demonstrates excellent photocatalytic activity in the reduction of CO2 to CO and CH4 using water molecules as electron donors under visible light irradiation, and the optimized 30% MnWO4/LaTiO2N composite displays significantly enhanced CO and CH4 yields of 3.94 and 0.81 μmol g-1 h-1, respectively, and the corresponding utilized photoelectron number reaches 14.7 μmol g-1 h-1, which is approximately 7.7 and 12.9 times that of LaTiO2N and MnWO4. The enhancement in photocatalytic activity of the composites can be ascribed to the construction of an S-scheme heterojunction, which exhibits improved charge transfer dynamics, retains the strongest redox capacity, and effectively suppresses back reactions. In situ Fourier-transform infrared imaging provides evidence, to a certain extent, for the existence of a temporal gradient order in the generation of multiple products during the photocatalytic reduction of CO2. © 2024 American Chemical Society.
Keyword ：
LaTiO2N LaTiO2N MnWO4 MnWO4 photocatalytic CO2 conversion photocatalytic CO2 conversion S-scheme heterojunction S-scheme heterojunction visible light visible light
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| GB/T 7714 | Qi, J. , Zhang, Z. , Zhang, L. et al. Anchoring MnWO4 Nanorods on LaTiO2N Nanoplates for Boosted Visible Light-Driven Overall CO2 Reduction [J]. | ACS Applied Materials and Interfaces , 2024 , 16 (36) : 47741-47750 . |
| MLA | Qi, J. et al. "Anchoring MnWO4 Nanorods on LaTiO2N Nanoplates for Boosted Visible Light-Driven Overall CO2 Reduction" . | ACS Applied Materials and Interfaces 16 . 36 (2024) : 47741-47750 . |
| APA | Qi, J. , Zhang, Z. , Zhang, L. , Fu, X. , Ji, T. , Su, W. . Anchoring MnWO4 Nanorods on LaTiO2N Nanoplates for Boosted Visible Light-Driven Overall CO2 Reduction . | ACS Applied Materials and Interfaces , 2024 , 16 (36) , 47741-47750 . |
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The interaction of low energy electrons (LEEs; 1-30 eV) with genomic material can induce multiple types of damage that may cause the loss of genetic information, mutations, genome instability, and cell death. For all damages measurable by electrophoresis, we provide the first complete set of G-values (yield of a specific product per energy deposited) induced in plasmid DNA by the direct and indirect effects of LEEs (G LEE) and 1.5 keV X-rays (G X) under identical conditions. Low energy photoelectrons are produced via X-rays incident on a tantalum (Ta) substrate covered with DNA and placed in a chamber filled with nitrogen at atmospheric pressure, under four different humidity levels, ranging from dry conditions to full hydration (Gamma = 2.5 to Gamma = 33, where Gamma is the number of water molecules/nucleotide). Damage yields are measured as a function of X-ray fluence and humidity. G LEE values are between 2 and 27 times larger than those for X-rays. At Gamma = 2.5 and 33, G LEE values for double strand breaks are 27 and 16 times larger than G X, respectively. The indirect effect contributes similar to 50% to the total damage. These G-values allow quantification of potentially lethal lesions composed of strand breaks and/or base damages in the presence of varying amounts of water, i.e., closer to cellular conditions.
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| GB/T 7714 | Gao, Yingxia , Dong, Yanfang , Wang, Xuran et al. Comparisons between the Direct and Indirect Effect of 1.5 keV X-rays and 0-30 eV Electrons on DNA: Base Lesions, Stand Breaks, Cross-Links, and Cluster Damages [J]. | JOURNAL OF PHYSICAL CHEMISTRY B , 2024 , 128 (45) : 11041-11053 . |
| MLA | Gao, Yingxia et al. "Comparisons between the Direct and Indirect Effect of 1.5 keV X-rays and 0-30 eV Electrons on DNA: Base Lesions, Stand Breaks, Cross-Links, and Cluster Damages" . | JOURNAL OF PHYSICAL CHEMISTRY B 128 . 45 (2024) : 11041-11053 . |
| APA | Gao, Yingxia , Dong, Yanfang , Wang, Xuran , Su, Wenyue , Cloutier, Pierre , Zheng, Yi et al. Comparisons between the Direct and Indirect Effect of 1.5 keV X-rays and 0-30 eV Electrons on DNA: Base Lesions, Stand Breaks, Cross-Links, and Cluster Damages . | JOURNAL OF PHYSICAL CHEMISTRY B , 2024 , 128 (45) , 11041-11053 . |
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Solar-powered photocatalytic water splitting for hydrogen evolution presents a promising solution to the energy crisis and contemporary environmental challenges. Herein, a Z-scheme ZnS/LaTiO2N heterojunction composite, incorporating zinc vacancies, has been successfully synthesized to enable photocatalytic hydrogen evolution under visible-light illumination. The optimized ZnS(VZn)/LaTiO2N composite demonstrates a hydrogen evolution activity 13 times higher than that of individual ZnS(VZn). The heterojunction between ZnS and LaTiO2N, in conjunction with zinc vacancies, expands the photoresponse spectrum and facilitates the spatial separation and transfer of photogenerated carriers. Consequently, this synergy significantly enhances the performance of photocatalytic hydrogen evolution. The collaborative action of the Z-scheme heterojunction and zinc vacancies paves the way for innovative approaches in designing future high-efficiency photocatalysts.
Keyword ：
LaTiO2N LaTiO2N Photocatalytic H 2 evolution Photocatalytic H 2 evolution ZnS(VZn) ZnS(VZn) Z-scheme heterojunction Z-scheme heterojunction
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| GB/T 7714 | Yu, Jiaqi , Qi, Jinwei , Lin, Nansong et al. Zinc-vacancy mediated Z-scheme photocatalyst of ZnS/LaTiO2N for hydrogen evolution under visible-light [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 976 . |
| MLA | Yu, Jiaqi et al. "Zinc-vacancy mediated Z-scheme photocatalyst of ZnS/LaTiO2N for hydrogen evolution under visible-light" . | JOURNAL OF ALLOYS AND COMPOUNDS 976 (2024) . |
| APA | Yu, Jiaqi , Qi, Jinwei , Lin, Nansong , Zhang, Zizhong , Ji, Tao , Su, Wenyue . Zinc-vacancy mediated Z-scheme photocatalyst of ZnS/LaTiO2N for hydrogen evolution under visible-light . | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 976 . |
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Simulating photosynthesis to convert CO2 into valuable chemicals is an effective strategy to achieve sustainable carbon recycles, and the high conversion efficiency and selectivity of photocatalytic conversion CO2 to specific chemicals are the key challenges. Herein, a direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst is successfully synthesized by electrostatic self-assembly method. The selectivity of CO2 reduction to CO is improved from 74% of La2Ti2O7 to nearly 100%, and the CO yield is 7.5 times that of individual La2Ti2O7. The improvement of the photocatalytic performance is attributed to the formation of Z-scheme heterojunction between Bi2WO6 and La2Ti2O7, which facilitates the separation and transfer of photogenerated carriers. This work provides a new insight for the construction of efficient photocatalyst for selective reduction of CO2 to CO.
Keyword ：
Bi2WO6 Bi2WO6 CO selectivity CO selectivity PhotocatalyticCO2 reduction PhotocatalyticCO2 reduction Z-scheme heterojunction Z-scheme heterojunction
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| GB/T 7714 | Chen, Jianxiong , Lin, Lichao , Lin, Peiling et al. A direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst for selective reduction of CO2 to CO [J]. | CHINESE JOURNAL OF STRUCTURAL CHEMISTRY , 2023 , 42 (4) . |
| MLA | Chen, Jianxiong et al. "A direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst for selective reduction of CO2 to CO" . | CHINESE JOURNAL OF STRUCTURAL CHEMISTRY 42 . 4 (2023) . |
| APA | Chen, Jianxiong , Lin, Lichao , Lin, Peiling , Xiao, Lujiang , Zhang, Lingqian , Lu, Ying et al. A direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst for selective reduction of CO2 to CO . | CHINESE JOURNAL OF STRUCTURAL CHEMISTRY , 2023 , 42 (4) . |
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Using solar-powered photocatalytic technology to convert CO2 to high value-added chemical products is a hopeful strategy to solve the energy and environmental problems of modern society. Herein, a direct Z-scheme InVO4/La2Ti2O7 photocatalyst is successfully synthesized, achieving efficient and selective CO2 re-duction to CO with nearly 100 % CO selectivity, and the CO yield is 4.2 and 3.3 times that of individual La2Ti2O7 and InVO4, respectively. The significantly enhanced photocatalytic performance is owing to the formation of Z-scheme charge transfer mechanism, fostering the spatial separation and transfer of pho-togenerated carriers. This work provides new perspectives for the rational design of La2Ti2O7-based pho-tocatalytic materials toward efficient and selective CO2 reduction to CO. (c) 2022 Elsevier B.V. All rights reserved.
Keyword ：
Direct Z-Scheme Direct Z-Scheme PhotocatalyticCO2 reduction PhotocatalyticCO2 reduction Selectivity Selectivity
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| GB/T 7714 | Xiao, Lujiang , Lin, Lichao , Song, Jia et al. Construction of a direct Z-scheme InVO4/La2Ti2O7 photocatalyst toward efficient and selective CO2 reduction to CO [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2023 , 935 . |
| MLA | Xiao, Lujiang et al. "Construction of a direct Z-scheme InVO4/La2Ti2O7 photocatalyst toward efficient and selective CO2 reduction to CO" . | JOURNAL OF ALLOYS AND COMPOUNDS 935 (2023) . |
| APA | Xiao, Lujiang , Lin, Lichao , Song, Jia , Zhang, Zizhong , Wang, Xuxu , Su, Wenyue . Construction of a direct Z-scheme InVO4/La2Ti2O7 photocatalyst toward efficient and selective CO2 reduction to CO . | JOURNAL OF ALLOYS AND COMPOUNDS , 2023 , 935 . |
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Coupling hydrogen production with selective organic synthesis in one cooperative manner offers a novel strategy for green synthesis by virtue of the photogenerated carriers. Herein, a dual-functional photocatalyst of CoSx/Cd0.7Zn0.3S without noble metals is reported for efficient selective benzaldehyde (BAD) synthesis coupled with H-2 production. The CoSx/Cd0.7Zn0.3S composite showed a higher photocatalytic performance than Cd0.7Zn0.3S and 1 wt% Pt/Cd0.7Zn0.3S, which was attributed to the loaded CoSx, as the cocatalyst, which could accumulate the photogenerated electrons from Cd0.7Zn0.3S, promote the separation of photogenerated charge carriers, and reduce the overpotential of hydrogen production. This study provides a new strategy for the design and synthesis of low-cost, high-efficiency composite materials for photocatalytic efficient selective benzaldehyde (BAD) synthesis coupled with H-2 production.
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| GB/T 7714 | Chen, Xinan , Yu, Jiaqi , Zhang, Zifan et al. Dual-functional photocatalyst of CoSx/Cd0.7Zn0.3S without noble metals for efficient selective benzaldehyde synthesis coupled with H2 production [J]. | CATALYSIS SCIENCE & TECHNOLOGY , 2023 , 13 (21) : 6291-6296 . |
| MLA | Chen, Xinan et al. "Dual-functional photocatalyst of CoSx/Cd0.7Zn0.3S without noble metals for efficient selective benzaldehyde synthesis coupled with H2 production" . | CATALYSIS SCIENCE & TECHNOLOGY 13 . 21 (2023) : 6291-6296 . |
| APA | Chen, Xinan , Yu, Jiaqi , Zhang, Zifan , Zhang, Zizhong , Ji, Tao , Su, Wenyue . Dual-functional photocatalyst of CoSx/Cd0.7Zn0.3S without noble metals for efficient selective benzaldehyde synthesis coupled with H2 production . | CATALYSIS SCIENCE & TECHNOLOGY , 2023 , 13 (21) , 6291-6296 . |
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Simulating photosynthesis to convert CO2 into valuable chemicals is an effective strategy to achieve sustainable carbon recycles,and the high conversion efficiency and selectivity of photocatalytic conversion CO2 to specific chemicals are the key challenges.Herein,a direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst is successfully syn-thesized by electrostatic self-assembly method.The selectivity of CO2 reduction to CO is improved from 74％of La2Ti2O7 to nearly 100％,and the CO yield is 7.5 times that of individual La2Ti2O7.The improvement of the photocatalytic performance is attributed to the formation of Z-scheme heterojunction between Bi2WO6 and La2Ti2O7,which facilitates the separation and transfer of photogenerated carriers.This work provides a new insight for the construction of efficient photocatalyst for selective reduction of CO2 to CO.
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| GB/T 7714 | Jianxiong Chen , Lichao Lin , Peiling Lin et al. A direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst for selective reduction of CO2 to CO [J]. | 结构化学 , 2023 , 42 (4) : 38-45 . |
| MLA | Jianxiong Chen et al. "A direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst for selective reduction of CO2 to CO" . | 结构化学 42 . 4 (2023) : 38-45 . |
| APA | Jianxiong Chen , Lichao Lin , Peiling Lin , Lujiang Xiao , Lingqian Zhang , Ying Lu et al. A direct Z-scheme Bi2WO6/La2Ti2O7 photocatalyst for selective reduction of CO2 to CO . | 结构化学 , 2023 , 42 (4) , 38-45 . |
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本发明涉及一种复合光催化剂MPc/La2Ti2O7及其制备方法与应用，其属于光催化领域。本发明将难溶的MPc超声分散成水分散液，分别加入钛源和镧源制成钛源MPc混合溶液和镧源MPc混合溶液，通过水热法合成所述复合光催化剂MPc/La2Ti2O7。本发明采用一步水热法制备复合光催化剂MPc/La2Ti2O7，无需引入模板剂，简单易行，环境友好，易于大规模推广。所得的复合光催化剂MPc/La2Ti2O7呈二维片状形貌，能够在可见光照射下还原CO2生成CO等重要工业原料，具有良好应用前景。
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| GB/T 7714 | 王心晨 , 林立超 , 苏文悦 et al. 复合光催化剂金属酞菁/钛酸镧及其制备方法与应用 : CN202111641769.8[P]. | 2021-12-30 00:00:00 . |
| MLA | 王心晨 et al. "复合光催化剂金属酞菁/钛酸镧及其制备方法与应用" : CN202111641769.8. | 2021-12-30 00:00:00 . |
| APA | 王心晨 , 林立超 , 苏文悦 , 林佩灵 , 肖鲁江 , 苏柠溪 . 复合光催化剂金属酞菁/钛酸镧及其制备方法与应用 : CN202111641769.8. | 2021-12-30 00:00:00 . |
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