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author:

Gu, Jianfeng (Gu, Jianfeng.) [1] | Huang, Jianren (Huang, Jianren.) [2] | Chen, Guoqi (Chen, Guoqi.) [3] | Hou, Linxi (Hou, Linxi.) [4] (Scholars:侯琳熙) | Zhang, Jin (Zhang, Jin.) [5] (Scholars:张进) | Zhang, Xi (Zhang, Xi.) [6] | Yang, Xiaoxiang (Yang, Xiaoxiang.) [7] | Guan, Lunhui (Guan, Lunhui.) [8] | Jiang, Xiancai (Jiang, Xiancai.) [9] (Scholars:江献财) | Liu, Huiyong (Liu, Huiyong.) [10] (Scholars:刘慧勇)

Indexed by:

EI Scopus SCIE

Abstract:

Hydrogels are important for stretchable and wearable multifunctional sensors, but their application is limited by their low mechanical strength and poor long-term stability. Herein, a conductive organohydrogel with a 3D honeycomb structure was prepared by integrating carbon nanotubes (CNTs) and carbon black (CB) into a poly(vinyl alcohol)/glycerol (PVA/Gly) organohydrogel. Such a nanocomposite organohydrogel is built on a physical cross-linking network formed by the hydrogen bonds among PVA, glycerol, and water. CNTs and CB had an add-in synergistic impact on the mechanical and electrical performances of the PVA/Gly organohydrogel because of the distinct aspect ratios and geometric shapes. The prepared organohydrogel integrated with a tensile strength of 4.8 MPa, a toughness of 15.93 MJ m(-3), and flexibility with an elongation at break up to 640%. The organohydrogels also showed good antifreezing feature, long-term moisture retention, self-healing, and thermoplasticity. Sensors designed from these organohydrogels displayed high stretching sensitivity to tensile strain and temperature, with a gauge factor of 2.1 within a relatively broad strain range (up to similar to 600% strain), a temperature coefficient of resistance of -0.935%.degrees C-1, and long-term durability. The sensors could detect full-range human physiological signals and respond to the change in temperature, which are highly desired for multifunctional wearable electronic devices.

Keyword:

antifreezing hydrogel electrolyte sensor thermoplasticity toughness

Community:

  • [ 1 ] [Gu, Jianfeng]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China
  • [ 2 ] [Chen, Guoqi]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China
  • [ 3 ] [Hou, Linxi]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China
  • [ 4 ] [Zhang, Jin]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China
  • [ 5 ] [Jiang, Xiancai]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China
  • [ 6 ] [Liu, Huiyong]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China
  • [ 7 ] [Huang, Jianren]Fuzhou Univ, Sch Mech Engn & Automat, Fuzhou 350108, Peoples R China
  • [ 8 ] [Yang, Xiaoxiang]Fuzhou Univ, Sch Mech Engn & Automat, Fuzhou 350108, Peoples R China
  • [ 9 ] [Huang, Jianren]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 10 ] [Guan, Lunhui]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 11 ] [Zhang, Xi]Sichuan Univ, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China
  • [ 12 ] [Jiang, Xiancai]Sichuan Univ, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China

Reprint 's Address:

  • 江献财 刘慧勇

    [Jiang, Xiancai]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China;;[Liu, Huiyong]Fuzhou Univ, Sch Chem Engn, Fuzhou 350108, Peoples R China;;[Jiang, Xiancai]Sichuan Univ, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China

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Source :

ACS APPLIED MATERIALS & INTERFACES

ISSN: 1944-8244

Year: 2020

Issue: 36

Volume: 12

Page: 40815-40827

9 . 2 2 9

JCR@2020

8 . 5 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:196

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 178

SCOPUS Cited Count: 154

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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