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author:

Li, Xiaolong (Li, Xiaolong.) [1] | Cai, Jiafeng (Cai, Jiafeng.) [2] | Li, Maoquan (Li, Maoquan.) [3] | Zhang, Lisha (Zhang, Lisha.) [4] | Chen, Zhigang (Chen, Zhigang.) [5]

Indexed by:

EI Scopus SCIE

Abstract:

Integrated membranes with filtration and photocatalytic functions have been considered as an effective strategy for purifying flowing wastewater, but the design and preparation of high-efficiency and low-cost membranes is still of great urgency. Herein, we report efficient recyclable BiOBrxI1-x fibrous filter membranous photocatalyst prepared through the in-situ growth of BiOBrxI1-x solid-solutions with tunable band-gaps on carbon fiber cloth (CFC). The fabrication was performed via a facile dipping-solvothermal synthesis of BiOBrxI1-x solid-solutions nanoplates on CFC with different I/Br ratios in the precursor solution. With the increase of I/Br ratio from 0 to 4, CFC/BiOBrxI1-x solid-solutions exhibit a re-shifted in the photoabsorption edge from 420 to 620 nm, leading to the tuning of the band-gap from 2.49 to 1.81 eV. Under visible light illumination for 120 min, CFC/ BiOBrxI1-x solid-solutions have the tuned photocatalytic activity, where CFC/BiOBr0.8I0.2 shows the highest degradation efficiency toward various antibiotics (such as levofloxacin (LVFX, 94.1%), ciprofloxacin (CIP, 94.5%), and tetracycline (TC, 98.9%)) as well as dyes (such as acid orange 7 (AO7, 91.4%). Especially, when CFC/BiOBr0.8I0.2 is used as a flexible membrane to a construct multi-grade unit for treating the flowing sewage, the degradation efficiency of LVFX goes up from 3.9% in the first grade to 96.2% in the tenth grade. Therefore, the present CFC/BiOBr0.8I0.2 not only possesses great potential as a flexible membrane-shaped photocatalyst for purifying the flowing sewage efficiently but also provides some insights for developing new types of purifying membranes and devices.

Keyword:

BiOBr x I 1-x solid-solution Carbon fiber cloth Filtration membrane Flowing wastewater Photocatalysis

Community:

  • [ 1 ] [Li, Xiaolong]Tongji Univ, Shanghai Peoples Hosp 10, Dept Intervent & Vasc Surg, Sch Med, Shanghai 200072, Peoples R China
  • [ 2 ] [Li, Maoquan]Tongji Univ, Shanghai Peoples Hosp 10, Dept Intervent & Vasc Surg, Sch Med, Shanghai 200072, Peoples R China
  • [ 3 ] [Chen, Zhigang]Tongji Univ, Shanghai Peoples Hosp 10, Dept Intervent & Vasc Surg, Sch Med, Shanghai 200072, Peoples R China
  • [ 4 ] [Li, Xiaolong]Donghua Univ, Coll Environm Sci & Engn, State Key Lab Modificat Chem Fibers & Polymer Mat, Shanghai 201620, Peoples R China
  • [ 5 ] [Cai, Jiafeng]Donghua Univ, Coll Environm Sci & Engn, State Key Lab Modificat Chem Fibers & Polymer Mat, Shanghai 201620, Peoples R China
  • [ 6 ] [Zhang, Lisha]Donghua Univ, Coll Environm Sci & Engn, State Key Lab Modificat Chem Fibers & Polymer Mat, Shanghai 201620, Peoples R China
  • [ 7 ] [Chen, Zhigang]Donghua Univ, Coll Mat Sci & Engn, Shanghai 201620, Peoples R China
  • [ 8 ] [Cai, Jiafeng]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350116, Peoples R China
  • [ 9 ] [Zhang, Lisha]Fuzhou Univ, State Key Lab Photocatalysis Energy & Environm, Fuzhou 350116, Peoples R China
  • [ 10 ] [Zhang, Lisha]Shanghai Inst Pollut Control & Ecol Secur, Shanghai 200092, Peoples R China

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Source :

JOURNAL OF CLEANER PRODUCTION

ISSN: 0959-6526

Year: 2023

Volume: 414

9 . 8

JCR@2023

9 . 8 0 0

JCR@2023

ESI Discipline: ENGINEERING;

ESI HC Threshold:35

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 8

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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