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author：

Zeng, R. (Zeng, R..) [1] | Lin, L. (Lin, L..) [2] | Gong, H. (Gong, H..) [3] | Li, Y. (Li, Y..) [4] | Xu, J. (Xu, J..) [5] | Huang, L. (Huang, L..) [6] | Wang, W. (Wang, W..) [7] | Lin, S. (Lin, S..) [8] | Tang, D. (Tang, D..) [9] | Guo, S. (Guo, S..) [10]

Indexed by：

ESCI Scopus

Abstract：

A　uric　acid　(UA)　electrooxidation-based　electrochemical　sensing　system　is　of　great　interest　in　the　field　of　measurement　science　and　technology;　however,　its　development　is　greatly　plagued　by　the　lack　of　efficient　electrocatalysts,　leading　to　low　detection　sensitivity.　Herein,　we　report　a　general　method　for　making　a　series　of　metal　single-atom　catalysts　(SACs)　on　nitrogen-doped　carbon　(M1-CN,　M　=　Mo,　Fe,　Ru,　Mn,　Co,　Cu,　Pt,　Ni)　to　tune　the　rate-determining　step　(RDS)　of　UA　electrooxidation　to　greatly　boost　its　electrocatalytic　performance.　We　experimentally　demonstrate　that　the　Mo1-CN　shows　the　highest　electrocatalytic　activity　for　UA　electrooxidation　among　the　investigated　M1-CN.　As　a　proof-of-concept　application,　we　construct　a　portable　and　wireless　biosensor　for　high-throughput　detection　of　disease　markers　(human　papillomavirus-16　[HPV-16])　based　on　the　particular　advantage　of　Mo1-CN　in　enhancing　the　UA　electrooxidation　performance.　©　2023

Keyword：

metal-nitrogen-carbon nucleic acid sensing rate-determining step SDG3: Good health and well-being single-atom-site catalysts uric acid electrooxidation

Community：

  • [ 1 ] [Zeng, R.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 2 ] [Zeng, R.]School of Materials Science and Engineering, Peking University, Beijing, 100871, China
  • [ 3 ] [Lin, L.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 4 ] [Gong, H.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 5 ] [Li, Y.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 6 ] [Xu, J.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 7 ] [Huang, L.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 8 ] [Wang, W.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 9 ] [Lin, S.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 10 ] [Tang, D.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), State Key Laboratory of Photocatalysis on Energy and Environment, Department of Chemistry, Fuzhou University, Fuzhou, 350108, China
  • [ 11 ] [Guo, S.]School of Materials Science and Engineering, Peking University, Beijing, 100871, China

Reprint 's Address：

  • [Tang, D.]Key Laboratory for Analytical Science of Food Safety and Biology (MOE & Fujian Province), China;;[Guo, S.]School of Materials Science and Engineering, China

Email：


dianping.tang@fzu.edu.cn |
guosj@pku.edu.cn
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Source ：

Chem Catalysis

ISSN： 2667-1107

Year： 2023

Issue： 2

Volume： 3

1 1 . 5

JCR@2023

1 1 . 5 0 0

JCR@2023

JCR Journal Grade：1

Cited Count：

WoS CC Cited Count： 0

SCOPUS Cited Count： 55

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 0

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