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author:

Li, Caicong (Li, Caicong.) [1] | Liu, Jie (Liu, Jie.) [2] | Peng, Hailong (Peng, Hailong.) [3] | Sui, Yuan (Sui, Yuan.) [4] | Song, Jian (Song, Jian.) [5] | Liu, Yang (Liu, Yang.) [6] | Huang, Wei (Huang, Wei.) [7] | Chen, Xiaowei (Chen, Xiaowei.) [8] | Shen, Jinghui (Shen, Jinghui.) [9] | Ling, Yao (Ling, Yao.) [10] | Huang, Chongyu (Huang, Chongyu.) [11] | Hong, Youwei (Hong, Youwei.) [12] | Huang, Weiguo (Huang, Weiguo.) [13]

Indexed by:

EI

Abstract:

Numerous emerging applications in modern society require humidity sensors that are not only sensitive and specific but also durable and intelligent. However, conventional humidity sensors do not have all of these simultaneously because they require very different or even contradictory design principles. Here, inspired by camel noses, we develop a porous zwitterionic capacitive humidity sensor. Relying on the synergistic effect of a porous structure and good chemical and thermal stabilities of hygroscopic zwitterions, this sensor simultaneously exhibits high sensitivity, discriminability, excellent durability, and, in particular, the highest respond speed among reported capacitive humidity sensors, with demonstrated applications in the fast discrimination between fresh, stale, and dry leaves, high-resolution touchless human-machine interactive input devices, and the real-time monitoring humidity level of a hot industrial exhaust. More importantly, this sensor exhibits typical synapse behaviors such as paired-pulse facilitation due to the strong binding interactions between water and zwitterions. This leads to learning and forgetting features with a tunable memory, thus giving the sensor artificial intelligence and enabling the location of water sources. This work offers a general design principle expected to be applied to develop other high-performance biochemical sensors and the next-generation intelligent sensors with much broader applications. ©

Keyword:

Binding energy Capacitive sensors Durability Humidity sensors Location

Community:

  • [ 1 ] [Li, Caicong]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 2 ] [Li, Caicong]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 3 ] [Liu, Jie]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 4 ] [Liu, Jie]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 5 ] [Liu, Jie]College of Chemistry and Materials Science, Fujian Normal University, Fujian, Fuzhou; 350002, China
  • [ 6 ] [Peng, Hailong]School of Resources,Environmental, and Chemical Engineering, Nanchang University, Nanchang; 330031, China
  • [ 7 ] [Sui, Yuan]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 8 ] [Sui, Yuan]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 9 ] [Song, Jian]Science and Technology on Microsystem Laboratory, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai; 200050, China
  • [ 10 ] [Liu, Yang]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 11 ] [Liu, Yang]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 12 ] [Liu, Yang]College of Chemistry and Materials Science, Fujian Normal University, Fujian, Fuzhou; 350002, China
  • [ 13 ] [Huang, Wei]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 14 ] [Huang, Wei]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 15 ] [Huang, Wei]College of Chemistry and Materials Science, Fujian Normal University, Fujian, Fuzhou; 350002, China
  • [ 16 ] [Chen, Xiaowei]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 17 ] [Chen, Xiaowei]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 18 ] [Chen, Xiaowei]College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 19 ] [Shen, Jinghui]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 20 ] [Shen, Jinghui]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 21 ] [Shen, Jinghui]University of Chinese Academy of Sciences, 19A Yuquan Road, Beijing; 100049, China
  • [ 22 ] [Ling, Yao]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 23 ] [Ling, Yao]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 24 ] [Ling, Yao]University of Chinese Academy of Sciences, 19A Yuquan Road, Beijing; 100049, China
  • [ 25 ] [Huang, Chongyu]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 26 ] [Huang, Chongyu]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 27 ] [Huang, Chongyu]University of Chinese Academy of Sciences, 19A Yuquan Road, Beijing; 100049, China
  • [ 28 ] [Hong, Youwei]Key Lab of Urban Environment and Health, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen; 361021, China
  • [ 29 ] [Huang, Weiguo]State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, 155 Yangqiao West Road, Fujian, Fuzhou; 350002, China
  • [ 30 ] [Huang, Weiguo]Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fujian, Fuzhou; 350002, China
  • [ 31 ] [Huang, Weiguo]University of Chinese Academy of Sciences, 19A Yuquan Road, Beijing; 100049, China

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Source :

ACS Nano

ISSN: 1936-0851

Year: 2022

Issue: 1

Volume: 16

Page: 1511-1522

1 7 . 1

JCR@2022

1 5 . 8 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:91

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 36

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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