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author:

Lu, Yongfeng (Lu, Yongfeng.) [1] | Wang, Wensong (Wang, Wensong.) [2] | Cheng, Hongrui (Cheng, Hongrui.) [3] | Qiu, Haijiang (Qiu, Haijiang.) [4] | Sun, Wenhao (Sun, Wenhao.) [5] | Fang, Xiao (Fang, Xiao.) [6] | Zhu, Jiefang (Zhu, Jiefang.) [7] | Zheng, Yuanhui (Zheng, Yuanhui.) [8]

Indexed by:

EI

Abstract:

Crystalline graphitic carbon nitride is an excellent photocatalyst for hydrogen production due to its non-toxicity, stability, elemental abundance, and visible-light response. Herein, we present a new type of composite photocatalysts, eco-friendly bamboo-charcoal-loaded graphitic carbon nitrides to accelerate the separation of electron-hole pairs. The suitable loading of bamboo charcoal on graphitic carbon nitrides shows an increased specific surface area from 85 to 120 m2 g−1, and excellent visible-light photocatalytic hydrogen production activity of 4.1 mmol g−1 h−1, which is 2.3 times higher than that of pristine carbon nitride (1.8 mmol g−1 h−1). Under irradiation, the photogenerated electrons fast migrate from graphitic carbon nitride to bamboo charcoal through an ohmic contact between them, reducing the recombination of electron-hole pairs. This study highlights the effect of carbonaceous material loading on photocatalytic activity of carbon nitrides and opens an avenue to design efficient loaded photocatalysts with natural abundant materials. © 2021 The Author(s)

Keyword:

Bamboo Carbon nitride Charcoal Electric contactors Hydrogen production Light Ohmic contacts Photocatalytic activity

Community:

  • [ 1 ] [Lu, Yongfeng]College of Chemistry, Fuzhou University, Fuzhou; 350116, China
  • [ 2 ] [Wang, Wensong]College of Chemistry, Fuzhou University, Fuzhou; 350116, China
  • [ 3 ] [Cheng, Hongrui]College of Chemistry, Fuzhou University, Fuzhou; 350116, China
  • [ 4 ] [Qiu, Haijiang]College of Chemistry, Fuzhou University, Fuzhou; 350116, China
  • [ 5 ] [Sun, Wenhao]College of Chemistry, Fuzhou University, Fuzhou; 350116, China
  • [ 6 ] [Fang, Xiao]College of Chemistry, Fuzhou University, Fuzhou; 350116, China
  • [ 7 ] [Zhu, Jiefang]Department of Chemistry - Ångstrom Laboratory, Uppsala University, Uppsala; SE-751 21, Sweden
  • [ 8 ] [Zheng, Yuanhui]College of Chemistry, Fuzhou University, Fuzhou; 350116, China
  • [ 9 ] [Zheng, Yuanhui]Fujian Science & Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou; 350116, China

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Source :

International Journal of Hydrogen Energy

ISSN: 0360-3199

Year: 2022

Issue: 6

Volume: 47

Page: 3733-3740

7 . 2

JCR@2022

8 . 1 0 0

JCR@2023

ESI HC Threshold:66

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 42

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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