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author:

Lu, Yongfeng (Lu, Yongfeng.) [1] | Wang, Wensong (Wang, Wensong.) [2] | Cheng, Hongrui (Cheng, Hongrui.) [3] | Qiu, Haijiang (Qiu, Haijiang.) [4] | Sun, Wenhao (Sun, Wenhao.) [5] | Fang, Xiao (Fang, Xiao.) [6] | Zhu, Jiefang (Zhu, Jiefang.) [7] | Zheng, Yuanhui (Zheng, Yuanhui.) [8] (Scholars:郑远辉)

Indexed by:

EI SCIE

Abstract:

Crystalline graphitic carbon nitride is an excellent photocatalyst for hydrogen production due to its non-toxicity, stability, elemental abundance, and visible-light response. Herein, we present a new type of composite photocatalysts, eco-friendly bamboo-charcoal-loaded graphitic carbon nitrides to accelerate the separation of electron-hole pairs. The suitable loading of bamboo charcoal on graphitic carbon nitrides shows an increased specific surface area from 85 to 120 m2 g-1, and excellent visible-light photocatalytic hydrogen production activity of 4.1 mmol g-1 h-1, which is 2.3 times higher than that of pristine carbon nitride (1.8 mmol g-1 h-1). Under irradiation, the photogenerated electrons fast migrate from graphitic carbon nitride to bamboo charcoal through an ohmic contact between them, reducing the recombination of electron-hole pairs. This study highlights the effect of carbonaceous material loading on photocatalytic activity of carbon nitrides and opens an avenue to design efficient loaded photocatalysts with natural abundant materials. (c) 2021 The Author(s). Published by Elsevier Ltd on behalf of Hydrogen Energy Publications LLC. This is an open access article under the CC BY license (http://creativecommons.org/ licenses/by/4.0/).

Keyword:

Bamboo-charcoal Graphitic carbon nitride Ohmic contact Photocatalytic hydrogen production

Community:

  • [ 1 ] [Lu, Yongfeng]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China
  • [ 2 ] [Wang, Wensong]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China
  • [ 3 ] [Cheng, Hongrui]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China
  • [ 4 ] [Qiu, Haijiang]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China
  • [ 5 ] [Sun, Wenhao]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China
  • [ 6 ] [Fang, Xiao]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China
  • [ 7 ] [Zheng, Yuanhui]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China
  • [ 8 ] [Zheng, Yuanhui]Fujian Sci & Technol Innovat Lab Optoelect Inform, Fuzhou 350116, Peoples R China
  • [ 9 ] [Zhu, Jiefang]Uppsala Univ, Dept Chem, Angstrom Lab, SE-75121 Uppsala, Sweden

Reprint 's Address:

  • 郑远辉

    [Zheng, Yuanhui]Fuzhou Univ, Coll Chem, Fuzhou 350116, Peoples R China;;[Zhu, Jiefang]Uppsala Univ, Dept Chem, Angstrom Lab, SE-75121 Uppsala, Sweden

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Source :

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY

ISSN: 0360-3199

Year: 2022

Issue: 6

Volume: 47

Page: 3733-3740

7 . 2

JCR@2022

8 . 1 0 0

JCR@2023

ESI Discipline: ENGINEERING;

ESI HC Threshold:66

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 35

SCOPUS Cited Count: 42

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 5

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