Charge　separation　and　transfer　are　essential　for　efficient　photocatalytic　reactions,　in　which　the　charge　carrier　dynamics　could　be　optimized　by　the　rational　design　of　composition　and　nanomorphology.　Inspired　in　nature　that　vine　can　effectively　harvest　sunlight　and　present　indomitable　vitality,　a　novel　raspberry　plant-like　ternary　heterostructure　has　been　constructed　for　the　first　time.　Its　novel　structure　originates　from　anchoring　raspberry-like　porous　Cd0.5Zn0.5S　nanosphere　on　a　highly　conductive　matrix　composited　of　MoS2　nanosheets　and　multiwall　carbon　nanotubes　(CNT).　The　ternary　CNT@MoS2/Cd0.5Zn0.5S　(C@M/CZS)　system　of　mutual　benefits　is　constructed　of　1D　CNT　as　‘stems’,　2D　MoS2　nanosheets　as　‘leaves’　and　Cd0.5Zn0.5S　nanospheres　as　‘fruits’.　The　constructed　raspberry　plant-like　C@M/CZS　heterostructure　exhibits　a　high-efficient　photocatalytic　H2　evolution　rate　of　46.23　mmol·g−1·h−1,　which　is　51.9　times　that　of　the　original　Cd0.5Zn0.5S.　It　is　found　that　the　vine-like　CNT@MoS2　matrix　and　interactive　ternary　heterostructure　are　favorable　for　effective　visible-light　absorption　and　charge　carriers’　separation-transfer-reaction,　and　thus　improving　the　photostability　and　photocatalytic　performance　of　the　biomimetic　photocatalytic　system.　©　2021　Elsevier　B.V.