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[期刊论文]

Photocatalytic hydrogen production over carbon nitride loaded with WS2 as cocatalyst under visible light

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author:

Hou, Yidong (Hou, Yidong.) [1] | Zhu, Yongsheng (Zhu, Yongsheng.) [2] | Xu, Yan (Xu, Yan.) [3] | Unfold

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EI

Abstract:

Mesoporous graphitic$ carbon nitride (mpg-CN) was loaded with WS2 via an impregnation-sulfidation approach. The resultant surface heterojunctions between WS2 and mpg-CN were evidently confirmed with transmission electron microscopy (TEM) and X-ray photoelectron spectroscopy (XPS). Photocatalytic H2 production on WS2/mpg-CN under visible light (λ>420nm) shows that WS2 plays an important role in catalyzing H2 production. The rate of hydrogen evolution reaches an optimum when the loading amount of WS2 is about 0.3at.%. Combined with the physicochemical and electrocatalytic properties of WS2/mpg-CN, it can be concluded that the enhanced photocatalytic H2 production activity on WS2/mpg-CN is mainly attributed to the thin layered junctions formed between WS2 and mpg-CN and the great performance of WS2 as a cocatalyst in H2 evolution reaction. © 2014 Elsevier B.V.

Keyword:

Carbon nitride Heterojunctions High resolution transmission electron microscopy Hydrogen production Light Nitrides Photocatalytic activity Physicochemical properties Tungsten compounds X ray photoelectron spectroscopy

Community:

  • [ 1 ] [Hou, Yidong]Research Institute of Photocatalysis, State Key Laboratory Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou 350002, China
  • [ 2 ] [Zhu, Yongsheng]Research Institute of Photocatalysis, State Key Laboratory Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou 350002, China
  • [ 3 ] [Xu, Yan]Research Institute of Photocatalysis, State Key Laboratory Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou 350002, China
  • [ 4 ] [Wang, Xinchen]Research Institute of Photocatalysis, State Key Laboratory Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou 350002, China

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Source :

Applied Catalysis B: Environmental

ISSN: 0926-3373

Year: 2014

Volume: 156-157

Page: 122-127

7 . 4 3 5

JCR@2014

2 0 . 3 0 0

JCR@2023

ESI HC Threshold:268

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count: 180

30 Days PV: 4

Affiliated Colleges:

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管理员  2024-08-24 12:34:18  更新被引

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管理员  2024-07-29 17:37:34  更新被引

管理员  2023-10-08 14:23:03  更新被引

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