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author:

Zhang, Ruding (Zhang, Ruding.) [1] | Huang, Jiajia (Huang, Jiajia.) [2] | Deng, Wenzhuo (Deng, Wenzhuo.) [3] | Bao, Jingze (Bao, Jingze.) [4] | Pan, Yilong (Pan, Yilong.) [5] | Huang, Shuping (Huang, Shuping.) [6] (Scholars:黄淑萍) | Sun, Chuan-Fu (Sun, Chuan-Fu.) [7]

Indexed by:

EI Scopus SCIE

Abstract:

A key challenge for potassium-ion batteries is to explore low-cost electrode materials that allow fast and reversible insertion of large-ionic-size K+. Here, we report an inorganic-open-framework anode (KTiOPO4), which achieves a reversible capacity of up to 102mAhg(-1) (307mAhcm(-3)), flat voltage plateaus at a safe average potential of 0.82V (vs. K/K+), a long lifespan of over 200 cycles, and K+-transport kinetics approximate to 10 times faster than those of Na-superionic conductors. Combined experimental analysis and first-principles calculations reveal a charge storage mechanism involving biphasic and solid solution reactions and a cell volume change (9.5%) even smaller than that for Li+-insertion into graphite (approximate to 10%). KTiOPO4 exhibits quasi-3D lattice expansion on K+ intercalation, enabling the disintegration of small lattice strain and thus high structural stability. The inorganic open-frameworks may open a new avenue for exploring low-cost, stable and fast-kinetic battery chemistry.

Keyword:

electrochemistry fast kinetics inorganic open-framework low strain potassium-ion batteries

Community:

  • [ 1 ] [Zhang, Ruding]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 2 ] [Deng, Wenzhuo]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 3 ] [Bao, Jingze]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 4 ] [Pan, Yilong]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 5 ] [Sun, Chuan-Fu]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China
  • [ 6 ] [Zhang, Ruding]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 7 ] [Deng, Wenzhuo]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 8 ] [Bao, Jingze]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 9 ] [Pan, Yilong]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 10 ] [Sun, Chuan-Fu]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China
  • [ 11 ] [Huang, Jiajia]Fuzhou Univ, Coll Chem, Fuzhou 350108, Fujian, Peoples R China
  • [ 12 ] [Huang, Shuping]Fuzhou Univ, Coll Chem, Fuzhou 350108, Fujian, Peoples R China

Reprint 's Address:

  • [Sun, Chuan-Fu]Chinese Acad Sci, Fujian Inst Res Struct Matter, CAS Key Lab Design & Assembly Funct Nanostruct, Fuzhou 350002, Fujian, Peoples R China;;[Sun, Chuan-Fu]Chinese Acad Sci, Fujian Inst Res Struct Matter, Fujian Key Lab Nanomat, Fuzhou 350002, Fujian, Peoples R China

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Source :

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION

ISSN: 1433-7851

Year: 2019

Issue: 46

Volume: 58

Page: 16474-16479

1 2 . 9 5 9

JCR@2019

1 6 . 1 0 0

JCR@2023

ESI Discipline: CHEMISTRY;

ESI HC Threshold:184

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 62

SCOPUS Cited Count: 57

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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