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[期刊论文]

Silicon-Based 3D All-Solid-State Micro-Supercapacitor with Superior Performance

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author:

Wang, Yurong (Wang, Yurong.) [1] | Sun, Leimeng (Sun, Leimeng.) [2] | Xiao, Dongyang (Xiao, Dongyang.) [3] | Unfold

Indexed by:

Scopus SCIE

Abstract:

The large-scale fabrication of high-performance on-chip micro-supercapacitors (MSCs) is the footstone for the development of next-generation miniaturized electronic devices. In practical applications, however, MSCs may suffer from a low areal energy density as well as a complicated fabrication strategy that is incompatible with semiconductor processing technology. Herein, we propose a scalable fabrication strategy for the realization of a silicon-based three-dimensional (3D) all-solid-state MSC via the combination of semiconductor-based electrode processing, chemical vapor deposition, and hydrothermal growth. The individual Si/C/MnO2 electrode shows a maximum specific capacitance of 223.74 mF cm(-2), while the symmetric electrodes present a maximum areal energy density of 5.01 mu Wh cm(-2) at the scan rate of 1 mV s(-1). The full 3D Si/C/MnO2 MSC delivers a high energy density of 2.62 mu Wh cm(-2), at a power density of 117.82 mu W cm(-2), as well as a long cycle life with capacitance retention >92% after 4000 cycles. Our proposed method enables the fabrication of 3D MSCs based on a thick silicon interdigitated electrode array, holding a great promise for the development of 3D on-chip microscale energy storage devices.

Keyword:

AC filter all-solid-state deep reactive ion etching micro-supercapacitor on-chip device

Community:

  • [ 1 ] [Wang, Yurong]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 2 ] [Sun, Leimeng]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 3 ] [Xiao, Dongyang]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 4 ] [Du, Huanhuan]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 5 ] [Yang, Zhenting]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 6 ] [Tu, Liangcheng]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 7 ] [Zhao, Chun]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 8 ] [Hu, Fangjing]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China
  • [ 9 ] [Wang, Yurong]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 10 ] [Sun, Leimeng]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 11 ] [Xiao, Dongyang]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 12 ] [Du, Huanhuan]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 13 ] [Yang, Zhenting]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 14 ] [Tu, Liangcheng]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 15 ] [Zhao, Chun]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 16 ] [Hu, Fangjing]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China
  • [ 17 ] [Wang, Yurong]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 18 ] [Sun, Leimeng]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 19 ] [Xiao, Dongyang]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 20 ] [Du, Huanhuan]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 21 ] [Yang, Zhenting]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 22 ] [Tu, Liangcheng]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 23 ] [Zhao, Chun]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 24 ] [Hu, Fangjing]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
  • [ 25 ] [Wang, Xinghui]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China
  • [ 26 ] [Lu, Bingan]Hunan Univ, Sch Phys & Elect, Changsha 410082, Peoples R China

Reprint 's Address:

  • 王星辉

    [Sun, Leimeng]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China;;[Hu, Fangjing]Huazhong Univ Sci & Technol, MOE Key Lab Fundamental Phys Quant Measurement, Wuhan 430074, Peoples R China;;[Sun, Leimeng]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China;;[Hu, Fangjing]Huazhong Univ Sci & Technol, PGMF, Hubei Key Lab Gravitat & Quantum Phys, Wuhan 430074, Peoples R China;;[Sun, Leimeng]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China;;[Hu, Fangjing]Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China;;[Wang, Xinghui]Fuzhou Univ, Coll Phys & Informat Engn, Inst Micronano Devices & Solar Cells, Fuzhou 350108, Peoples R China;;[Lu, Bingan]Hunan Univ, Sch Phys & Elect, Changsha 410082, Peoples R China

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Version:

Source :

ACS APPLIED MATERIALS & INTERFACES

ISSN: 1944-8244

Year: 2020

Issue: 39

Volume: 12

Page: 43864-43875

9 . 2 2 9

JCR@2020

8 . 5 0 0

JCR@2023

ESI Discipline: MATERIALS SCIENCE;

ESI HC Threshold:196

JCR Journal Grade:1

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count: 53

SCOPUS Cited Count: 56

30 Days PV: 0

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