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学者姓名：蔡伟龙
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Abstract ：
Alkaline water electrolysis is one of the most prospective technologies for large-scale production of green hydrogen. Nevertheless, current porous membranes face the problem of weak ion transport or poor gas barrier performance. Here, we demonstrate a facile yet massive two-step casting and phase separation strategy to design a thin, asymmetric pore-structure modulated composite membrane for efficient, safe, and industrial-grade alkaline water electrolysis. The prepared composite membrane shows better electrolytic performance (1.71 V at 1 A cm-2) and stability (working for 6352 h). In addition, an industrial-grade electrolyzer equipped with composite membranes exhibits higher hydrogen production efficiency (1.03 Nm3h-1), H2 purity (99.9%), and faster dynamic response (less than 20 min) compared to mainstream commercial membranes. Ultimately, we propose a semi-empirical model based on the operational characteristics of an electrolyzer equipped with composite membranes and predicting its matching behavior with dynamic renewable energy sources. This work explores the viability of manufacturing high-performance alkaline water electrolysis membranes for green hydrogen production under industrial conditions.
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| GB/T 7714 | You, Jian , Lu, Jinyu , Liu, Chuanli et al. A rationally thin composite membrane with differentiated pore structure for industrial-scale alkaline water electrolysis [J]. | NATURE COMMUNICATIONS , 2025 , 16 (1) . |
| MLA | You, Jian et al. "A rationally thin composite membrane with differentiated pore structure for industrial-scale alkaline water electrolysis" . | NATURE COMMUNICATIONS 16 . 1 (2025) . |
| APA | You, Jian , Lu, Jinyu , Liu, Chuanli , Wang, Wei , Li, Yongzhao , Gao, Yuanzhong et al. A rationally thin composite membrane with differentiated pore structure for industrial-scale alkaline water electrolysis . | NATURE COMMUNICATIONS , 2025 , 16 (1) . |
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Phytate (PhA) holds considerable promise for constructing molecular sieve membranes due to its high density of long-range electrostatic attractions, customizable charge density, and excellent polymer affinity. Herein, PhA-Fe3+ complexes constructed by controllable coordination assembly are presented, based on metal-organophosphorus biphasic interfacial coordination reactions, and use the PhA-Fe3+ complexes to regulate the interfacial polymerization (IP) process to generate polyamide (PA) nanofiltration membranes. The PhA-Fe3+ complexes impart a high density of long-range electrostatic and short-range hydrogen bonding forces to the amine monomers and provide tunable charge densities through flexible metal-organophosphate coordination. Hydrogen bonding and strong electrostatic interactions spatially enrich the amine monomers and temporally slow down their diffusion into the hexane phase, as demonstrated by molecular simulations, resulting in a PA/PhA-Fe3+ membrane with increased surface area, enhanced microporosity, lower thickness, higher water density near pores, and nanoscale spotted structures. Those structures are recognized as the key factor in achieving a water permeance of 19.2 L m(-2) h(-1) bar(-1), alongside a MgCl2 rejection of 96.7% and a Li+/Mg2+ selectivity of 24.1 (Mg2+/Li+ mass ratio = 20), surpassing those of reported nanofiltration membranes. This PhA-Fe(3+ )complexes-modulated IP strategy offers fresh perspectives for constructing a highly permeable membrane for lithium extraction from salt lake brines.
Keyword ：
electrostatic attraction electrostatic attraction Li+/Mg2+ selectivity Li+/Mg2+ selectivity metal-organophosphate coordination metal-organophosphate coordination nanofiltration nanofiltration phytate phytate
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| GB/T 7714 | Lai, Xing , Xu, Weiye , Gou, Yukui et al. An Electrostatic-Interaction Engineering on Phytate-Coordinated Polyamide Membranes for High-Efficiency Lithium Extraction [J]. | ADVANCED FUNCTIONAL MATERIALS , 2025 . |
| MLA | Lai, Xing et al. "An Electrostatic-Interaction Engineering on Phytate-Coordinated Polyamide Membranes for High-Efficiency Lithium Extraction" . | ADVANCED FUNCTIONAL MATERIALS (2025) . |
| APA | Lai, Xing , Xu, Weiye , Gou, Yukui , Zhang, Hongxiang , Huang, Jianying , Cai, Weilong et al. An Electrostatic-Interaction Engineering on Phytate-Coordinated Polyamide Membranes for High-Efficiency Lithium Extraction . | ADVANCED FUNCTIONAL MATERIALS , 2025 . |
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Layered bismuth-rich oxyhalides exhibit broad light absorption and high electron-hole separation efficiency. However, their photocatalytic performance remains limited by high recombination rates, resulting in low quantum efficiency. These challenges in interfacial charge separation can be effectively addressed through the strategic design of heterojunctions and the introduction of surface defects. In this study, a novel Z-scheme Bi24O31Cl10/BiPO4 (Bi-24-P) photocatalyst was synthesized using a straightforward stirring method, incorporating PO43- to enhance photocatalytic degradation efficiency. The effects of various preparation conditions and application scenarios on the photocatalytic activity of Bi-24-P were systematically investigated. Under visible light irradiation, the optimized Bi-24-P photocatalyst (0.1 g/L dosage) achieved an 82.30 % degradation rate for 50 mL of 20 mg/L tetracycline (TC) within 2 h, with a pseudo-first-order reaction rate constant twice that of Bi-24 alone. The Bi-24-P catalyst also demonstrated exceptional salt tolerance, reusability, versatility, and broad spectral response. Mechanistic studies utilizing photoelectric measurements, density functional theory (DFT) analysis, and scavenger experiments revealed that the enhanced degradation performance is primarily attributed to the synergistic coupling of semiconductor interfaces and oxygen vacancies within the composite catalyst. This structure facilitates the formation of a Z-scheme heterojunction, optimizing internal electron transfer pathways. Additionally, toxicity assessments confirmed a significant reduction in water toxicity after photodegradation. These findings offer valuable insights for the development of BixOyClz-based catalysts to address the challenges of antibiotic-contaminated wastewater treatment.
Keyword ：
Antibiotic degradation Antibiotic degradation Bi24O31Cl10 Bi24O31Cl10 BiPO4 BiPO4 Oxygen vacancies Oxygen vacancies Z-scheme heterojunction Z-scheme heterojunction
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| GB/T 7714 | Lu, Tianyu , Meng, Zheyi , Zhu, Liping et al. Enhanced antibiotic photodegradation by Bi24O31Cl10/BiPO4 Z-scheme photocatalyst: DFT calculation, photocatalytic mechanism insight and toxicity evolution [J]. | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 74 . |
| MLA | Lu, Tianyu et al. "Enhanced antibiotic photodegradation by Bi24O31Cl10/BiPO4 Z-scheme photocatalyst: DFT calculation, photocatalytic mechanism insight and toxicity evolution" . | JOURNAL OF WATER PROCESS ENGINEERING 74 (2025) . |
| APA | Lu, Tianyu , Meng, Zheyi , Zhu, Liping , Cai, Weilong , Zhu, Meifang . Enhanced antibiotic photodegradation by Bi24O31Cl10/BiPO4 Z-scheme photocatalyst: DFT calculation, photocatalytic mechanism insight and toxicity evolution . | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 74 . |
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As the raw material for fabricating polyphenylene sulfide (PPS) fibers, PPS resin exhibits great processing and application value. However, the oxidative cross-linking among PPS molecules at high temperatures causes increasing melt viscosity and decreasing fluidity, making PPS processing difficult and lower production quality and efficiency. In this research, we realize the dual improvement of PPS resin in the fluidity and oxidation resistance by introducing a new AO-g-C3N4 composite modifier. First, an antioxidant (AO) was grafted onto the surface of graphitic carbon nitride (g-C3N4) through amination to synthesize AO-g-C3N4. Subsequently, AO-g-C3N4 was incorporated into PPS resin using the melt extrusion process, yielding a novel flow-enhancing and antioxidant PPS-based composite material. It is found that the AO-g-C3N4/PPS material possesses excellent properties with a significantly raised melt index (>50 %) and notably decreased shear viscosity (>20 %). Besides, the dynamic oxidation induction temperature of AO-g-C3N4/PPS has increased, indicating inhibited oxidative cross-linking, while the crystallinity has increased. These suggest that the incorporation of AO-g-C3N4 into PPS resin can enhance its fluidity and antioxidation properties, providing valuable insight for the modification research of PPS resin. The AO-g-C3N4/PPS exhibits the characteristic of easier processing, which offers promising prospects for developing the downstream industry of PPS resin.
Keyword ：
Antioxidant (AO) Antioxidant (AO) Flow-antioxidation Flow-antioxidation Graphitic carbon nitride (g-C3N4) Graphitic carbon nitride (g-C3N4) Melt blending Melt blending Polyphenylene sulfide (PPS) Polyphenylene sulfide (PPS)
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| GB/T 7714 | Wang, Wei , Cao, Hong , You, Jian et al. Dual synergistic effects of novel modifier AO-g-C3N4 on the fluidity and oxidation resistance for high performance PPS resin [J]. | COMPOSITES COMMUNICATIONS , 2025 , 57 . |
| MLA | Wang, Wei et al. "Dual synergistic effects of novel modifier AO-g-C3N4 on the fluidity and oxidation resistance for high performance PPS resin" . | COMPOSITES COMMUNICATIONS 57 (2025) . |
| APA | Wang, Wei , Cao, Hong , You, Jian , Li, Yongzhao , Yu, Weihe , Chen, Huaiyin et al. Dual synergistic effects of novel modifier AO-g-C3N4 on the fluidity and oxidation resistance for high performance PPS resin . | COMPOSITES COMMUNICATIONS , 2025 , 57 . |
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Highly permeable polyamide (PA) membranes with precise ion selection can be used for many energy-efficient chemical separations but are limited by membrane inefficiencies. Herein, polyphenol-mediated ZIF-8 nano- particles with hydroxyl-rich hollow structure were synthesized by tannic acid tailored regulation. PA-based membranes with fast penetration, high retention, and precise Cl-/SO42- selection were then synthesized through spatially and temporally controlling interfacial polymerization with modified ZIF-8 nanoparticles (tZIF8) as aqueous phase additives or as interlayers. The effects of the embedding position of tZIF-8 on the structure, morphology, physicochemical properties, and performance of PA-based membranes were explored through a sequence of characterization techniques. The results revealed that the PA-based membrane with tZIF-8 embedded in the PA layer could achieve a high water permeance of 24.8 L m- 2 h- 1 bar- 1 with a high retention of 99.4 % Na2SO4 and a Cl-/SO42- selectivity of 141, which was superior to most state-of-the-art PA-based membranes. Comparatively, the Cl-/SO42- selection of the PA-based membrane with tZIF-8 embedded between the PA layer and the substrate was 136, while the water permeance was slightly enhanced to 28.2 L m- 2 h- 1 bar- 1 . Excitingly, the resulting membranes all exhibit superior antifouling properties and stability. Our facile strategy for tuning membrane microstructures provides new ideals into the development of highly permeable and excellently selective PA-based membranes for precise ion sieving.
Keyword ：
Different embedding positions Different embedding positions Interfacial polymerization Interfacial polymerization Ion sieving Ion sieving Nanoparticles Nanoparticles Spatial-temporal regulation Spatial-temporal regulation
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| GB/T 7714 | Lai, Xing , Zhang, Hongxiang , Xu, Weiye et al. Polyamide membranes with tannic acid-ZIF-8 for highly permeable and selective ion-ion separation [J]. | JOURNAL OF MEMBRANE SCIENCE , 2025 , 714 . |
| MLA | Lai, Xing et al. "Polyamide membranes with tannic acid-ZIF-8 for highly permeable and selective ion-ion separation" . | JOURNAL OF MEMBRANE SCIENCE 714 (2025) . |
| APA | Lai, Xing , Zhang, Hongxiang , Xu, Weiye , You, Jian , Chen, Huaiyin , Li, Yongzhao et al. Polyamide membranes with tannic acid-ZIF-8 for highly permeable and selective ion-ion separation . | JOURNAL OF MEMBRANE SCIENCE , 2025 , 714 . |
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The growing complexity of dyeing and printing effluents has presented considerable challenges for their effective treatment and recycling. Recently, there has been a notable increase in the development of loose nanofiltration (NF) membranes, which are characterised by their exceptional environmental resilience, high throughput, and superior dye/salt selectivity. This work presents the development of a new loose NF membrane prepared from a modified polymer called poly(ether sulfone ether ketone ketone) (PESEKK). The membrane features a dense- loose-support structure and is prepared through a straightforward one-step, non-solvent induced phase separation (NIPS) technique, eliminating the need for heating or post-treatment. Precise regulation of membrane pore size down to 4.27 nm can be achieved through modulation of PESEKK and pore-former composition. The membranes could separate positively and negatively charged dyes in mixed dye solutions accurately and selectively. Additionally, the membrane demonstrated exceptional dye/salt selective separation with a high water flux of 230.7 L m- 2 h- 1 bar- 1 , Congo red rejection of 99.91 +/- 0.13 %, NaCl rejection of 2.71 +/- 0.23 %, and a separation factor (alpha) of 347.4, outperforming state-of-the-art membranes. Remarkably, PESEKK membrane maintained outstanding stability and separation performance for up to 200 h under extreme environments, including NaOH solution (up to 9 mol L-1), NaClO solution (up to 40,000 mg L-1 h), n-hexane, isopropanol, and methanol. This high-performing loose NF membrane, developed using innovative polymer materials, offers a promising solution for treating the challenging wastewater generated by printing and dyeing processes.
Keyword ：
Dense-loose-supporting structure Dense-loose-supporting structure Dye/salt separation Dye/salt separation Loose nanofiltration Loose nanofiltration Non-solvent induced phase separation Non-solvent induced phase separation Poly(ether sulfone ether ketone ketone) Poly(ether sulfone ether ketone ketone)
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| GB/T 7714 | Zhang, Hongxiang , Lai, Xing , You, Jian et al. Facile construction of novel poly(ether sulfone ether ketone ketone) loose nanofiltration membrane for efficient dye/salt separation [J]. | DESALINATION , 2025 , 601 . |
| MLA | Zhang, Hongxiang et al. "Facile construction of novel poly(ether sulfone ether ketone ketone) loose nanofiltration membrane for efficient dye/salt separation" . | DESALINATION 601 (2025) . |
| APA | Zhang, Hongxiang , Lai, Xing , You, Jian , Wang, Wei , Wu, Meihua , Liu, Longmin et al. Facile construction of novel poly(ether sulfone ether ketone ketone) loose nanofiltration membrane for efficient dye/salt separation . | DESALINATION , 2025 , 601 . |
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Green hydrogen is currently the dominant trend in the evolution of hydrogen energy, producing almost no greenhouse gas emissions. Alkaline water electrolysis (AWE) is recognized as a leading and well-established technology for producing green hydrogen. However, safety hazards may occur during hydrogen production currently as defective commercial separate membranes used in the AWE process. Therefore, it is imperative to create a membrane characterized by low area resistance, high stability, and high bubble point pressure (BPP) to realize high-performance AWE. Herein, we synthesize alumina-based composite membranes with Y2O3-added and polyethylene glycol coupling agent functionalized Al2O3 for AWE through a phase inversion method. The porous composite membrane exhibits excellent hydrophilicity, with a lower contact angle of approximately 55 degrees. It also presents exceptional performance metrics, including a low area resistance of about 0.17 Omega cm(2), an ultrahigh BBP of approximately 4.4 bar, and excellent mechanical properties with a tensile strength of around 25 MPa. The membranes achieved a current density of up to 2.5 A cm(-2) under 2.0 V voltage in a 30 wt% KOH solution at 80 degrees C by utilizing commercial catalysts. Notably, the composite membranes exhibited remarkable stability, maintaining operation for over 1200 h at a 2.0 A cm(-2) current density without any performance degradation at 80 degrees C. Furthermore, this composite membrane possesses outstanding gas-barrier capability with H-2 and O-2 purity higher than 98.70 % and 99.69 %, respectively. The above results demonstrate that the prepared novel high-performance alumina-based composite membrane for hydrogen generation has significant potential for applications within the AWE process.
Keyword ：
Alkaline water electrolysis Alkaline water electrolysis Composite membrane Composite membrane Functionalized alumina Functionalized alumina High current density High current density Hydrophilicity Hydrophilicity
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| GB/T 7714 | Lu, Jinyu , You, Jian , Chang, Ben et al. Polyethylene glycol functionalized alumina-based composite membrane with high-performance for alkaline water electrolysis [J]. | JOURNAL OF MEMBRANE SCIENCE , 2025 , 725 . |
| MLA | Lu, Jinyu et al. "Polyethylene glycol functionalized alumina-based composite membrane with high-performance for alkaline water electrolysis" . | JOURNAL OF MEMBRANE SCIENCE 725 (2025) . |
| APA | Lu, Jinyu , You, Jian , Chang, Ben , Wang, Wei , Li, Yongzhao , Lin, Jiabin et al. Polyethylene glycol functionalized alumina-based composite membrane with high-performance for alkaline water electrolysis . | JOURNAL OF MEMBRANE SCIENCE , 2025 , 725 . |
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Thermochromic smart windows offer energy-saving potential through temperature-responsive optical transmittance adjustments, yet face challenges in achieving anti-UV radiation, fast response, and high-temperature stability characteristics for long-term use. Herein, the rational design of Hofmeister effect-enhanced, nanoparticle-shielded composite hydrogels, composed of hydroxypropylmethylcellulose (HPMC), poly(N,N-dimethylacrylamide) (PDMAA), sodium sulfate, and polydopamine nanoparticles, for anti-UV, fast-response, and all-day-modulated smart windows is reported. Specifically, a three-dimensional network of PDMAA is created as the supporting skeleton, markedly enhancing the thermal stability of pristine HPMC hydrogels. Sodium sulfate induces a Hofmeister effect, lowering the lower critical solution temperature to 32 degrees C while accelerating phase transition rates fivefold (30 s vs. 150 s). Intriguingly, small-sized polydopamine nanoparticles simultaneously enable high luminous transmittance of 66.9% and outstanding anti-UV capability. Additionally, the smart window showcases a high solar modulation (51.2%) and maintains a 10.2 degrees C temperature reduction versus a glass window during all-day modulation applications. The design strategy is effective, opening up new avenues for manufacturing fast-response and durable thermochromic smart windows for energy savings and emission reduction.
Keyword ：
anti-UV anti-UV hydroxypropylmethylcellulose hydroxypropylmethylcellulose phase change rate phase change rate smart window smart window thermal stability thermal stability thermochromism thermochromism
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| GB/T 7714 | Wang, Kai , Liu, Shuzhi , Yu, Jiahui et al. Hofmeister Effect-Enhanced, Nanoparticle-Shielded, Thermally Stable Hydrogels for Anti-UV, Fast-Response, and All-Day-Modulated Smart Windows [J]. | ADVANCED MATERIALS , 2025 , 37 (14) . |
| MLA | Wang, Kai et al. "Hofmeister Effect-Enhanced, Nanoparticle-Shielded, Thermally Stable Hydrogels for Anti-UV, Fast-Response, and All-Day-Modulated Smart Windows" . | ADVANCED MATERIALS 37 . 14 (2025) . |
| APA | Wang, Kai , Liu, Shuzhi , Yu, Jiahui , Hong, Peixin , Wang, Wenyi , Cai, Weilong et al. Hofmeister Effect-Enhanced, Nanoparticle-Shielded, Thermally Stable Hydrogels for Anti-UV, Fast-Response, and All-Day-Modulated Smart Windows . | ADVANCED MATERIALS , 2025 , 37 (14) . |
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The filter material is the key to controlling flue gas pollution with bag filter technology. Surface treatment of filter media using the PTFE membrane can improve its filtration performance. Badly, the reprocessing of used filter media has become a major challenge due to the ecological impact and potential human toxicity of PTFE. Herein, a novel PPS-based gradient filtration material (mPPS-25/NF-5) with high efficiency, low resistance, and controllability was prepared by combining numerical simulation, high-temperature melt-blown process, and lamination technology with PPS micronano-embedded fiber membranes (mPPS) as the surface layer structure. Benefiting from the three-dimensional porous network structure formed by the staggered arrangement of fibers in mPPS and the effective prediction and optimization of the structural performance of the designed filter media in advance, mPPS-25/NF-5 demonstrated superior filtration performance. Specifically, compared with commercial PTFE membrane lamination filter media, the average cleaning cycle of mPPS-25/NF-5 has been improved by 188.13 s, while the average residual resistance has been reduced by 41.84 Pa, which truly realizes a high efficiency, low resistance, and long service life. This work may offer fresh insight into new materials and their rapid and controllable production methods for flue gas purification under "ultralow emission" measures.
Keyword ：
bag filter bag filter cleaning performance cleaning performance gas pollution gas pollution gradient filtration material gradient filtration material numerical simulation numerical simulation PPS micronano-embedded fiber membrane PPS micronano-embedded fiber membrane PTFE microporousmembrane PTFE microporousmembrane
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| GB/T 7714 | You, Jian , Zhang, Hongxiang , Li, Yongzhao et al. PPS Gradient Filter Material with High Efficiency and Excellent Dust Removal Capacity for Industrial Flue Gas Treatment by Integrating Numerical Modeling and Melt-Blown-Lamination Technology [J]. | ENVIRONMENTAL SCIENCE & TECHNOLOGY , 2025 , 59 (21) : 10368-10379 . |
| MLA | You, Jian et al. "PPS Gradient Filter Material with High Efficiency and Excellent Dust Removal Capacity for Industrial Flue Gas Treatment by Integrating Numerical Modeling and Melt-Blown-Lamination Technology" . | ENVIRONMENTAL SCIENCE & TECHNOLOGY 59 . 21 (2025) : 10368-10379 . |
| APA | You, Jian , Zhang, Hongxiang , Li, Yongzhao , Wang, Wei , Liu, Longmin , Chen, Huaiyin et al. PPS Gradient Filter Material with High Efficiency and Excellent Dust Removal Capacity for Industrial Flue Gas Treatment by Integrating Numerical Modeling and Melt-Blown-Lamination Technology . | ENVIRONMENTAL SCIENCE & TECHNOLOGY , 2025 , 59 (21) , 10368-10379 . |
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Particulate emissions from high temperature pose a significant threat to air quality, necessitating advanced air filtration materials capable of withstanding extreme temperatures and complex environmental conditions. Here, we report a high-efficiency and high-temperature resistant polyimide/SiO2 (PI/SiO2) nanofiber membrane with excellent air permeability (146 mm/s) and electrostatic effects (-1500 V), fabricated via multi-needle electrospinning followed by thermal imidization. Interface regulation through SiO2 incorporation enhances the membrane's permeability by expanding fiber spacing and increasing tortuosity, thereby prolonging particle-fiber collision time and improving passive filtration performance. The PI/SiO2 fibers also generate self-sustained electrostatic charges through friction with air and inter-fiber contact, imparting active filtration capability. By controlling and increasing the SiO2 content at a constant spinning amount, a balance between filtration efficiency and pressure drop was achieved through enhanced air permeability. Under continuous filtration at 260 degrees C for 240 min, the membrane exhibited exceptional PM0.3 filtration efficiency (99.1668 %) with a modest pressure drop (109 Pa). Furthermore, by integrating electrospun membranes with filter bags and conducting industrial dust simulations, it achieved an ultrahigh filtration efficiency of 99.9993 % with a pressure drop of only 133 Pa. The successful development of PI/SiO2 nanofiber membranes provides a promising strategy for next-generation high-temperature-resistant air filters.
Keyword ：
Air permeability Air permeability Electrostatic effect Electrostatic effect High temperature High temperature PI/SiO2 nanofiber membrane PI/SiO2 nanofiber membrane PM filtration PM filtration
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| GB/T 7714 | Lu, Nan , Yi, Mengtong , Wu, Zuheng et al. Versatile high-temperature air purification with durable, breathable electrostatic filters for ultra-efficient particle capture [J]. | JOURNAL OF MEMBRANE SCIENCE , 2025 , 734 . |
| MLA | Lu, Nan et al. "Versatile high-temperature air purification with durable, breathable electrostatic filters for ultra-efficient particle capture" . | JOURNAL OF MEMBRANE SCIENCE 734 (2025) . |
| APA | Lu, Nan , Yi, Mengtong , Wu, Zuheng , Yang, Yuchen , Gou, Yukui , He, Shaofan et al. Versatile high-temperature air purification with durable, breathable electrostatic filters for ultra-efficient particle capture . | JOURNAL OF MEMBRANE SCIENCE , 2025 , 734 . |
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