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学者姓名：肖高
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Abstract ：
农林生物质废弃物作为一种价廉易得的可再生资源,具有丰富的碳源和多孔通道优势.其通过炭化和活化等制备方法及其他复合改性方法可得到具有优良性能的新型多孔材料,该材料在储能方面具有广阔的应用前景.特别是在锂离子电池中的应用方面,生物质衍生多孔碳具备可提高电池的循环性能、容量和倍率性能等优势.该文对基于生物质构建锂离子电池负极材料的应用现状进行了总结,主要介绍了稻壳、玉米秸秆、棉花和果壳等生物质衍生多孔碳应用于锂离子电池负极的电化学性能,并探讨了目前生物质基负极材料存在的问题.另外,还讨论了未来生物质在储能领域的研究方向和应用前景,为化工新型碳材料和锂离子电池的可持续发展提供了新途径和新思路.
Keyword ：
农林废弃物 农林废弃物 应用方向 应用方向 生物质衍生多孔碳 生物质衍生多孔碳 负极材料 负极材料 锂离子电池 锂离子电池
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| GB/T 7714 | 肖高 , 郑明珠 , 毛诗钰 et al. 农林生物质衍生多孔碳构筑锂电池负极新材料 [J]. | 精细化工 , 2025 , 42 (2) : 233-243 . |
| MLA | 肖高 et al. "农林生物质衍生多孔碳构筑锂电池负极新材料" . | 精细化工 42 . 2 (2025) : 233-243 . |
| APA | 肖高 , 郑明珠 , 毛诗钰 , 李晓慧 . 农林生物质衍生多孔碳构筑锂电池负极新材料 . | 精细化工 , 2025 , 42 (2) , 233-243 . |
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Transforming spent coffee grounds and tea residues into valuable hierarchical porous materials presents a sustainable solution for environmental remediation due to the low cost, extensive availability, and versatile functionalized interface. Here, we systematically investigated tea polyphenol-mediated morphological transformation of spent coffee grounds to the synthesis of three-dimensional (3D) mesoporous metal-organic framework (MOF)-derived nanoarchitectured carbon composites. We adopted the sustainable cost-effective tea-coffee derivative to remove typical marine micropollutants, such as antibiotic wastewater, radioactive pollutants, and microplastics. This innovative adsorbent shows remarkable efficiency in antibiotic adsorption, achieving up to 99.62% removal of tetracycline (TC), with an impressive maximum adsorption capacity of 373.1 mg/g. It also demonstrates a remarkable ability to remove marine microplastics and radioactive pollutants with immediate nuclear threats and global sanitation and health crisis posed by Fukushima nuclear waste toward the world. The innovative strategy of treating waste with waste highlights economic potential in wastewater treatment.
Keyword ：
Fukushima nuclear waste uranium Fukushima nuclear waste uranium Metal-organicframeworks (MOFs) Metal-organicframeworks (MOFs) Microplastics Microplastics Spent coffee grounds Spent coffee grounds Sustainable marine micropollutant mitigation Sustainable marine micropollutant mitigation Tea residues Tea residues
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| GB/T 7714 | Xiao, Gao , Guo, Junling , Zheng, Mingzhu et al. Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater [J]. | NANO LETTERS , 2024 , 24 (49) : 15509-15516 . |
| MLA | Xiao, Gao et al. "Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater" . | NANO LETTERS 24 . 49 (2024) : 15509-15516 . |
| APA | Xiao, Gao , Guo, Junling , Zheng, Mingzhu , Zhang, Jun , Chen, Liyin , Dai, Manna et al. Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater . | NANO LETTERS , 2024 , 24 (49) , 15509-15516 . |
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Conductive hydrogels have shown a great potential in the field of flexible electronics. However, it is difficult to combine high strength and high toughness in conductive hydrogels prepared by conventional methods, which limits their applications in various fields. In this work, we pioneered a facile and cost-effective strategy to prepare soy protein isolate/poly(vinyl alcohol) (SPI/PVA) conductive hydrogels with high strength, toughness, low- temperature resistance, and recyclability by introducing all the salts into the prescuor solution directly. To solve the problem of unable to directly introducing high concentration Na3Cit into the soy protein isolate/PVA solution, MgCl2 was used to alleviate the strong salting-out effect of Na3Cit. Thus the stable SPI/PVA/EG/MgCl2/ Na3Cit complex solution was obtained and the SPI/PVA/EG/MgCl2/Na3Cit (SPEMS) organohydrogel was prepared by the freezing/thawing process. The optimum tensile strength of the SPEMS organohydrogel was 1.1 +0.07 MPa, and the elongation at break was 701.3+23.67 %, respectively. Meanwhile, the ionic conductivity of the organohydrogel was as high as 1.7+0.01 S/m. Finally, the EG/H2O binary solvent system endowed the organohydrogel with excellent low-temperature resistance (freezing point of-19.4 degrees C). The strain sensors assembled with SPEMS organohydrogels were characterized by high sensitivity (GF = 3.2, strain range from 20 %-500 %) and long-term stability. The flexible all-solid-state supercapacitor assembled with SPEMS organohydrogel as the electrolyte and activated carbon as the electrodes has a high area specific capacitance (113.76 mF/cm2) and good cycling stability (capacitance retention of 81.62 % after 1,000 charging and discharging cycles) at room temperature.
Keyword ：
Hofmeister effect Hofmeister effect One-pot preparation One-pot preparation Poly(vinyl alcohol) Poly(vinyl alcohol) Soy protein isolate Soy protein isolate Strain sensor Strain sensor
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| GB/T 7714 | Hu, Mingqiang , Deng, Yingxue , Qian, Xing et al. One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices [J]. | EUROPEAN POLYMER JOURNAL , 2024 , 221 . |
| MLA | Hu, Mingqiang et al. "One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices" . | EUROPEAN POLYMER JOURNAL 221 (2024) . |
| APA | Hu, Mingqiang , Deng, Yingxue , Qian, Xing , Ye, Dezhan , Jiang, Xiancai , Xiao, Gao . One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices . | EUROPEAN POLYMER JOURNAL , 2024 , 221 . |
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The use of hydrogel-based interfacial solar evaporators for desalination is a green, sustainable, and extremely concerned freshwater acquisition strategy. However, developing evaporators that are easy to manufacture, cheap, and have excellent porous structures still remains a considerable challenge. This work proposes a novel strategy for preparing a self-assembling sponge-like poly(vinyl alcohol)/graphite composite hydrogel based on the Hofmeister effect for the first time. The sponge-like hydrogel interfacial solar evaporator (PGCNG) is successfully obtained after combining with graphite. The whole process is environmental-friendly and of low-carbon free of freezing process. The PGCNG can be conventionally dried and stored. PGCNG shows impressive water storage performance and water transmission capacity, excellent steam generation performance and salt resistance. PGCNG has a high evaporation rate of 3.5 kg m-2 h-1 under 1 kW m-2 h-1 solar irradiation and PGCNG demonstrates stable evaporation performance over both 10 h of continuous brine evaporation and 30 cycles of brine evaporation. Its excellent performance and simple, scalable preparation strategy make it a valuable material for practical interface solar seawater desalination devices. This paper presents a novel and facile method for obtaining a sponge-like hydrogel with excellent pore structure, outstanding water transport and solar interfacial evaporation performance. The method is based on the Hofmeister effect, whereby the polymer nanofibers are coiled by a combination of salting and salting effects, resulting in the formation of a pore structure. image
Keyword ：
desalination desalination hofmeister effect hofmeister effect phase separation phase separation porous hydrogels porous hydrogels solar steam generation solar steam generation
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| GB/T 7714 | Yang, Mohan , Wu, Yaowei , Chen, Mengdie et al. Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation [J]. | SMALL , 2024 , 20 (43) . |
| MLA | Yang, Mohan et al. "Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation" . | SMALL 20 . 43 (2024) . |
| APA | Yang, Mohan , Wu, Yaowei , Chen, Mengdie , Wang, Yuhao , Zhang, Lei , Deng, Yingxue et al. Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation . | SMALL , 2024 , 20 (43) . |
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Glioma, in which a malignant tumor cell occurs in neural mesenchymal cells, has a rapid progression and poor prognosis, which is still far from desirable in clinical treatments. We developed a lab-on-a-chip (LOC) device for the rapid and efficient preparation of vitexin/indocyanine green (ICG) liposomes. Vitexin could be released from liposome to kill cancer cell, which can potentially improve the glioma therapeutic effect and reduce the treatment time through synergistic photodynamic/photothermal therapies (PDT/PTT). The vitexin/ICG liposome was fabricated via LOC and its physicochemical property and release in vitro were evaluated. 3-(4,5-Dimethylthiazol-2-yl)-2,5-diphenyltetrazolium bromide (MTT) method and live/dead staining were used to examine the enhanced antitumor effect of vitexin/ICG liposome in cooperation with PDT/PTT, while the related mechanism was explored by flow cytometry and western blot. The results were as follows: (1) The prepared vitexin/ICG liposome was smaller in size, homogenous in particle size distribution with significant low polydispersity index (PDI), and enhanced cumulative release in vitro. (2) We found that the formulated liposome presented strong cancer cell inhibition and suppression of its migration in a dose-dependent manner. (3) Further mechanistic studies showed that liposome combined with near-infrared irradiation could significantly upregulate levels of B cell lymphoma 2-associated X (Bax) protein and decrease B cell lymphoma 2 (Bcl-2) at protein levels. The vitexin/ICG liposomes prepared based on a simple LOC platform can effectively enhance the solubility of insoluble drugs, and the combined effect of PTT/PDT can effectively increase their antitumor effect, which provides a simple and valid method for the clinical translation of liposomes.
Keyword ：
indocyanine green indocyanine green lab-on-a-chip lab-on-a-chip liposome liposome near-infrared ray near-infrared ray vitexin vitexin
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| GB/T 7714 | Cao, Xia , Liu, Qi , Adu-Frimpong, Michael et al. Microfluidic Generation of Near-Infrared Photothermal Vitexin/ICG Liposome with Amplified Photodynamic Therapy [J]. | AAPS PHARMSCITECH , 2023 , 24 (4) . |
| MLA | Cao, Xia et al. "Microfluidic Generation of Near-Infrared Photothermal Vitexin/ICG Liposome with Amplified Photodynamic Therapy" . | AAPS PHARMSCITECH 24 . 4 (2023) . |
| APA | Cao, Xia , Liu, Qi , Adu-Frimpong, Michael , Shi, Wenwan , Liu, Kai , Deng, Tianwen et al. Microfluidic Generation of Near-Infrared Photothermal Vitexin/ICG Liposome with Amplified Photodynamic Therapy . | AAPS PHARMSCITECH , 2023 , 24 (4) . |
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The emission of volatile organic compounds (VOCs) has resulted in increasingly severe harm to the environment and human health. In recent years, biological methods have become the preferred technology for VOC removal due to their environmental friendliness and economic advantages. Based on the theory of bibliometrics, this study analyzed research articles and reviews on biological methods for VOC removal published in the Web of Science Core Collection (WOSCC) database from 1966 to 2021. The knowledge map visualization software CiteSpace was utilized to analyze research progress in different countries, co-citation clustering, co-citation bursts, and keyword clustering in the literature data. The results indicated that early research on VOC biological treatment focused on the removal of odorous gases and single components of volatile organic waste gases. Subsequently, benzene contents (BTEX), hydrophobic VOCs, and multi-component VOCs have gradually become the focus of research. In recent years, improving VOC removal efficiency by studying packing materials and microbial communities has become an important research topic both domestically and internationally. Future research should focus on continuously improving the performance of reactors, developing novel reactors, and investigating technologies for treating complex and recalcitrant VOCs.
Keyword ：
bibliometrics bibliometrics biological methods biological methods CiteSpace CiteSpace clustering analysis clustering analysis volatile organic compounds volatile organic compounds
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| GB/T 7714 | Wang, Yuan , Zhou, Bin , Yang, Mengrong et al. Bibliometrics and Knowledge Map Analysis of Research Progress on Biological Treatments for Volatile Organic Compounds [J]. | SUSTAINABILITY , 2023 , 15 (12) . |
| MLA | Wang, Yuan et al. "Bibliometrics and Knowledge Map Analysis of Research Progress on Biological Treatments for Volatile Organic Compounds" . | SUSTAINABILITY 15 . 12 (2023) . |
| APA | Wang, Yuan , Zhou, Bin , Yang, Mengrong , Xiao, Gao , Xiao, Hang , Dai, Xiaorong . Bibliometrics and Knowledge Map Analysis of Research Progress on Biological Treatments for Volatile Organic Compounds . | SUSTAINABILITY , 2023 , 15 (12) . |
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Synergisticadsorption and catalytic conversion of SO2 were achievedby metal-phenolic modification of waste collagenfibers at a high efficiency with industrialization potential. SO2 removal is critical to flue gas purification.However,based on performance and cost, materials under development are hardlyadequate substitutes for active carbon-based materials. Here, we engineeredbiomass-derived nanostructured carbon nanofibers integrated with highlydispersed bimetallic Ti/CoO x nanoparticlesthrough the thermal transition of metal-phenolic functionalized industrialleather wastes for synergistic SO2 adsorption and in situcatalytic conversion. The generation of surface-SO3 (2-) and peroxide species (O-2 (2-)) by Ti/CoO x achieved catalytic conversionof adsorbed SO2 into value-added liquid H2SO4, which can be discharged from porous nanofibers. This approachcan also avoid the accumulation of the adsorbed SO2, therebyachieving high desulfurization activity and a long operating lifeover 6000 min, preceding current state-of-the-art active carbon-baseddesulfurization materials. Combined with the techno-economic and carbonfootprint analysis from 36 areas in China, we demonstrated an economicallyviable and scalable solution for real-world SO2 removalon the industrial scale.
Keyword ：
adsorption adsorption biomass biomass desulfurization desulfurization heterogeneous catalysis heterogeneous catalysis metal oxide metal oxide
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| GB/T 7714 | Xiao, Gao , Xie, Qiuping , He, Yunxiang et al. Synergistic Adsorption and In Situ Catalytic Conversion of SO2 by Transformed Bimetal-Phenolic Functionalized Biomass [J]. | ENVIRONMENTAL SCIENCE & TECHNOLOGY , 2023 . |
| MLA | Xiao, Gao et al. "Synergistic Adsorption and In Situ Catalytic Conversion of SO2 by Transformed Bimetal-Phenolic Functionalized Biomass" . | ENVIRONMENTAL SCIENCE & TECHNOLOGY (2023) . |
| APA | Xiao, Gao , Xie, Qiuping , He, Yunxiang , Huang, Xin , Richardson, Joseph J. , Dai, Manna et al. Synergistic Adsorption and In Situ Catalytic Conversion of SO2 by Transformed Bimetal-Phenolic Functionalized Biomass . | ENVIRONMENTAL SCIENCE & TECHNOLOGY , 2023 . |
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本发明公开了一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球及其制备方法和应用。通过多酚网络的功能化改性手段，将Ce基金属有机框架与共价有机聚合物碳球紧密结合，得到具有优异氧化还原性能的纳米复合材料COP‑HB@CeMOF‑BT。本发明有效改善了Ce基催化剂的电化学性能，实现了稀土多酚网络与共价有机聚合物的独特协同作用。制得的纳米复合材料作为燃料电池催化剂具有高电位、优异的极限电流、优良的稳定性以及优异的甲醇耐受性等优点，应用前景广阔。
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| GB/T 7714 | 肖高 , 胡凡莹 , 刘明华 . 一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球 : CN202111230306.2[P]. | 2021-10-22 00:00:00 . |
| MLA | 肖高 et al. "一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球" : CN202111230306.2. | 2021-10-22 00:00:00 . |
| APA | 肖高 , 胡凡莹 , 刘明华 . 一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球 : CN202111230306.2. | 2021-10-22 00:00:00 . |
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本发明提供一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法，属于氧还原电催化技术领域。利用价廉易得的微生物酵母菌为碳模板，开发了以单宁酸络合铁离子的金属多酚超分子为表面黏附功能组装模块为基元，继而在氮气氛下高温碳化处理而得的多孔铁基碳纳米复合材料CTA‑Yeast@Fe NPs。该方法制备工艺简单、成本低、催化剂得率高、形貌均一、比表面积大。多孔铁纳米复合碳材料CTA‑Yeast@Fe NPs作为氧还原电催化剂具有较高起始电位、半坡电位、优异的极限电流以及高稳定性和较强的抗甲醇中毒能力，可替代传统商业Pt/C的高效电催化剂，具有很大的潜在应用价值和产业化前景。
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| GB/T 7714 | 肖高 , 张佳敏 , 刘明华 . 一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法 : CN202210080932.6[P]. | 2022-01-24 00:00:00 . |
| MLA | 肖高 et al. "一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法" : CN202210080932.6. | 2022-01-24 00:00:00 . |
| APA | 肖高 , 张佳敏 , 刘明华 . 一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法 : CN202210080932.6. | 2022-01-24 00:00:00 . |
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本发明公开了一种镧基有机框架复合改性的废铬屑衍生的多孔碳纳米负极电催化剂材料及其制备方法，所述纳米材料活性物质为Cr‑La/CCF‑BT。燃料电池催化剂目前普遍面临着，前驱体单一和合成成本高昂的问题，而商业铂碳催化剂不仅成本高且稳定性差。为克服这些问题，本发明涉及一种镧基有机框架复合改性的废铬屑衍生的多孔碳纳米负极材料的制备，所述材料采用生物模板法，以La‑MOFs稀土金属有机框架修饰改性的废铬屑为模板和碳源，杨梅单宁作为前驱体制备连接La‑MOFs和废铬屑生物模板的桥梁分子，利用废铬屑本身天然的纤维态分级结构制备出具有天然独特形貌的La(MOFs)‑BT@Cr‑CF纳米复合材料前驱体，经高温煅烧最终形成Cr‑La/CCF‑BT。
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| GB/T 7714 | 肖高 , 胡钰花 . 一种镧基有机框架复合改性的废铬屑衍生的多孔碳纳米负极材料的制备 : CN202210873340.X[P]. | 2022-07-21 00:00:00 . |
| MLA | 肖高 et al. "一种镧基有机框架复合改性的废铬屑衍生的多孔碳纳米负极材料的制备" : CN202210873340.X. | 2022-07-21 00:00:00 . |
| APA | 肖高 , 胡钰花 . 一种镧基有机框架复合改性的废铬屑衍生的多孔碳纳米负极材料的制备 : CN202210873340.X. | 2022-07-21 00:00:00 . |
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