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农林生物质衍生多孔碳构筑锂电池负极新材料
期刊论文 | 2025 , 42 (2) , 233-243 | 精细化工
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Abstract :

农林生物质废弃物作为一种价廉易得的可再生资源,具有丰富的碳源和多孔通道优势.其通过炭化和活化等制备方法及其他复合改性方法可得到具有优良性能的新型多孔材料,该材料在储能方面具有广阔的应用前景.特别是在锂离子电池中的应用方面,生物质衍生多孔碳具备可提高电池的循环性能、容量和倍率性能等优势.该文对基于生物质构建锂离子电池负极材料的应用现状进行了总结,主要介绍了稻壳、玉米秸秆、棉花和果壳等生物质衍生多孔碳应用于锂离子电池负极的电化学性能,并探讨了目前生物质基负极材料存在的问题.另外,还讨论了未来生物质在储能领域的研究方向和应用前景,为化工新型碳材料和锂离子电池的可持续发展提供了新途径和新思路.

Keyword :

农林废弃物 农林废弃物 应用方向 应用方向 生物质衍生多孔碳 生物质衍生多孔碳 负极材料 负极材料 锂离子电池 锂离子电池

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GB/T 7714 肖高 , 郑明珠 , 毛诗钰 et al. 农林生物质衍生多孔碳构筑锂电池负极新材料 [J]. | 精细化工 , 2025 , 42 (2) : 233-243 .
MLA 肖高 et al. "农林生物质衍生多孔碳构筑锂电池负极新材料" . | 精细化工 42 . 2 (2025) : 233-243 .
APA 肖高 , 郑明珠 , 毛诗钰 , 李晓慧 . 农林生物质衍生多孔碳构筑锂电池负极新材料 . | 精细化工 , 2025 , 42 (2) , 233-243 .
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农林生物质衍生多孔碳构筑锂电池负极新材料
期刊论文 | 2025 , 42 (02) , 233-243 | 精细化工
农林生物质衍生多孔碳构筑锂电池负极新材料 Scopus
期刊论文 | 2025 , 42 (2) , 233-243 | 精细化工
农林生物质衍生多孔碳构筑锂电池负极新材料 EI
期刊论文 | 2025 , 42 (2) , 233-243 | 精细化工
High-throughput continuous microfluidic magnifiable manufactured microstructured MOFs-mediated micropollutants mitigation (M7) SCIE
期刊论文 | 2025 , 362 | SEPARATION AND PURIFICATION TECHNOLOGY
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Abstract :

Organic micropollutants in wastewater containing arsanilic acid (p-ASA) can undergo a transformation into a highly toxic inorganic arsenic, impacting both the environment and human health. Adsorption materials such as Metal-organic frameworks (MOFs) have attracted great interest, yet their production methods are often complex, costly, and time-consuming, hindering large-scale production. We introduces an innovative, high-throughput microfluidic magnifiable manufacturing approach to expedite MOFs creation, enabling rapid, continuous, and parallel expandable scalable production of MOFs with a uniform microstructure in mere minutes, significantly outpacing the traditional, intermittently operated hydrothermal synthesis. The microfluidic-generated microstructured MF-UIO-66 has better organic arsenic adsorption capacity (333.3 mg/g), and maintained an 89.2 % effectiveness even after four cycles of reuse without generating harmful by-products. When compared to UIO-66 produced via conventional hydrothermal methods, the microfluidically synthesized MF-UIO-66 showcases not only a faster and more effective removal of varying concentrations of organic arsenic but also enhanced chemical stability and longevity. The novel microfluidic fabrication strategy holds great potential for the industrial-scale production of MF-UIO-66 at reduced costs and increased yields.

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GB/T 7714 Xiao, Gao , Zhang, Jun , Zheng, Mingzhu et al. High-throughput continuous microfluidic magnifiable manufactured microstructured MOFs-mediated micropollutants mitigation (M7) [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 362 .
MLA Xiao, Gao et al. "High-throughput continuous microfluidic magnifiable manufactured microstructured MOFs-mediated micropollutants mitigation (M7)" . | SEPARATION AND PURIFICATION TECHNOLOGY 362 (2025) .
APA Xiao, Gao , Zhang, Jun , Zheng, Mingzhu , Chen, Liyin , Afewerki, Samson , Dai, Manna et al. High-throughput continuous microfluidic magnifiable manufactured microstructured MOFs-mediated micropollutants mitigation (M7) . | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 362 .
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High-throughput continuous microfluidic magnifiable manufactured microstructured MOFs-mediated micropollutants mitigation (M7) Scopus
期刊论文 | 2025 , 362 | Separation and Purification Technology
High-throughput continuous microfluidic magnifiable manufactured microstructured MOFs-mediated micropollutants mitigation (M7) EI
期刊论文 | 2025 , 362 | Separation and Purification Technology
One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices SCIE
期刊论文 | 2024 , 221 | EUROPEAN POLYMER JOURNAL
WoS CC Cited Count: 1
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Abstract :

Conductive hydrogels have shown a great potential in the field of flexible electronics. However, it is difficult to combine high strength and high toughness in conductive hydrogels prepared by conventional methods, which limits their applications in various fields. In this work, we pioneered a facile and cost-effective strategy to prepare soy protein isolate/poly(vinyl alcohol) (SPI/PVA) conductive hydrogels with high strength, toughness, low- temperature resistance, and recyclability by introducing all the salts into the prescuor solution directly. To solve the problem of unable to directly introducing high concentration Na3Cit into the soy protein isolate/PVA solution, MgCl2 was used to alleviate the strong salting-out effect of Na3Cit. Thus the stable SPI/PVA/EG/MgCl2/ Na3Cit complex solution was obtained and the SPI/PVA/EG/MgCl2/Na3Cit (SPEMS) organohydrogel was prepared by the freezing/thawing process. The optimum tensile strength of the SPEMS organohydrogel was 1.1 +0.07 MPa, and the elongation at break was 701.3+23.67 %, respectively. Meanwhile, the ionic conductivity of the organohydrogel was as high as 1.7+0.01 S/m. Finally, the EG/H2O binary solvent system endowed the organohydrogel with excellent low-temperature resistance (freezing point of-19.4 degrees C). The strain sensors assembled with SPEMS organohydrogels were characterized by high sensitivity (GF = 3.2, strain range from 20 %-500 %) and long-term stability. The flexible all-solid-state supercapacitor assembled with SPEMS organohydrogel as the electrolyte and activated carbon as the electrodes has a high area specific capacitance (113.76 mF/cm2) and good cycling stability (capacitance retention of 81.62 % after 1,000 charging and discharging cycles) at room temperature.

Keyword :

Hofmeister effect Hofmeister effect One-pot preparation One-pot preparation Poly(vinyl alcohol) Poly(vinyl alcohol) Soy protein isolate Soy protein isolate Strain sensor Strain sensor

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GB/T 7714 Hu, Mingqiang , Deng, Yingxue , Qian, Xing et al. One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices [J]. | EUROPEAN POLYMER JOURNAL , 2024 , 221 .
MLA Hu, Mingqiang et al. "One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices" . | EUROPEAN POLYMER JOURNAL 221 (2024) .
APA Hu, Mingqiang , Deng, Yingxue , Qian, Xing , Ye, Dezhan , Jiang, Xiancai , Xiao, Gao . One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices . | EUROPEAN POLYMER JOURNAL , 2024 , 221 .
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One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices Scopus
期刊论文 | 2024 , 221 | European Polymer Journal
One-pot preparation of strong, tough, frost-resistant and recyclable organohydrogels via Hofmeister effect and its application for electronic devices EI
期刊论文 | 2024 , 221 | European Polymer Journal
Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation SCIE
期刊论文 | 2024 , 20 (43) | SMALL
WoS CC Cited Count: 13
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Abstract :

The use of hydrogel-based interfacial solar evaporators for desalination is a green, sustainable, and extremely concerned freshwater acquisition strategy. However, developing evaporators that are easy to manufacture, cheap, and have excellent porous structures still remains a considerable challenge. This work proposes a novel strategy for preparing a self-assembling sponge-like poly(vinyl alcohol)/graphite composite hydrogel based on the Hofmeister effect for the first time. The sponge-like hydrogel interfacial solar evaporator (PGCNG) is successfully obtained after combining with graphite. The whole process is environmental-friendly and of low-carbon free of freezing process. The PGCNG can be conventionally dried and stored. PGCNG shows impressive water storage performance and water transmission capacity, excellent steam generation performance and salt resistance. PGCNG has a high evaporation rate of 3.5 kg m-2 h-1 under 1 kW m-2 h-1 solar irradiation and PGCNG demonstrates stable evaporation performance over both 10 h of continuous brine evaporation and 30 cycles of brine evaporation. Its excellent performance and simple, scalable preparation strategy make it a valuable material for practical interface solar seawater desalination devices. This paper presents a novel and facile method for obtaining a sponge-like hydrogel with excellent pore structure, outstanding water transport and solar interfacial evaporation performance. The method is based on the Hofmeister effect, whereby the polymer nanofibers are coiled by a combination of salting and salting effects, resulting in the formation of a pore structure. image

Keyword :

desalination desalination hofmeister effect hofmeister effect phase separation phase separation porous hydrogels porous hydrogels solar steam generation solar steam generation

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GB/T 7714 Yang, Mohan , Wu, Yaowei , Chen, Mengdie et al. Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation [J]. | SMALL , 2024 , 20 (43) .
MLA Yang, Mohan et al. "Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation" . | SMALL 20 . 43 (2024) .
APA Yang, Mohan , Wu, Yaowei , Chen, Mengdie , Wang, Yuhao , Zhang, Lei , Deng, Yingxue et al. Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation . | SMALL , 2024 , 20 (43) .
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Hofmeister Effect‐Assisted Facile Fabrication of Self‐Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge‐Like Hydrogel for Solar Steam Generation
期刊论文 | 2024 , 20 (43) , n/a-n/a | Small
Hofmeister Effect-Assisted Facile Fabrication of Self-Assembled Poly(Vinyl Alcohol)/Graphite Composite Sponge-Like Hydrogel for Solar Steam Generation Scopus
期刊论文 | 2024 | Small
Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater SCIE
期刊论文 | 2024 , 24 (49) , 15509-15516 | NANO LETTERS
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Abstract :

Transforming spent coffee grounds and tea residues into valuable hierarchical porous materials presents a sustainable solution for environmental remediation due to the low cost, extensive availability, and versatile functionalized interface. Here, we systematically investigated tea polyphenol-mediated morphological transformation of spent coffee grounds to the synthesis of three-dimensional (3D) mesoporous metal-organic framework (MOF)-derived nanoarchitectured carbon composites. We adopted the sustainable cost-effective tea-coffee derivative to remove typical marine micropollutants, such as antibiotic wastewater, radioactive pollutants, and microplastics. This innovative adsorbent shows remarkable efficiency in antibiotic adsorption, achieving up to 99.62% removal of tetracycline (TC), with an impressive maximum adsorption capacity of 373.1 mg/g. It also demonstrates a remarkable ability to remove marine microplastics and radioactive pollutants with immediate nuclear threats and global sanitation and health crisis posed by Fukushima nuclear waste toward the world. The innovative strategy of treating waste with waste highlights economic potential in wastewater treatment.

Keyword :

Fukushima nuclear waste uranium Fukushima nuclear waste uranium Metal-organicframeworks (MOFs) Metal-organicframeworks (MOFs) Microplastics Microplastics Spent coffee grounds Spent coffee grounds Sustainable marine micropollutant mitigation Sustainable marine micropollutant mitigation Tea residues Tea residues

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GB/T 7714 Xiao, Gao , Guo, Junling , Zheng, Mingzhu et al. Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater [J]. | NANO LETTERS , 2024 , 24 (49) : 15509-15516 .
MLA Xiao, Gao et al. "Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater" . | NANO LETTERS 24 . 49 (2024) : 15509-15516 .
APA Xiao, Gao , Guo, Junling , Zheng, Mingzhu , Zhang, Jun , Chen, Liyin , Dai, Manna et al. Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater . | NANO LETTERS , 2024 , 24 (49) , 15509-15516 .
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Tea/Coffee Sustainable Nanoarchitectures Purify Wastewater Scopus
期刊论文 | 2024 | Nano Letters
Enhancing Anticancer Efficacy of Formononetin Microspheres via Microfluidic Fabrication SCIE
期刊论文 | 2023 , 24 (8) | AAPS PHARMSCITECH
WoS CC Cited Count: 4
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Abstract :

Formononetin is a flavonoid compound with anti-tumor and anti-inflammatory properties. However, its low solubility limits its clinical use. We employed microfluidic technology to prepare formononetin-loaded PLGA-PEGDA microspheres (Degradable polymer PLGA, Crosslinking agent PEGDA), which can encapsulate and release drugs in a controlled manner. We optimized and characterized the microspheres, and evaluated their antitumor effects. The microspheres had uniform size, high drug loading efficiency, high encapsulation efficiency, and stable release for 35 days. They also inhibited the proliferation, migration, and apoptosis. The antitumor mechanism involved the induction of reactive oxygen species and modulation of Bcl-2 family proteins. These findings suggested that formononetin-loaded PLGA-PEGDA microspheres, created using microfluidic technology, could be a novel drug delivery system that can overcome the limitations of formononetin and enhance its antitumor activity.

Keyword :

anti-tumor anti-tumor formononetin formononetin lung cancer lung cancer microfluidic microfluidic microspheres microspheres

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GB/T 7714 Cao, Xia , Li, Qingwen , Li, Xiaoli et al. Enhancing Anticancer Efficacy of Formononetin Microspheres via Microfluidic Fabrication [J]. | AAPS PHARMSCITECH , 2023 , 24 (8) .
MLA Cao, Xia et al. "Enhancing Anticancer Efficacy of Formononetin Microspheres via Microfluidic Fabrication" . | AAPS PHARMSCITECH 24 . 8 (2023) .
APA Cao, Xia , Li, Qingwen , Li, Xiaoli , Liu, Qi , Liu, Kai , Deng, Tianwen et al. Enhancing Anticancer Efficacy of Formononetin Microspheres via Microfluidic Fabrication . | AAPS PHARMSCITECH , 2023 , 24 (8) .
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Enhancing Anticancer Efficacy of Formononetin Microspheres via Microfluidic Fabrication Scopus
期刊论文 | 2023 , 24 (8) | AAPS PharmSciTech
一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法 incoPat
专利 | 2022-01-24 00:00:00 | CN202210080932.6
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本发明提供一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法,属于氧还原电催化技术领域。利用价廉易得的微生物酵母菌为碳模板,开发了以单宁酸络合铁离子的金属多酚超分子为表面黏附功能组装模块为基元,继而在氮气氛下高温碳化处理而得的多孔铁基碳纳米复合材料CTA‑Yeast@Fe NPs。该方法制备工艺简单、成本低、催化剂得率高、形貌均一、比表面积大。多孔铁纳米复合碳材料CTA‑Yeast@Fe NPs作为氧还原电催化剂具有较高起始电位、半坡电位、优异的极限电流以及高稳定性和较强的抗甲醇中毒能力,可替代传统商业Pt/C的高效电催化剂,具有很大的潜在应用价值和产业化前景。

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GB/T 7714 肖高 , 张佳敏 , 刘明华 . 一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法 : CN202210080932.6[P]. | 2022-01-24 00:00:00 .
MLA 肖高 et al. "一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法" : CN202210080932.6. | 2022-01-24 00:00:00 .
APA 肖高 , 张佳敏 , 刘明华 . 一种基于酵母菌碳模板构筑多孔铁纳米复合碳材料的方法 : CN202210080932.6. | 2022-01-24 00:00:00 .
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一种处理利福平抗生素的铁钴多酚超分子改性有机框架复合材料及其制备方法 incoPat
专利 | 2022-01-24 00:00:00 | CN202210080920.3
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本发明公开了一种处理利福平抗生素的铁钴多酚超分子改性有机框架复合材料及其制备方法。所述一种处理利福平抗生素的铁钴多酚超分子改性有机框架复合材料为MIL‑53(Fe)@TA‑Co。本发明的方法合成方法简单,反应条件温和,是一种经济有效的方法。能将此MIL‑53(Fe)@TA‑Co直接作为处理利福平的新型复合材料。解决现有利福平分子去除材料和方法少的现状,用本发明提供的新型复合吸附剂材料具有良好的吸附性能。MIL‑53(Fe)@TA‑Co作为利福平分子去除材料具有很大的潜在应用价值。

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GB/T 7714 肖高 , 杨帆 , 刘明华 . 一种处理利福平抗生素的铁钴多酚超分子改性有机框架复合材料及其制备方法 : CN202210080920.3[P]. | 2022-01-24 00:00:00 .
MLA 肖高 et al. "一种处理利福平抗生素的铁钴多酚超分子改性有机框架复合材料及其制备方法" : CN202210080920.3. | 2022-01-24 00:00:00 .
APA 肖高 , 杨帆 , 刘明华 . 一种处理利福平抗生素的铁钴多酚超分子改性有机框架复合材料及其制备方法 : CN202210080920.3. | 2022-01-24 00:00:00 .
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一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球 incoPat
专利 | 2021-10-22 00:00:00 | CN202111230306.2
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本发明公开了一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球及其制备方法和应用。通过多酚网络的功能化改性手段,将Ce基金属有机框架与共价有机聚合物碳球紧密结合,得到具有优异氧化还原性能的纳米复合材料COP‑HB@CeMOF‑BT。本发明有效改善了Ce基催化剂的电化学性能,实现了稀土多酚网络与共价有机聚合物的独特协同作用。制得的纳米复合材料作为燃料电池催化剂具有高电位、优异的极限电流、优良的稳定性以及优异的甲醇耐受性等优点,应用前景广阔。

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GB/T 7714 肖高 , 胡凡莹 , 刘明华 . 一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球 : CN202111230306.2[P]. | 2021-10-22 00:00:00 .
MLA 肖高 et al. "一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球" : CN202111230306.2. | 2021-10-22 00:00:00 .
APA 肖高 , 胡凡莹 , 刘明华 . 一种稀土多酚超分子包覆的共价有机聚合物铈基纳米碳球 : CN202111230306.2. | 2021-10-22 00:00:00 .
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一种铜多酚超分子网络界面修饰的稀土基有机框架负极材料的制备及应用 incoPat
专利 | 2022-04-19 00:00:00 | CN202210409833.8
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本发明公开了一种铜多酚超分子网络界面修饰的稀土基有机框架负极材料电催化剂材料及其制备方法,所述纳米材料活性物质为Ce‑MOF@BT‑Cu。燃料电池催化剂目前普遍面临着,前驱体单一和合成成本高昂的问题,而商业铂碳催化剂不仅成本高且稳定性差。为克服这些问题,本发明基于金属多酚网络的独特结构,开发了一种铜多酚超分子网络界面修饰的稀土基有机框架负极材料。该材料呈现出均匀的颗粒状结构和丰富的孔道结构,具有高电位和良好的极限电流,拥有优良的稳定性。所采用的合成方法,操作简便,成本低廉,且制备时间短,有利于实现大规模商业化生产。

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GB/T 7714 肖高 , 胡钰花 . 一种铜多酚超分子网络界面修饰的稀土基有机框架负极材料的制备及应用 : CN202210409833.8[P]. | 2022-04-19 00:00:00 .
MLA 肖高 et al. "一种铜多酚超分子网络界面修饰的稀土基有机框架负极材料的制备及应用" : CN202210409833.8. | 2022-04-19 00:00:00 .
APA 肖高 , 胡钰花 . 一种铜多酚超分子网络界面修饰的稀土基有机框架负极材料的制备及应用 : CN202210409833.8. | 2022-04-19 00:00:00 .
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