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学者姓名：林梅金
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Abstract ：
将嫁接理论引入区域产教融合培养模式的研究,分析单一地区产教融合模式中区域、产业、高校的特质以及三者之间的交互作用.追踪观察福州大学材料学科产教融合模式培养实例,结果表明:产教融合模式对企业增效、科研成果产出、创新人才培养起到了促进作用.产教融合团队作为串联线索,间接推动区域内多类资源良性循环.但此模式还需解决创新赛道开辟、人文教育补充等问题,以便进一步完善区域创新人才产教融合培养模式.
Keyword ：
产教融合 产教融合 区域创新 区域创新 嫁接理论 嫁接理论
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| GB/T 7714 | 梁滢 , 林梅金 , 黄艳 . 区域创新人才产教融合培养模式探索:嫁接理论视角 [J]. | 中国轻工教育 , 2025 , 28 (1) : 19-27 . |
| MLA | 梁滢 等. "区域创新人才产教融合培养模式探索:嫁接理论视角" . | 中国轻工教育 28 . 1 (2025) : 19-27 . |
| APA | 梁滢 , 林梅金 , 黄艳 . 区域创新人才产教融合培养模式探索:嫁接理论视角 . | 中国轻工教育 , 2025 , 28 (1) , 19-27 . |
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Donor-acceptor crystalline hybrid materials are a new type of photoactive hybrid complex composed of two semiconductor components at the molecular level. Naphthalenediimide (NDI) and perylenediimide (PDI) based donor-acceptor crystalline hybrid materials have garnered significant interest in recent years owing to the structural diversity of the inorganic semiconductors and excellent redox activity in the NDI/PDI, which can effectively achieve long-lived charge separation and transfer under irradiation. In this review, we summarize recent research progress in the construction of NDI/PDI-based crystalline hybrid materials using POMs, metal halides, and transition-metal ions, and their applications in photochromism, photo-controllable fluorescence/ phosphorescence, photocatalytic organic transformations, and photothermal conversion, and as antibacterials, to provide useful guidance for the design, preparation and application of these materials in the future.
Keyword ：
Donor-acceptor Donor-acceptor Hybrid material Hybrid material NDI NDI PDI PDI POMs POMs
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| GB/T 7714 | Liu, Zhengfen , Li, Xiaobo , Dai, Weijun et al. Naphthalenediimide and perylenediimide based donor-acceptor crystalline hybrid materials: Structures and applications [J]. | COORDINATION CHEMISTRY REVIEWS , 2025 , 526 . |
| MLA | Liu, Zhengfen et al. "Naphthalenediimide and perylenediimide based donor-acceptor crystalline hybrid materials: Structures and applications" . | COORDINATION CHEMISTRY REVIEWS 526 (2025) . |
| APA | Liu, Zhengfen , Li, Xiaobo , Dai, Weijun , Liu, Jian-Jun , Lin, Mei-Jin . Naphthalenediimide and perylenediimide based donor-acceptor crystalline hybrid materials: Structures and applications . | COORDINATION CHEMISTRY REVIEWS , 2025 , 526 . |
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Heavy doping critically minimizes depletion region widths for efficient charge transport in organic solar cells (OSCs), yet systematic studies elucidating its underlying mechanisms remain scarce. To address this, two polydopamine-polyoxometalate composites (PDA-PMA and PDA-PMA(N)) are designed via innovative mutual doping pathways. PDA-PMA achieved ultrahigh doping density (1.17 x 1023 cm-3) through H3[P(Mo3O10)4] (PMA) initiated oxidative polymerization of dopamine, where electron transfer simultaneously induced p-doped PDA and n-doped PMA. Remarkably, neutralization with ammonia yielded PDA-PMA(N), which retained even higher doping density (3.74 x 1023 cm-3) via structural rearrangement-driven organic doping. XPS/ESR studies revealed distinct pathways: dual organic/inorganic doping in PDA-PMA versus organic-dominated doping in PDA-PMA(N). This deep doping compressed depletion region widths from 44.42 nm in undoped controls (the blend of PDA and PMA) to 0.052 nm (PDA-PMA(N)), surpassing PEDOT:PSS (0.238 nm) and enabling barrier-free hole transport. Consequently, PBDB-TF:BTP-eC9-based OSCs with PDA-PMA and PDA-PMA(N) achieved exceptional power conversion efficiencies (PCEs) of 20.02% and 20.29%, respectively. Furthermore, the neutralized PDA-PMA(N) demonstrated superior stability (86.2% PCE retention after 1800 h illumination) by suppressing interfacial corrosion. This work elucidates structure-dependent doping mechanisms and provides a universal strategy for developing high-performance hole transport layers through tailored doping, advancing OSC commercialization.
Keyword ：
doping mechanism doping mechanism hole transport materials hole transport materials ohmic contact ohmic contact organic solar cells organic solar cells polyoxometalate polyoxometalate
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| GB/T 7714 | Han, Xiaona , Yu, Jiawu , Chen, Yudong et al. Polydopamine-Polyoxometalate Composites in Neutral pH Enable High-Efficiency and Ultra-Stable Organic Solar Cells via Mutual Doping Mechanism [J]. | ADVANCED MATERIALS , 2025 . |
| MLA | Han, Xiaona et al. "Polydopamine-Polyoxometalate Composites in Neutral pH Enable High-Efficiency and Ultra-Stable Organic Solar Cells via Mutual Doping Mechanism" . | ADVANCED MATERIALS (2025) . |
| APA | Han, Xiaona , Yu, Jiawu , Chen, Yudong , Qu, Hang , Ruan, Zining , Lin, Meijin et al. Polydopamine-Polyoxometalate Composites in Neutral pH Enable High-Efficiency and Ultra-Stable Organic Solar Cells via Mutual Doping Mechanism . | ADVANCED MATERIALS , 2025 . |
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The synthesis, characterization, and properties of phthalimide-fused phenanthrenone (PIP) and its dicyano derivative (PIPCN) are reported in this study. A three-step synthetic route was established for the preparation of PIP. Single-crystal X-ray diffraction revealed PIP's rigid pi-conjugated framework and significant intermolecular interactions. Systematic UV-vis absorption spectra and DFT calculations demonstrated that the dicyano group in PIPCN enhances intramolecular charge transfer effects, resulting in lower LUMO energy levels compared to classical imide units such as naphthalene diimide (NDI) and perylene diimide (PDI). Furthermore, Z-scan experiments highlighted PIPCN's pronounced third-order nonlinear optical properties. These findings demonstrate that PIP and PIPCN are promising candidates for applications in organic electronics and nonlinear optical materials.
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| GB/T 7714 | Chen, Songhua , Wei, Shengchen , Wu, Shuai et al. Synthesis, Characterization, and Properties of Phthalimide-Fused Phenanthrenone [J]. | ORGANIC LETTERS , 2025 , 27 (33) : 9265-9269 . |
| MLA | Chen, Songhua et al. "Synthesis, Characterization, and Properties of Phthalimide-Fused Phenanthrenone" . | ORGANIC LETTERS 27 . 33 (2025) : 9265-9269 . |
| APA | Chen, Songhua , Wei, Shengchen , Wu, Shuai , Shi, Dan , Zhu, Xiangzhao , Yang, Sha et al. Synthesis, Characterization, and Properties of Phthalimide-Fused Phenanthrenone . | ORGANIC LETTERS , 2025 , 27 (33) , 9265-9269 . |
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Photochromic materials, renowned for their reversible light-induced responses, have found widespread applications in areas such as optical storage, photosensitive devices and anti-counterfeiting technologies. Recently, metal-organic framework (MOF) radiochromic materials have attracted increasing attention due to their advantageous properties of good design flexibility, visualization capabilities, cost-effectiveness and rapid radiation response. These properties position MOFs as promising substitutes for traditional commercial radiation detection materials. In this review, we primarily discuss MOF radiation-induced chromic materials, which are driven by photoinduced electron transfer mechanisms resulting in radical generation, characterized by rapid radiation response and structural adaptability. Firstly, we explore the chromic mechanisms, performance evaluation parameters, and structural categories of MOF chromic materials. Subsequently, we discuss their multifunctional applications, followed by an analysis and summary of the modulation of their photoelectric response. Finally, we present our insights into the future development and structural modulation of MOF radiation-induced chromic materials, emphasizing their research significance and potential applications in radiation detection.
Keyword ：
Electron transfer Electron transfer Metal-organic framework Metal-organic framework Photoelectric response Photoelectric response Radiochromism Radiochromism
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| GB/T 7714 | Wei, Qing-Song , Di, Yi-Ming , You, Ming-Hua et al. Metal-organic framework radiochromic materials: Recent advances and applications [J]. | COORDINATION CHEMISTRY REVIEWS , 2025 , 534 . |
| MLA | Wei, Qing-Song et al. "Metal-organic framework radiochromic materials: Recent advances and applications" . | COORDINATION CHEMISTRY REVIEWS 534 (2025) . |
| APA | Wei, Qing-Song , Di, Yi-Ming , You, Ming-Hua , Chen, Hong-Ming , Lin, Mei-Jin . Metal-organic framework radiochromic materials: Recent advances and applications . | COORDINATION CHEMISTRY REVIEWS , 2025 , 534 . |
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Organic fluorescent glassy scintillators hold great promise for security screening and medical imaging due to their excellent optical transparency and good processability. However, their limited exciton utilization, particularly the inefficient harvesting of 75% triplet excitons, restricts radioluminescence (RL) efficiency and imaging resolution. Herein, a general host-guest doping strategy is proposed to enhance triplet exciton harvesting and scintillation performance in organic fluorescent glass. Specifically, using 1,3-Bis(9H-carbazol-9-yl)benzene (mCP) as a glass-forming host and doping it with three types of high triplet-utilization emitters (HMB, IrPA, and HXF), the obtained HMB@mCPG, IrPA@mCPG, and HXF@mCPG glasses exhibit thermally activated delayed fluorescence, phosphorescence and delayed fluorescence from inverted singlet-triplet gap, respectively. Compared to pristine mCP glass, these doped glasses exhibit RL intensity enhancements of 3.4-fold (HMB@mCPG), 6.2-fold (IrPA@mCPG), and 3.4-fold (HXF@mCPG), respectively. The improvements are attributed to efficient host-guest energy transfer, which enables effective harvesting of triplet excitons and suppression of aggregation-induced quenching in glassy materials. Furthermore, all samples enable X-ray imaging with spatial resolutions exceeding 20 lp mm-1, with HXF@mCPG even achieving over 30 lp mm-1. This work highlights a versatile and effective triplet-harvesting strategy for advancing the performance of organic glassy scintillators, paving the way toward high-resolution X-ray imaging applications.
Keyword ：
host-guest doping host-guest doping organic glassy scintillator organic glassy scintillator triplet excitons harvesting triplet excitons harvesting X-ray imaging X-ray imaging
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| GB/T 7714 | Fang, Xin , Zheng, Jiaqi , Chen, Jingru et al. Triplet Excitons Harvesting in Host-Guest Doped Organic Glassy Scintillators for High-Resolution X-Ray Imaging [J]. | ADVANCED FUNCTIONAL MATERIALS , 2025 . |
| MLA | Fang, Xin et al. "Triplet Excitons Harvesting in Host-Guest Doped Organic Glassy Scintillators for High-Resolution X-Ray Imaging" . | ADVANCED FUNCTIONAL MATERIALS (2025) . |
| APA | Fang, Xin , Zheng, Jiaqi , Chen, Jingru , Xu, Xiaocong , Ye, Yuanji , Chen, Hongming et al. Triplet Excitons Harvesting in Host-Guest Doped Organic Glassy Scintillators for High-Resolution X-Ray Imaging . | ADVANCED FUNCTIONAL MATERIALS , 2025 . |
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Metal-organic single-molecule magnets (SMMs), especially single-ion magnets (SIMs), attract growing attention due to their unique magnetic behavior, which can be used for the development of computing technologies. Herein, we report the synthesis of a new mononuclear Dy(iii) complex (2-Dy) using a calix[4]arene ligand (2), decorated with two lower rim-appended salicylideneamine groups, bearing azophenyl moieties. The structures of both the ligand and Dy(iii) complex were thoroughly characterized in the crystalline phase. X-ray diffraction of ligand 2 revealed the formation of a racemic mixture of left-handed and right-handed conformers. Upon binding to the Dy(iii) atom, the macrocycle 2 behaves as a highly coordinating ligand by totally capping the metal coordination sphere, leading to the formation of a distorted triangular dodecahedron coordination sphere (D2d symmetry). In the crystalline phase, for 2-Dy, two complex enantiomer counterparts were stacked into 1D homochiral chains due to weak CH/pi interactions. Analysis of magnetic properties showed that the obtained complex exhibited slow magnetic relaxation behavior at a temperature up to 10 K in the absence of an external dc field.
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| GB/T 7714 | Strelnikova, Iuliia V. , Iova, Angelina A. , Ovsyannikov, Alexander S. et al. New mononuclear Dy(iii) complex based on a calix[4]arene ligand with two appended salicylideneamine groups decorated with azophenyl fragments: synthesis, crystalline assembly and slow magnetic relaxation behavior [J]. | DALTON TRANSACTIONS , 2025 , 54 (24) : 9584-9593 . |
| MLA | Strelnikova, Iuliia V. et al. "New mononuclear Dy(iii) complex based on a calix[4]arene ligand with two appended salicylideneamine groups decorated with azophenyl fragments: synthesis, crystalline assembly and slow magnetic relaxation behavior" . | DALTON TRANSACTIONS 54 . 24 (2025) : 9584-9593 . |
| APA | Strelnikova, Iuliia V. , Iova, Angelina A. , Ovsyannikov, Alexander S. , Islamov, Daut R. , Litvonov, Igor A. , Lazarenko, Vladimir A. et al. New mononuclear Dy(iii) complex based on a calix[4]arene ligand with two appended salicylideneamine groups decorated with azophenyl fragments: synthesis, crystalline assembly and slow magnetic relaxation behavior . | DALTON TRANSACTIONS , 2025 , 54 (24) , 9584-9593 . |
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Crystalline donor-acceptor (D-A) hybrid materials show a significant potential for photocatalytic applications, but achieving broad light absorption and high photocatalytic efficiency remains a challenge. To address this issue, herein, heteropoly blues, as electron donors, and N,N '-bis(N,N-dimethylaminoethyl)-1,4,5,8-naphthalenediimide (NDIDMA), as electron acceptors, have been introduced to these D-A hybrid materials to enhance their light-harvesting and photocatalytic capabilities. Consequently, heteropoly blue/naphthalenediimide D-A hybrid materials H2NDIDMA[H5PMo8 VIMo4 VO40]2DMF (1) have been synthesized. For comparison, the isostructural fully oxidized polyoxometalate-containing counterpart, H2NDIDMAHPW12O402DMF (2), has also been prepared. As expected, hybrid 1 exhibited a broad light absorption range (300-2500 nm) and demonstrated superior photocatalytic decontamination abilities against mustard gas simulants under full-spectrum and near-infrared (NIR) light irradiation compared to hybrid 2. Remarkably, the heteropoly blues in hybrid 1 demonstrated high stability under catalytic conditions and in ambient environments. Additionally, these stable hybrids exhibited excellent recyclability without a loss of activity after five cycles.
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| GB/T 7714 | Song, Yu-Ping , Di, Yi-Ming , Zhang, Shu-Quan et al. Panchromatic Donor-Acceptor Hybrid Materials for Near-Infrared-Activatable Photocatalytic Detoxification of Mustard Gas Simulants [J]. | INORGANIC CHEMISTRY , 2025 , 64 (18) : 9277-9286 . |
| MLA | Song, Yu-Ping et al. "Panchromatic Donor-Acceptor Hybrid Materials for Near-Infrared-Activatable Photocatalytic Detoxification of Mustard Gas Simulants" . | INORGANIC CHEMISTRY 64 . 18 (2025) : 9277-9286 . |
| APA | Song, Yu-Ping , Di, Yi-Ming , Zhang, Shu-Quan , Lin, Mei-Jin . Panchromatic Donor-Acceptor Hybrid Materials for Near-Infrared-Activatable Photocatalytic Detoxification of Mustard Gas Simulants . | INORGANIC CHEMISTRY , 2025 , 64 (18) , 9277-9286 . |
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Poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) is a widely used anode interlayer (AIL) in organic solar cells (OSCs). However, the intrinsic acidity and hygroscopic nature of PSS ions in PEDOT:PSS have been proven to cause electrode corrosion and deteriorate device performance. Herein, a straightforward method is reported to enhance the water resistance of PEDOT:PSS by incorporating tris[bis(methoxymethyl)amino]-1,3,5-triazine (HM) as a cross-linker. The cross-linking reaction between PSS and HM neutralizes the acidity of PEDOT:PSS and forms a stable, hydrophobic network. Additionally, the aggregation morphology of PEDOT:PSS was regulated by HM, improving the conductivity and work function, thereby resulting in enhanced hole extraction and transport ability. Devices incorporating PEDOT:PSS-HM demonstrated improved power conversion efficiency (PCE) of 19.03% compared to 17.88% for those using standard PEDOT:PSS. The neutral pH and water-resistant nature of PEDOT:PSS-HM effectively improved the long-term stability of OSCs with a T80 of over 400 h under continuous illumination. Moreover, after aging the PEDOT: PSS-HM film for 216 h at 80% relative humidity and 40 degrees C, it can be still used as AIL to fabricate efficient OSC devices. This work presents a simple and effective approach to preparing a non-corrosive and stable PEDOT derivative, offering valuable insights for the development of high-performance AIL materials.
Keyword ：
anode interlayer anode interlayer cross-linking cross-linking organic solar cells organic solar cells PEDOT:PSS PEDOT:PSS water-resistant water-resistant
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| GB/T 7714 | Shan, Xin , Fang, Minghai , Wu, Liang et al. Enhanced water resistance of PEDOT:PSS through crosslinking agent incorporation for efficient and stable organic solar cells [J]. | SCIENCE CHINA-MATERIALS , 2025 , 68 (5) : 1452-1461 . |
| MLA | Shan, Xin et al. "Enhanced water resistance of PEDOT:PSS through crosslinking agent incorporation for efficient and stable organic solar cells" . | SCIENCE CHINA-MATERIALS 68 . 5 (2025) : 1452-1461 . |
| APA | Shan, Xin , Fang, Minghai , Wu, Liang , Rong, Hongchen , Liao, Qing , Qian, Deping et al. Enhanced water resistance of PEDOT:PSS through crosslinking agent incorporation for efficient and stable organic solar cells . | SCIENCE CHINA-MATERIALS , 2025 , 68 (5) , 1452-1461 . |
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Metal-free molecular perovskites have shown great potential for X-ray detection due to their tunable chemical structures, low toxicity, and excellent photophysical properties. However, their limited X-ray absorption and environmental instability restrict their practical application. In this study, cesium-based molecular perovskites (MDABCO-CsX3, X = Cl, Br, I) are developed by introducing Cs+ at the B-site to enhance X-ray absorption while retaining low toxicity. The effects of halide modulation on the physical properties and device performance are systematically investigated. Among the variants, MDABCO-CsBr3 exhibited superior environmental stability, attributed to the optimal ionic radius and high chemical stability of Br-. This stability is further enhanced by a higher tolerance factor, which promotes a stable 3D cubic structure and suppresses ion migration within the crystal. Consequently, MDABCO-CsBr3-based X-ray detectors demonstrated reduced ionic migration, minimal dark current drift, and a stable current response under X-ray exposure, achieving a high sensitivity of 4124 mu C Gy-1 cm-2 and a low detection limit of 0.45 mu Gy s-1. Moreover, the devices exhibit excellent thermal stability, operating effectively at temperatures up to 130 degrees C. These results highlight MDABCO-CsBr3 as a promising candidate for stable and efficient X-ray detection, expanding the applicability of molecular perovskites in advanced radiation detection technologies.
Keyword ：
cesium-substituted cesium-substituted environmental stability environmental stability molecular perovskite molecular perovskite X-ray detection X-ray detection
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| GB/T 7714 | Wu, Liang , Wei, Qingsong , Di, Yiming et al. Cesium-Based Molecular Perovskites With Superior Stability for High-Performance X-Ray Detection [J]. | SMALL , 2025 , 21 (10) . |
| MLA | Wu, Liang et al. "Cesium-Based Molecular Perovskites With Superior Stability for High-Performance X-Ray Detection" . | SMALL 21 . 10 (2025) . |
| APA | Wu, Liang , Wei, Qingsong , Di, Yiming , Chen, Fuhai , Qiu, Qiangwen , Shan, Xin et al. Cesium-Based Molecular Perovskites With Superior Stability for High-Performance X-Ray Detection . | SMALL , 2025 , 21 (10) . |
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