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学者姓名：黄文仕
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Abstract ：
The water gas shift reaction is an important procedure in high-purity hydrogen production, and achieving high CO conversion in one single reactor is a key optimization objective. This work has developed a novel radial flow fixed-bed reactor for water gas shift reaction with integrated variable heat exchange and numerically investigated the system optimization concepts. The continuous heat removal from the catalyst bed has been proven to fully improve CO conversion at a lower H2O/CO molar ratio. The heat transfer rate distribution can also be flexibly adjusted to ensure sufficiently high and low temperatures in the early and late stages of the reaction, respectively, for a higher conversion. With sufficient coolant, low-temperature and high-temperature catalysts for water gas shift reaction can be combined in one reactor to increase CO conversion to over 98%, and the delayed heat removal configuration can achieve the highest CO conversion (98.50%) with the least proportion of low-temperature catalysts (9.2%). © 2024 Hydrogen Energy Publications LLC
Keyword ：
Low temperature production Low temperature production Radial flow Radial flow Water gas shift Water gas shift
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| GB/T 7714 | Huang, Yunyun , Huang, Wenshi , Lin, Li et al. Design of a radial flow fixed-bed reactor with integrated variable heat exchange for more efficient and purer hydrogen production via water gas shift reaction [J]. | International Journal of Hydrogen Energy , 2025 , 99 : 685-696 . |
| MLA | Huang, Yunyun et al. "Design of a radial flow fixed-bed reactor with integrated variable heat exchange for more efficient and purer hydrogen production via water gas shift reaction" . | International Journal of Hydrogen Energy 99 (2025) : 685-696 . |
| APA | Huang, Yunyun , Huang, Wenshi , Lin, Li , Cao, Yanning , Luo, Yu , Lin, Xingyi et al. Design of a radial flow fixed-bed reactor with integrated variable heat exchange for more efficient and purer hydrogen production via water gas shift reaction . | International Journal of Hydrogen Energy , 2025 , 99 , 685-696 . |
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Ammonia is a carbon-free energy carrier with 17.6 wt% hydrogen content. The design of an efficient and compact ammonia decomposition reactor based on low-temperature catalysts is the key to realizing industrial hydrogen production from ammonia. In this work, a multiscale model was developed by bridging the particle-scale characteristics of catalysts and reactor performances, to fully comprehend the ammonia decomposition process. The effects of catalyst porosity and pore diameters on the reactor size, precious metal loading, and the profile of temperature and heat flux were systematically evaluated. An improved reactor design was further proposed by applying the segmented reactor packed with two-stage egg-shell-type low-temperature catalysts, which decreased the precious metal usage by 61.6% and the temperature drop by 42.9 K. This segmentation strategy balanced the reaction rate and heat flux, indicating a significant potential in highly efficient, economical, and reliable hydrogen production from ammonia.
Keyword ：
ammonia decomposition ammonia decomposition catalyst micro-structure catalyst micro-structure hydrogen production hydrogen production multiscale model multiscale model precious metal reduction precious metal reduction
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| GB/T 7714 | Zhang, Lixuan , Wu, Yifan , Huang, Wenshi et al. Multiscale modeling of a low-temperature NH3 decomposition reactor for precious metal reduction and temperature control [J]. | AICHE JOURNAL , 2025 . |
| MLA | Zhang, Lixuan et al. "Multiscale modeling of a low-temperature NH3 decomposition reactor for precious metal reduction and temperature control" . | AICHE JOURNAL (2025) . |
| APA | Zhang, Lixuan , Wu, Yifan , Huang, Wenshi , Lin, Li , Wang, Luqiang , Wu, Zeyun et al. Multiscale modeling of a low-temperature NH3 decomposition reactor for precious metal reduction and temperature control . | AICHE JOURNAL , 2025 . |
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The ongoing spontaneous combustion of coal seams beneath the earth’s surface leads to the exhaustion of nonrenewable resources and poses a substantial threat to environmental integrity. Precise and efficacious monitoring of subsurface coal fire activities is an indispensable precondition for the prevention and management of coalfield conflagrations, as well as for the exploitation of geothermal energy resources. The accurate detection and localization of covert coal fires depend on the procurement and analytical assessment of distribution data for parameters that are intrinsically linked to the activities associated with coal combustion. To this end, our review work investigated the theoretical foundations, application effects, and inherent limitations of the diverse detection techniques currently available. It has been observed that the ambiguities inherent to individual detection tools can be effectively mitigated through the cross validation of findings derived from multiple detection tools. The role of detection tools can be extended to the entire process of coal fire management, yet the distinct contributions of each tool throughout the various stages of the process warrant further investigation and elucidation. In addition, the potential of emerging technologies such as machine learning algorithms and 5 G networks to promote automation and intelligence in coal fire management work was also discussed. It is our hope that the insights presented herein will serve as a valuable resource for policymakers and stakeholders in the formulation of effective strategies for the prevention and control of coalfield fires. © 2024 Taylor & Francis Group, LLC.
Keyword ：
Coal fire Coal fire detection and location detection and location electrical resistivity electrical resistivity electromagnetic radiation electromagnetic radiation remote sensing remote sensing
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| GB/T 7714 | Gu, Y. , Li, H. , Dou, L. et al. Advance in Detection and Management for Underground Coal Fires: A Global Technological Overview [J]. | Combustion Science and Technology , 2024 . |
| MLA | Gu, Y. et al. "Advance in Detection and Management for Underground Coal Fires: A Global Technological Overview" . | Combustion Science and Technology (2024) . |
| APA | Gu, Y. , Li, H. , Dou, L. , Wu, M. , Guo, H. , Huang, W. et al. Advance in Detection and Management for Underground Coal Fires: A Global Technological Overview . | Combustion Science and Technology , 2024 . |
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The influence of high jet velocity on the ignition characteristics of pulverized coal is very important for the Moderate or Intense Low-oxygen Dilution (MILD) combustion technology of pulverized coal. This paper conducts experimental and numerical simulation research on the ignition characteristics of the pulverized coal jet in a high-temperature environment based on the Hencken-type flat flame burner. The results show that when the ambient temperature is 1873 K and the ambient oxygen mole fraction is 5 %, the ignition delay distance of the pulverized coal jet decreases as the jet velocity increases from 15 m/s to 100 m/s for the formation of MILD combustion. The adoption of the turbulent particle heat transfer model and the non-spherical particle motion model effectively improves the prediction of particle dispersion, ignition delay, and reaction zone in the highvelocity coal jet flame. The enhancement of gas-solid heat transfer by turbulent fluctuation plays a dominant role in advancing the coal ignition in the high-velocity jet, while the non-spherical shape of coal particles mainly improves the uniformity of reaction distribution. The influence of ignition characteristics in the high-velocity jet on the MILD combustion formation of pulverized coal has been also analyzed in detail.
Keyword ：
Coal ignition Coal ignition Coal jet flame Coal jet flame MILD combustion MILD combustion Particle dispersion Particle dispersion
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| GB/T 7714 | Huang, Wenshi , Wu, Yuxin , Feng, Lele et al. Ignition characteristics of the high-velocity pulverized coal jet in MILD combustion mode: Experiments and prediction improvements [J]. | FUEL , 2023 , 360 . |
| MLA | Huang, Wenshi et al. "Ignition characteristics of the high-velocity pulverized coal jet in MILD combustion mode: Experiments and prediction improvements" . | FUEL 360 (2023) . |
| APA | Huang, Wenshi , Wu, Yuxin , Feng, Lele , Zhang, Hai . Ignition characteristics of the high-velocity pulverized coal jet in MILD combustion mode: Experiments and prediction improvements . | FUEL , 2023 , 360 . |
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