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学者姓名：陈鸿铭
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Abstract ：
Harnessing supramolecular interactions to regulate the structure and performance of functional materials is a key challenge in materials chemistry. Herein, the study utilizes 18-crown-6 (18C6) ether-assisted alkali-metal (Na, K, Cs) copper(I) iodide supramolecular assemblies to precisely regulate the material structures. This approach facilitated the transition from 1D mono-royal crown coordination (18C6@KCuI2, CKCI) to 0D di-royal crown ((18C6)(2)@Na-2(H2O)(3)Cu4I6, CNCI) and tri-royal crown ((18C6)(3)@Cs2Cu2I4, CCCI) structures. Interestingly, the CCCI single-crystal exhibits outstanding scintillation properties, with a high relative light yield of 71 000 photons MeV-1 and an ultralow detection limit of 39.3 nGy s(-1), which can be attributed to the synergistic effects of 18C6 and copper-iodide clusters. It stabilizes the self-trapped exciton state, enhances exciton localization, and reduces non-radiative losses, thus resulting in a large Stokes shift of 193 nm and near-unity photoluminescence quantum yield of 99.4%. Additionally, 18C6 can promote crystal nucleation and growth, making it easy to prepare centimeter-scale transparent single crystals with >80% transmittance, such as CCCI single crystal can achieve an ultrahigh-resolution X-ray imaging of 26.3 lp mm(-1). It demonstrates that the structure and performance of halide scintillators can be regulated through supramolecular interactions, which provides a new approach for developing high-performance scintillator materials.
Keyword ：
18-crown-6 18-crown-6 copper(I) iodide copper(I) iodide self-trapped exciton state self-trapped exciton state supramolecular scintillators supramolecular scintillators X-ray imaging X-ray imaging
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| GB/T 7714 | Ye, Yuanji , Di, Yiming , Zhou, Jiahao et al. Crown Ether-Assisted Alkali-Metal Copper(I) Iodide Supramolecular Scintillators with Near-Unity Emission for Ultrahigh-Resolution X-Ray Imaging [J]. | ADVANCED FUNCTIONAL MATERIALS , 2025 . |
| MLA | Ye, Yuanji et al. "Crown Ether-Assisted Alkali-Metal Copper(I) Iodide Supramolecular Scintillators with Near-Unity Emission for Ultrahigh-Resolution X-Ray Imaging" . | ADVANCED FUNCTIONAL MATERIALS (2025) . |
| APA | Ye, Yuanji , Di, Yiming , Zhou, Jiahao , Qiu, Qiangwen , Chen, Yuhua , Zhong, Shanyuan et al. Crown Ether-Assisted Alkali-Metal Copper(I) Iodide Supramolecular Scintillators with Near-Unity Emission for Ultrahigh-Resolution X-Ray Imaging . | ADVANCED FUNCTIONAL MATERIALS , 2025 . |
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Lanthanide-based metal-organic framework (Ln-MOF) scintillators are promising for X-ray imaging owing to their structural tunability and high X-ray attenuation. However, achieving efficient triplet-sensitized scintillation remains challenging due to the inefficient energy transfer between organic ligand triplets and lanthanide centers, leading to weak radioluminescence and limited imaging resolution. Herein, we propose a dual-antenna ligand strategy by synergizing 4,4 '-oxybis (benzoic acid) (Oba) and phenanthroline derivatives (1,10-phenanthroline = Phen; or Bathophenanthroline = Bphen) with Eu3+ ions, constructing ultrabright Eu-O-Phen and Eu-O-Bphen scintillators. Notably, Eu-O-Bphen demonstrated a record relative light yield of 60331 +/- 28 photons MeV-1, outperforming Eu-O-Phen by 71%. This superior scintillation performance originates from an 86.3 +/- 0.19% photoluminescence quantum yield, attributed to enhanced ligand-to-metal energy transfer efficiency and the suppression of pi-pi stacking among organic chromophore ligands. Besides, the fabrication of flexible Eu-O-Bphen films achieves a spatial resolution of 37.0 lp mm-1 in static imaging and enables real-time dynamic X-ray imaging at 60 fps (2 K). Additionally, it exhibited exceptional water stability, with negligible performance degradation in water for over 100 days, allowing clear underwater visualization of circuit boards under X-ray irradiation. It provides a promising strategy for developing high-performance water-stable scintillators via ligand engineering.
Keyword ：
Dual-antenna ligands Dual-antenna ligands Dynamic X-ray imaging Dynamic X-ray imaging Metal-organic frameworks Metal-organic frameworks Scintillators Scintillators Water-stable Water-stable
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| GB/T 7714 | Chen, Hongming , Yang, Xi , Ye, Yuanji et al. Ultrabright and Water-Stable Eu(III)-Based MOF Scintillators Sensitized by Dual-Antenna Ligands for Real-Time and Underwater X-Ray Imaging [J]. | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION , 2025 . |
| MLA | Chen, Hongming et al. "Ultrabright and Water-Stable Eu(III)-Based MOF Scintillators Sensitized by Dual-Antenna Ligands for Real-Time and Underwater X-Ray Imaging" . | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2025) . |
| APA | Chen, Hongming , Yang, Xi , Ye, Yuanji , Hong, Hongyang , Wei, Qingsong , Zhu, Yanan et al. Ultrabright and Water-Stable Eu(III)-Based MOF Scintillators Sensitized by Dual-Antenna Ligands for Real-Time and Underwater X-Ray Imaging . | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION , 2025 . |
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Metal-free molecular perovskites have shown great potential for X-ray detection due to their tunable chemical structures, low toxicity, and excellent photophysical properties. However, their limited X-ray absorption and environmental instability restrict their practical application. In this study, cesium-based molecular perovskites (MDABCO-CsX3, X = Cl, Br, I) are developed by introducing Cs+ at the B-site to enhance X-ray absorption while retaining low toxicity. The effects of halide modulation on the physical properties and device performance are systematically investigated. Among the variants, MDABCO-CsBr3 exhibited superior environmental stability, attributed to the optimal ionic radius and high chemical stability of Br-. This stability is further enhanced by a higher tolerance factor, which promotes a stable 3D cubic structure and suppresses ion migration within the crystal. Consequently, MDABCO-CsBr3-based X-ray detectors demonstrated reduced ionic migration, minimal dark current drift, and a stable current response under X-ray exposure, achieving a high sensitivity of 4124 mu C Gy-1 cm-2 and a low detection limit of 0.45 mu Gy s-1. Moreover, the devices exhibit excellent thermal stability, operating effectively at temperatures up to 130 degrees C. These results highlight MDABCO-CsBr3 as a promising candidate for stable and efficient X-ray detection, expanding the applicability of molecular perovskites in advanced radiation detection technologies.
Keyword ：
cesium-substituted cesium-substituted environmental stability environmental stability molecular perovskite molecular perovskite X-ray detection X-ray detection
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| GB/T 7714 | Wu, Liang , Wei, Qingsong , Di, Yiming et al. Cesium-Based Molecular Perovskites With Superior Stability for High-Performance X-Ray Detection [J]. | SMALL , 2025 , 21 (10) . |
| MLA | Wu, Liang et al. "Cesium-Based Molecular Perovskites With Superior Stability for High-Performance X-Ray Detection" . | SMALL 21 . 10 (2025) . |
| APA | Wu, Liang , Wei, Qingsong , Di, Yiming , Chen, Fuhai , Qiu, Qiangwen , Shan, Xin et al. Cesium-Based Molecular Perovskites With Superior Stability for High-Performance X-Ray Detection . | SMALL , 2025 , 21 (10) . |
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Organic thermally activated delayed fluorescent (TADF) scintillators hold promising potential for applications in medical radiography and security detection, but the poor X-ray absorption ability and inferior radioluminescence (RL) hampered their progression. Herein, the study has pioneered the development of high-performance TADF Ag(I)-based scintillators from M2X2(dppb)2 (M = Ag, Cu; X = Cl, Br, I) complexes with 1,2-Bis(diphenylphosphino)benzene (dppb) ligand. In comparison with Cu(I) complexes, the Ag(I) series generally exhibited superior scintillation performance. Notably, Ag2Cl2(dppb)2 (Ag1) stands out with exceptionally high RL intensity (approximate to 125% higher than that of CsI:Tl) and a low detection limit of 59.8 nGy s-1. The outstanding scintillation performance of Ag1 is primarily attributed to the synergistic effect of the high exciton utilization efficiency origin from a small singlet-triplet energy gap, enhanced X-ray absorption capacity by heavy atoms, and the high photoluminescence quantum yield (76.47% in ambient atmosphere). By fabricating a flexible film constructed with Ag1 submicron crystalline powders, a high spatial resolution of 25.0 lp mm-1 for X-ray imaging is obtained. It offers new opportunities for utilizing TADF metal-organic complexes for highly efficient X-ray scintillation and imaging. Scintillators with good radioluminescence performance are prepared by combining the TADF mechanism to optimize the utilization of triplet excitons, coupled with increased X-ray absorption through heavy atoms, verifying the advantages of Ag(I)-halide complexes on radioluminescence. Besides, the influence of halogens on photoluminescence and radioluminescence are investigated. As a practical application, Ag2Cl2(dppb)2 is applied to fabricate flexible scintillator films, achieving high-resolution imaging of 25 lp mm-1. image
Keyword ：
scintillators scintillators silver-based complexes silver-based complexes thermally activated delayed fluorescence thermally activated delayed fluorescence X-ray imaging X-ray imaging
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| GB/T 7714 | Yuan, Siqi , Zhang, Guozhen , Chen, Fuhai et al. Thermally Activated Delayed Fluorescent Ag(I) Complexes for Highly Efficient Scintillation and High-Resolution X-Ray Imaging [J]. | ADVANCED FUNCTIONAL MATERIALS , 2024 , 34 (33) . |
| MLA | Yuan, Siqi et al. "Thermally Activated Delayed Fluorescent Ag(I) Complexes for Highly Efficient Scintillation and High-Resolution X-Ray Imaging" . | ADVANCED FUNCTIONAL MATERIALS 34 . 33 (2024) . |
| APA | Yuan, Siqi , Zhang, Guozhen , Chen, Fuhai , Chen, Jingru , Zhang, Yang , Di, Yiming et al. Thermally Activated Delayed Fluorescent Ag(I) Complexes for Highly Efficient Scintillation and High-Resolution X-Ray Imaging . | ADVANCED FUNCTIONAL MATERIALS , 2024 , 34 (33) . |
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Phosphates are ideal candidates in the search for deep ultraviolet (DUV) nonlinear optical (NLO) materials due to their wide DUV transmission. However, the small optical anisotropy of the highly symmetric [PO4](3-) tetrahedron hinders phase matching (PM) in the DUV wavelength range. In this work, the polar tetrahedron [PO2(NHCONH2)(2)](-), which combines the pi-conjugated urea unit and the non-pi-conjugated [PO4](3-) unit via covalent bonds, is proposed as a new DUV NLO-active unit. [PO2(NHCONH2)(2)](-) tetrahedron exhibits greatly improved polarizability, anisotropy, and hyperpolarizability while maintaining a large highest occupied molecular orbital-lowest unoccupied molecular orbital gap. Accordingly, two DUV transparent alkali metal N, N-bis(aminocarbonyl)-phosphorodiamidates [A[PO2(NHCONH2)(2)] (A = K, Rb)] are screened out, and their nonlinear properties are systematically evaluated by first-principles methods. The results show that K[PO2(NHCONH2)(2)] (KPOU) achieves significant enhancements in multiple properties compared to the existing phosphate DUV NLO materials, including a strong SHG effect (3.44 x KDP) and the largest birefringence (0.088@532 nm) for DUV PM. Moreover, the shortest PM wavelength (lambda(PM)) of KPOU is 196 nm, making it a promising DUV NLO candidate for practical applications. This work proposes an excellent NLO-active unit and offers a new direction for exploring novel high-performance DUV NLO materials.
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| GB/T 7714 | Chen, Fuhai , Mo, Fuxiang , Chen, Hongming et al. KPO2(NHCONH2)2: A Promising Deep-Ultraviolet Nonlinear Optical Phosphate Containing Polar [PO2(NHCONH2)2]- Tetrahedra [J]. | CHEMISTRY OF MATERIALS , 2024 , 36 (6) : 2985-2992 . |
| MLA | Chen, Fuhai et al. "KPO2(NHCONH2)2: A Promising Deep-Ultraviolet Nonlinear Optical Phosphate Containing Polar [PO2(NHCONH2)2]- Tetrahedra" . | CHEMISTRY OF MATERIALS 36 . 6 (2024) : 2985-2992 . |
| APA | Chen, Fuhai , Mo, Fuxiang , Chen, Hongming , Lin, Mei-Jin , Chen, Yong . KPO2(NHCONH2)2: A Promising Deep-Ultraviolet Nonlinear Optical Phosphate Containing Polar [PO2(NHCONH2)2]- Tetrahedra . | CHEMISTRY OF MATERIALS , 2024 , 36 (6) , 2985-2992 . |
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The development of high-quality organic scintillators encounters challenges primarily associated with the weak X-ray absorption ability resulting from the presence of low atomic number elements. An effective strategy involves the incorporation of halogen-containing molecules into the system through co-crystal engineering. Herein, we synthesized a highly fluorescent dye, 2,5-di(4-pyridyl)thiazolo[5,4-d]thiazole (Py2TTz), with a fluorescence quantum yield of 12.09%. Subsequently, Py2TTz was co-crystallized with 1,4-diiodotetrafluorobenzene (I2F4B) and 1,3,5-trifluoro-2,4,6-triiodobenzene (I3F3B) obtaining Py2TTz-I2F4 and Py2TTz-I3F3. Among them, Py2TTz-I2F4 exhibited exceptional scintillation properties, including an ultrafast decay time (1.426 ns), a significant radiation luminescence intensity (146% higher than Bi3Ge4O12), and a low detection limit (70.49 nGy s-1), equivalent to 1/78th of the detection limit for medical applications (5.5 mu Gy s-1). This outstanding scintillation performance can be attributed to the formation of halogen-bonding between I2F4B and Py2TTz. Theoretical calculations and single-crystal structures demonstrate the formation of halogen-bond-induced rather than pi-pi-induced charge-transfer cocrystals, which not only enhances the X-ray absorption ability and material conductivity under X-ray exposure, but also constrains molecular vibration and rotation, and thereby reducing non-radiative transition rate and sharply increasing its fluorescence quantum yields. Based on this, the flexible X-ray film prepared based on Py2TTz-I2F4 achieved an ultrahigh spatial resolution of 26.8 lp per mm, underscoring the superiority of this strategy in developing high-performance organic scintillators. Two organic halogen co-crystal scintillators with strong halogen-bond-induced charge-transfer interactions enable a fast response, low detection limit and ultra-high-resolution imaging.
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| GB/T 7714 | Chen, Yu-Hua , Zhang, Guo-Zhen , Chen, Fu-Hai et al. Halogen-bonded charge-transfer co-crystal scintillators for high-resolution X-ray imaging [J]. | CHEMICAL SCIENCE , 2024 , 15 (20) : 7659-7666 . |
| MLA | Chen, Yu-Hua et al. "Halogen-bonded charge-transfer co-crystal scintillators for high-resolution X-ray imaging" . | CHEMICAL SCIENCE 15 . 20 (2024) : 7659-7666 . |
| APA | Chen, Yu-Hua , Zhang, Guo-Zhen , Chen, Fu-Hai , Zhang, Shu-Quan , Fang, Xin , Chen, Hong-Ming et al. Halogen-bonded charge-transfer co-crystal scintillators for high-resolution X-ray imaging . | CHEMICAL SCIENCE , 2024 , 15 (20) , 7659-7666 . |
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Semiconductive metal-organic frameworks (MOFs) with donor-acceptor (D-A) characteristics have garnered attractive attention due to their capacity for separating and transferring photogenerated charges, making them promising candidates for high-performance X-ray detectors. However, the low charge transfer efficiency between the metal nodes and organic ligands limits the X-ray-to-electricity conversion efficiency of these materials. Herein, an additional photoactive donor (D') is introduced by incorporating a heavy atom-containing polyoxometalate (POM) [alpha-SiW12O40](4-) into a binary {[Nibcbp(H2O)(2)](H2O)(4)Cl}(n) (Ni-bcbp, bcbp: H(2)bcbp2Cl = 1,1 '-bis(4-carboxyphenyl)(4,4 '-bipyridinium) dichloride) MOF, resulting in a semiconductive ternary D-D'-A framework {[Ni-2(bcbp)(2)(H2O)(4)(DMA)](SiW12O40)}(n) (SiW@Ni-bcbp, DMA: dimethylacetamide). The obtained material features an unprecedented porous 8-connected bcu-net structure that accommodates nanoscale [alpha-SiW12O40](4-) counterions, displaying uncommon optoelectronic responses. In contrast to binary Ni-bcbp, the SiW@Ni-bcbp framework exhibits distinctive photochromism and robust X-ray responsiveness, which can be attributed to the synergistic effects of the electron reservoir and multiple photoinduced electron transfer originating from the POMs. As a result, the X-ray detector based on SiW@Ni-bcbp demonstrates a sensitivity of 5741.6 mu C Gy(air)(-1) cm(-2) with a low detection limit of 0.49 mu Gy(air) s(-1). Moreover, the devices demonstrated the capability of producing clearness X-ray images, providing a feasible and stable solution for constructing high-performance direct X-ray detectors.
Keyword ：
direct X-ray detector direct X-ray detector metal-organic framework metal-organic framework multiple electron transfer multiple electron transfer photoelectric conversion photoelectric conversion
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| GB/T 7714 | Wei, Qingsong , Liu, Jingyan , Wu, Liang et al. Multiple Electron Transfer in Semiconductive Ternary D-D'-A Metal-Organic Framework for Enhanced X-Ray Detection and Imaging [J]. | SMALL , 2024 . |
| MLA | Wei, Qingsong et al. "Multiple Electron Transfer in Semiconductive Ternary D-D'-A Metal-Organic Framework for Enhanced X-Ray Detection and Imaging" . | SMALL (2024) . |
| APA | Wei, Qingsong , Liu, Jingyan , Wu, Liang , Chen, Fuhai , Ye, Yuanji , Zhang, Shuquan et al. Multiple Electron Transfer in Semiconductive Ternary D-D'-A Metal-Organic Framework for Enhanced X-Ray Detection and Imaging . | SMALL , 2024 . |
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Energy storage devices with high power and energy density are in demand owing to the rapidly growing population, and lithium-ion batteries (LIBs) are promising rechargeable energy storage devices. However, there are many issues associated with the development of electrode materials with a high theoretical capacity, which need to be addressed before their commercialization. Extensive research has focused on the modification and structural design of electrode materials, which are usually expensive and sophisticated. Besides, polymer binders are pivotal components for maintaining the structural integrity and stability of electrodes in LIBs. Polyvinylidene difluoride (PVDF) is a commercial binder with superior electrochemical stability, but its poor adhesion, insufficient mechanical properties, and low electronic and ionic conductivity hinder its wide application as a high-capacity electrode material. In this review, we highlight the recent progress in developing different polymeric materials (based on natural polymers and synthetic non-conductive and electronically conductive polymers) as binders for the anodes and cathodes in LIBs. The influence of the mechanical, adhesion, and self-healing properties as well as electronic and ionic conductivity of polymers on the capacity, capacity retention, rate performance and cycling life of batteries is discussed. Firstly, we analyze the failure mechanisms of binders based on the operation principle of lithium-ion batteries, introducing two models of "interface failure" and "degradation failure". More importantly, we propose several binder parameters applicable to most lithium-ion batteries and systematically consider and summarize the relationships between the chemical structure and properties of the binder at the molecular level. Subsequently, we select silicon and sulfur active electrode materials as examples to discuss the design principles of the binder from a molecular structure point of view. Finally, we present our perspectives on the development directions of binders for next-generation high-energy-density lithium-ion batteries. We hope that this review will guide researchers in the further design of novel efficient binders for lithium-ion batteries at the molecular level, especially for high energy density electrode materials. The design of binders for lithium-ion batteries is highlighted, with an emphasis on key parameters affecting device performance and failure mechanisms. These issues are discussed in detail using the example of a silicon anode and a sulfur cathode.
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| GB/T 7714 | He, Qiang , Ning, Jiaoyi , Chen, Hongming et al. Achievements, challenges, and perspectives in the design of polymer binders for advanced lithium-ion batteries [J]. | CHEMICAL SOCIETY REVIEWS , 2024 , 53 (13) : 7091-7157 . |
| MLA | He, Qiang et al. "Achievements, challenges, and perspectives in the design of polymer binders for advanced lithium-ion batteries" . | CHEMICAL SOCIETY REVIEWS 53 . 13 (2024) : 7091-7157 . |
| APA | He, Qiang , Ning, Jiaoyi , Chen, Hongming , Jiang, Zhixiang , Wang, Jianing , Chen, Dinghui et al. Achievements, challenges, and perspectives in the design of polymer binders for advanced lithium-ion batteries . | CHEMICAL SOCIETY REVIEWS , 2024 , 53 (13) , 7091-7157 . |
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Chiral self-discrimination plays a critical role in supramolecular chemistry and materials science. However, an ideal strategy for achieving chiral self-discrimination remains elusive due to the inevitable nonspecific binding of incorrect enantiomers, and insufficient intrinsic optical activity of chiral molecules. Herein, a novel 1,1 '-binaphthol (BINOL) derivative with an imide group fused at the peri-position of one naphthol scaffold is developed, which combines the dual functionalities of aggregation-induced emission characteristic of BINOLs, and high emission of 1,8-naphthalimides. The multiple molecular recognition between two hydroxyl groups in BINOL units and two carbonyl groups in 1,8-naphthalimide moieties endows the precise chiral self-discrimination behaviors. As expected, the homochiral aggregates exhibit reversible phase transitions, switching from non-emission to bright green emission upon absorption and desorption of methanol vapor. In contrast, the heterochiral conglomerates exhibit irreversible yellow emission changes due to the impact of chiral self-discrimination. Such chiral self-discrimination-induced luminescence vapochromism can be further applied to high-level anti-counterfeiting and data encryption. This work provides a new perspective on smart chiral organic materials based on chiral self-discrimination. Novel binaphthol-derived imide dyes with C1 axial chirality and racemism-enhanced emission are developed, which display chiral self-discrimination-induced luminescence vapochromism for anti-counterfeiting and data encryption. image
Keyword ：
aggregation-induced emission aggregation-induced emission binaphthol Imides binaphthol Imides chiral self-discrimination chiral self-discrimination data encryption data encryption luminescence vapochromism luminescence vapochromism
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| GB/T 7714 | Zhang, Yang , Chen, Hong-Ming , Lin, Mei-Jin . Chiral Self-Discrimination Induced Luminescence Vapochromism of Binaphthol Imides for Anti-Counterfeiting and Data Encryption [J]. | ADVANCED OPTICAL MATERIALS , 2024 , 12 (24) . |
| MLA | Zhang, Yang et al. "Chiral Self-Discrimination Induced Luminescence Vapochromism of Binaphthol Imides for Anti-Counterfeiting and Data Encryption" . | ADVANCED OPTICAL MATERIALS 12 . 24 (2024) . |
| APA | Zhang, Yang , Chen, Hong-Ming , Lin, Mei-Jin . Chiral Self-Discrimination Induced Luminescence Vapochromism of Binaphthol Imides for Anti-Counterfeiting and Data Encryption . | ADVANCED OPTICAL MATERIALS , 2024 , 12 (24) . |
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Correction for 'Halogen-bonded charge-transfer co-crystal scintillators for high-resolution X-ray imaging' by Yu-Hua Chen et al., Chem. Sci., 2024, https://doi.org/10.1039/d4sc00735b.
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| GB/T 7714 | Chen, Yu-Hua , Zhang, Guo-Zhen , Chen, Fu-Hai et al. Halogen-bonded charge-transfer co-crystal scintillators for high-resolution X-ray imaging (20 Apr, 10.1039/d4sc00735b, 2024) [J]. | CHEMICAL SCIENCE , 2024 , 15 (21) : 8249-8249 . |
| MLA | Chen, Yu-Hua et al. "Halogen-bonded charge-transfer co-crystal scintillators for high-resolution X-ray imaging (20 Apr, 10.1039/d4sc00735b, 2024)" . | CHEMICAL SCIENCE 15 . 21 (2024) : 8249-8249 . |
| APA | Chen, Yu-Hua , Zhang, Guo-Zhen , Chen, Fu-Hai , Zhang, Shu-Quan , Fang, Xin , Chen, Hong-Ming et al. Halogen-bonded charge-transfer co-crystal scintillators for high-resolution X-ray imaging (20 Apr, 10.1039/d4sc00735b, 2024) . | CHEMICAL SCIENCE , 2024 , 15 (21) , 8249-8249 . |
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