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学者姓名：陈飞飞
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In this study, divalent calcium cation with large radius and trivalent yttrium cation with small radius were introduced to develop co-stabilized zirconia ceramics with both superior mechanical properties and aging resistance. Through a reverse coprecipitation-hydrothermal method, a series of ultrafine xCaO-yY2O3-ZrO2 (x = 2.0, 3.0, y = 0.5, 1.0, 1.5, 2.0) raw powders with high quality were fabricated for the production of nanostructured ceramics via low-temperature pressurelessly sintering. The sintering process was optimized by investigating the effects of sintering temperature on densification, grain growth and phase evolution. The minimally doped 2.0CaO-0.5Y2O3-ZrO2 ceramic retained pure tetragonal phase at room temperature, achieving a balance of excellent toughness and high aging resistance. The impacts of chemical composition on microstructure, hardness, toughness and aging resistance were examined for these xCaO-yY2O3-ZrO2 (x = 2.0, 3.0, y = 0.5, 1.0, 1.5, 2.0) ceramics. The segregation of calcium and yttrium cations at grain boundaries effectively tailored the microstructure. It was observed that substituting small trivalent yttrium cations for large divalent calcium cations effectively enhanced the aging resistance without sacrificing mechanical properties, due to the strengthened grain boundaries and asymmetrical distribution of cations among grains. This work not only produces low-doped zirconia ceramics with both excellent mechanical properties and aging resistance, but also presents straightforward method for preparation of high-quality raw powders and delicate microstructural engineering during sintering for developing advanced structural ceramics. © 2025 Elsevier Ltd and Techna Group S.r.l.
Keyword ：
Ceramic materials Ceramic materials Grain growth Grain growth High temperature engineering High temperature engineering Low temperature production Low temperature production Microstructural evolution Microstructural evolution Powders Powders Rockwell hardness Rockwell hardness Sintering Sintering Yttria stabilized zirconia Yttria stabilized zirconia Yttrium Yttrium Yttrium metallography Yttrium metallography
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| GB/T 7714 | Feng, Ya-Nan , Wang, Fei-Fan , Xiao, Weiwei et al. Mechanical properties and aging resistance of calcia-yttria co-stabilized zirconia: from powder to ceramic [J]. | Ceramics International , 2025 , 51 (13) : 17368-17378 . |
| MLA | Feng, Ya-Nan et al. "Mechanical properties and aging resistance of calcia-yttria co-stabilized zirconia: from powder to ceramic" . | Ceramics International 51 . 13 (2025) : 17368-17378 . |
| APA | Feng, Ya-Nan , Wang, Fei-Fan , Xiao, Weiwei , Xia, Yan , Wei, Bin , Wang, Shuaihua et al. Mechanical properties and aging resistance of calcia-yttria co-stabilized zirconia: from powder to ceramic . | Ceramics International , 2025 , 51 (13) , 17368-17378 . |
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Heterojunction photocatalysts, which consist of two or more semiconductors, have garnered significant attention owing to their extensive benefits, including a broad-spectrum response, efficient carrier separation and migration, as well as robust redox capabilities. Among the myriad of semiconductors, graphitic carbon nitride (g-C3N4) and zinc indium sulfide (ZnIn2S4) have been extensively researched due to their low toxicity, straightforward and scalable synthesis processes, controllable microstructures, and exceptional chemical stability. Recently, there has been a trend towards integrating these two semiconductors to complement each other's strengths. Consequently, a systematic summary and outlook on g-C3N4/ZnIn2S4 heterojunction photocatalysts is both urgent and valuable. This review summarizes the advancements in the g-C3N4/ZnIn2S4 heterojunctions in the last 10 years. We first analyzed the charge-transfer mechanisms in the type-I, type-II, Z-scheme and S-scheme heterojunctions. Then the typical synthesis methods employed for creating g-C3N4/ZnIn2S4 heterojunctions are introduced. Subsequently, we delve into the regulation strategies for g-C3N4/ZnIn2S4 heterojunctions, including morphology optimization, heteroatom doping, defect engineering, and the construction of multinary composites. The design concept and superiorities of these strategies are thoroughly discussed. Following this, we systematically showcase the photocatalytic applications of g-C3N4/ZnIn2S4 heterojunctions, encompassing CO2 reduction, H2 evolution, pollutant degradation, H2O2 production, biomass conversion, photoelectrochemical sensors, and so forth. Last, we propose the challenges that lie ahead in future research endeavors. This comprehensive review is expected to provide an instructive guideline for rational design and applications of g-C3N4/ZnIn2S4 heterojunctions.
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| GB/T 7714 | Lu, Yongjun , Zhuang, Zanyong , Li, Lingyun et al. Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts [J]. | JOURNAL OF MATERIALS CHEMISTRY A , 2025 , 13 (7) : 4718-4745 . |
| MLA | Lu, Yongjun et al. "Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts" . | JOURNAL OF MATERIALS CHEMISTRY A 13 . 7 (2025) : 4718-4745 . |
| APA | Lu, Yongjun , Zhuang, Zanyong , Li, Lingyun , Chen, Fei-Fei , Wei, Peishu , Yu, Yan . Advancements and challenges in g-C3N4/ZnIn2S4 heterojunction photocatalysts . | JOURNAL OF MATERIALS CHEMISTRY A , 2025 , 13 (7) , 4718-4745 . |
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The eradication of bacteria and the degradation of organic pollutants in contaminated water hold paramount importance for both ecological systems and human health. Herein, we report the development of a bifunctional material, constructed from metal-organic frameworks (MOFs) and their derived metal/carbon composites, which demonstrates remarkable efficacy in disinfecting and degrading dyes and antibiotics. Notably, the synthesized Co-MOFs and their derived Co@C composites exhibit a progressive enhancement in antibacterial activity: (i) In comparison to 3D Co-MOF polyhedra, 2D Co-MOF nanosheets demonstrate superior efficacy in killing both E. coli and S. aureus. This enhanced antibacterial performance is attributed to the generation of a higher quantity of reactive oxygen species and the unique nanosheet structure. (ii) Following heat treatment of the 2D Co-MOFs, carbon-encapsulated cobalt nanoparticles (Co@C) are obtained. These nanoparticles further reduce the minimum inhibitory concentration (MIC) and minimum bactericidal concentration (MBC) values compared to the pristine 2D Co-MOFs. (iii) Additionally, the carbon layers impart exceptional photothermal properties to the materials, leading to a further enhancement in antibacterial efficacy. With irradiation with NIR for just 10 min, the bactericidal rates against E. coli and S. aureus can be as high as 97 % and 100 %, respectively. Furthermore, the cobalt nanoparticles within the carbon layers serve as catalysts for Fenton-like catalytic degradation of organic pollutants in the presence of peroxymonosulfate. Nearly 100 % of cationic Methylene Blue and anionic Congo Red, as well as 77 % of Enrofloxacin, can be degraded within 60 seconds.
Keyword ：
Antibacterial Antibacterial Degradation Degradation Metal-organic frameworks Metal-organic frameworks Organic pollutants Organic pollutants Photothermal Photothermal
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| GB/T 7714 | He, Yupeng , Lin, Ang , Lin, Gengbing et al. MOF-based bifunctional materials enables stepwise enhancement in antibacterial activity and Fenton-like catalytic degradation of organic pollutants [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2025 , 1024 . |
| MLA | He, Yupeng et al. "MOF-based bifunctional materials enables stepwise enhancement in antibacterial activity and Fenton-like catalytic degradation of organic pollutants" . | JOURNAL OF ALLOYS AND COMPOUNDS 1024 (2025) . |
| APA | He, Yupeng , Lin, Ang , Lin, Gengbing , Wu, Zhi-Chao , Chen, Fei-Fei , Guo, Nan et al. MOF-based bifunctional materials enables stepwise enhancement in antibacterial activity and Fenton-like catalytic degradation of organic pollutants . | JOURNAL OF ALLOYS AND COMPOUNDS , 2025 , 1024 . |
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The strong CO2 adsorption and facile CO desorption are a trade-off issue for CO2-to-CO photoreduction pathways. Synchronous optimization of these two steps remains a substantial hurdle and has been less explored. Herein, an O/N mixed coordinated Co-NTA (NTA: nitrilotriacetic acid), featuring an ultralong nanofiber architecture, is reported for efficient CO2 photoreduction. The mixed coordination can regulate the positions of d-band center of Co sites and also d-p orbital coupling with coordination atoms, which are recognized as main activity descriptors. Consequently, free energies of both steps of CO2 ->*CO2 and *CO -> CO are well optimized, making the CO2-to-CO photoreduction pathways more favorable thermodynamically. By contrast, the classic N-coordinated Co-MeIm (MeIm: 2-methylimidazole) and O-coordinated Co-BDC (BDC: 1,4-benzenedicarboxylic acid) suffer from unfavorable CO2 adsorption and intractable CO desorption, respectively. In addition, achiral NTA molecules can direct the growth of Co-NTA into one-dimensional (1D) nanofibers, while Co-BDC and Co-MeIm possess typical 2D nanosheet and 3D polyhedron architectures. The fast electron transport along the axis directions makes charge-transfer kinetics most efficient over 1D Co-NTA. The thermodynamic and kinetic benefits jointly contribute to the 1.8-fold increase in CO production over 1D Co-NTA.
Keyword ：
d-band center d-band center Metal-organic frameworks Metal-organic frameworks Nanofibers Nanofibers Orbital coupling Orbital coupling
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| GB/T 7714 | Yang, Yong , Jiang, Jianfeng , Feng, Ya-Nan et al. Manipulating d-band center and d-p orbital coupling to mitigate adsorption-desorption trade-off for efficient CO2-to-CO photoreduction over MOF nanofibers [J]. | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2025 , 379 . |
| MLA | Yang, Yong et al. "Manipulating d-band center and d-p orbital coupling to mitigate adsorption-desorption trade-off for efficient CO2-to-CO photoreduction over MOF nanofibers" . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY 379 (2025) . |
| APA | Yang, Yong , Jiang, Jianfeng , Feng, Ya-Nan , Zhuang, Zanyong , Chen, Fei-Fei , Zhang, Dantong et al. Manipulating d-band center and d-p orbital coupling to mitigate adsorption-desorption trade-off for efficient CO2-to-CO photoreduction over MOF nanofibers . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2025 , 379 . |
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Enhancing the flame retardancy of cable tape coatings while maintaining low electrical conductivity during fire incidents remains a significant challenge. In this study, we address this issue by incorporating waste aluminum sludge (AS) into an intumescent flame retardant (IFR)/vinyl acetate-ethylene (VAE) coatings, thus optimizing the flame retardancy, mechanical properties, and electrical insulation of fiberglass tapes. AS, composed of boehmite and bayerite phases with a sheet-like structure, interacts chemically with IFR/VAE during combustion, yielding thermally stable minerals (Al(PO3)3 and AlPO4). Concurrently, its layered morphology promotes the formation of a compact and well-ordered carbonaceous char. The resulting hybrid mineral/carbon char acts as a robust physical barrier, effectively impeding heat and mass transfer, while disrupting the conductive carbon network. This dual mechanism leads to a remarkable enhancement in fire safety and electrical insulation performance, including: a 77.2 % reduction in peak heat release rate, a 29.0 % decrease in total heat release, a 58.5 % suppression in total smoke production, a 759.2 % increase in surface resistivity, a 45.7 % improvement in tensile strength, and a 2.4 % rise in limiting oxygen index. This work not only presents a sustainable strategy for upcycling industrial waste into high-performance flame retardants but also elucidates the mechanistic role of aluminum oxides/hydroxides in modifying the combustion behavior of IFR systems.
Keyword ：
Cable tapes Cable tapes Electrical properties Electrical properties Flame retardants Flame retardants Intumescent Intumescent Waste aluminum sludge Waste aluminum sludge
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| GB/T 7714 | Yuan, Chenggong , Li, Shang , Zou, Hongfei et al. Extraordinary roles of waste aluminum sludge in enhancing flame retardancy, smoke suppression and electric insulation of intumescent flame-retardant coating for reliable cable tapes [J]. | POLYMER DEGRADATION AND STABILITY , 2025 , 242 . |
| MLA | Yuan, Chenggong et al. "Extraordinary roles of waste aluminum sludge in enhancing flame retardancy, smoke suppression and electric insulation of intumescent flame-retardant coating for reliable cable tapes" . | POLYMER DEGRADATION AND STABILITY 242 (2025) . |
| APA | Yuan, Chenggong , Li, Shang , Zou, Hongfei , Lu, Baokun , Zhang, Cancan , Chen, Kongjian et al. Extraordinary roles of waste aluminum sludge in enhancing flame retardancy, smoke suppression and electric insulation of intumescent flame-retardant coating for reliable cable tapes . | POLYMER DEGRADATION AND STABILITY , 2025 , 242 . |
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Traditional nanofiltration membranes allow high rejection of low molecular weight organic matter, yet suffer from a low flux and a high operation pressure, and they pose an environmental concern because they are made of petroleum-based polymers. Herein, a novel environmentally friendly filter membrane for ultrafast molecular separation has been developed using natural and artificial biomaterials as building units. Cellulose micron fibers, a natural biopolymer, serve as a stable substrate for the growth of hydroxyapatite (HAP) nanowire bunches, which are the main inorganic components of bones and teeth. The vertically aligned HAP nanowire bunches provide abundant nanoscale surfaces and confinement space for the attachment of dopamine and subsequently self-polymerization into polydopamine (PDA) sub-micron particles, which are a melanin-like bioactive polymer. On the one hand, the as-built micro-nano hierarchical configuration enables ultrahigh permeance (>6000 L m(-2) h(-1) bar(-1)) through the filter membrane at a low pressure (62 mbar). On the other hand, molecular dynamics simulations reveal that synergy between multiple molecular interactions of HAP and PDA contributes to the universal separation of different organic pollutants from water (i.e., cationic and anionic dyes and antibiotics) at a high removal rate of > 97 %. Overall, this work ingeniously uses biocompatible biomaterials to build a hierarchical filter membrane, thereby enabling ultrafast and efficient molecular separation.
Keyword ：
Biomaterials Biomaterials Cellulose Cellulose Filter Membranes Filter Membranes Hydroxyapatite Nanowires Hydroxyapatite Nanowires Polydopamine Polydopamine
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| GB/T 7714 | Wu, Linhan , Shi, Dehuan , Lin, Fuwang et al. Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 361 . |
| MLA | Wu, Linhan et al. "Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study" . | SEPARATION AND PURIFICATION TECHNOLOGY 361 (2025) . |
| APA | Wu, Linhan , Shi, Dehuan , Lin, Fuwang , Chen, Fei-Fei , Yang, Chengkai , Yu, Yan . Ultrafast molecular separation through all-biomaterial membranes with a hierarchical configuration and mechanism study . | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 361 . |
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Regulating charge transfer and reaction pathways are effective strategies for boosting photocatalytic CO2 reduction. Herein, Co3O4/ZrO2 mesoporous octahedrons are synthesized through facile pyrolysis of UIO-66@ZIF-67 core/shell octahedrons. The as-obtained Co3O4/ZrO2 mesoporous octahedrons are assembled by highly dispersive and small-sized nanoparticles, with 13 nm average particle size and 5.8 nm pore width, leading to a high specific surface area of 43.11 m(2) g(-1). Benefiting from active-site engineering, the charge-transfer kinetics and CO2 adsorption are successfully enhanced. In addition, density functional theory calculations reveal that ZrO2 tailors the reaction pathway of CO2 reduction by promoting CO2 activation to *CO2 and intermediate formation (*COOH and *CO), as well as decreasing the energy barrier of the rate-limiting step (*CO -> CO). Thus, the Co3O4/ZrO2 mesoporous octahedrons afford a turnover frequency of 28.82 h(-1), 16.95-fold larger than pure Co3O4.
Keyword ：
CO2 reduction CO2 reduction mesoporous mesoporous metal-organic frameworks metal-organic frameworks oxides oxides photocatalysis photocatalysis
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| GB/T 7714 | Liu, Haibing , Qiu, Yanbin , Gan, Wenxiu et al. MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction [J]. | SCIENCE CHINA-MATERIALS , 2024 , 67 (2) : 588-597 . |
| MLA | Liu, Haibing et al. "MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction" . | SCIENCE CHINA-MATERIALS 67 . 2 (2024) : 588-597 . |
| APA | Liu, Haibing , Qiu, Yanbin , Gan, Wenxiu , Zhuang, Guoxin , Chen, Fei-Fei , Yang, Chengkai et al. MOF-derived Co3O4/ZrO2 mesoporous octahedrons with optimized charge transfer and intermediate conversion for efficient CO2 photoreduction . | SCIENCE CHINA-MATERIALS , 2024 , 67 (2) , 588-597 . |
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Flexible metal-organic framework (MOF) films are greatly desired for the separation of hazardous molecules and ions from wastewater. The current MOF films are usually horizontally deposited on the substrates, and thus restricted by brittleness, low exposure of surface area, as well as poor separation functions. Here, an organic-inorganic mixed substrate is firstly fabricated by growing hydroxyapatite (HA) nanowire arrays on the cellulose fiber (CF). Subsequently, MIL-100(Fe) nanocrystals are assembled on the surfaces of HA nanowire arrays through a layer-by-layer manner, leading to a unique vertical MOF film. The resulting vertical MOF films show competitive advantages over the horizontal counterparts: (i) they show excellent flexibility and they are tolerant to serious physical damage; (ii) they have multiple separation functions including ion exchange of HA, excellent adsorption of MOFs, and strong electrostatic interaction of CF; and (iii) the agglomeration of MIL-100(Fe) nanocrystals is effectively suppressed. Therefore, the average roughness, specific surface area, and average pore size of films are optimized. As a result, the vertical MOF films show universal separation of positively/ negatively-charged dyes and Pb2+ ion, with high removal rates of > 94 %. More appealing, the mixed pollutants in the complex wastewater can be one-step separated through the vertical MOF films, with high removal rates of > 96 %.
Keyword ：
Dyes Dyes Heavy metal ions Heavy metal ions Hydroxyapatite Hydroxyapatite Metal -organic frameworks Metal -organic frameworks Separation Separation
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| GB/T 7714 | Gan, Wenxiu , Zheng, Ziyang , Yan, Jiawei et al. Vertical MOF film supported on an organic-inorganic mixed substrate for complex wastewater purification [J]. | APPLIED SURFACE SCIENCE , 2024 , 652 . |
| MLA | Gan, Wenxiu et al. "Vertical MOF film supported on an organic-inorganic mixed substrate for complex wastewater purification" . | APPLIED SURFACE SCIENCE 652 (2024) . |
| APA | Gan, Wenxiu , Zheng, Ziyang , Yan, Jiawei , He, Xi , Zhuang, Zanyong , Chen, Fei-Fei et al. Vertical MOF film supported on an organic-inorganic mixed substrate for complex wastewater purification . | APPLIED SURFACE SCIENCE , 2024 , 652 . |
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Beyond traditional paper, multifunctional nanopaper has received much attention in recent years. Currently, many nanomaterials have been successfully used as building units of nanopaper. However, it remains a great challenge to prepare flexible and freestanding metal-organic framework (MOF) nanopaper owing to the low aspect ratio and brittleness of MOF nanocrystals. Herein, this work develops a flexible and free-standing MOF nanopaper with MOF nanowires as building units. The manganese-based MOF (Mn-MOF) nanowires with lengths up to 100 mu m are synthesized by a facile solvothermal method. Through a paper-making technique, the Mn-MOF nanowires interweave with each other to form a three-dimensional architecture, thus creating a flexible and free-standing Mn-MOF nanowire paper. Furthermore, the surface properties can be engineered to obtain high hydrophobicity by modifying polydimethylsiloxane (PDMS) on the surfaces of the Mn-MOF nanowire paper. The water contact angle reaches 130 degrees. As a proof of concept, this work presents two potential applications of the Mn-MOF/PDMS nanowire paper: (i) The as-prepared Mn-MOF/PDMS nanowire paper is compatible with a commercial printer. The as-printed colorful patterns are of high quality, and (ii) benefiting from the highly hydrophobic surfaces, the Mn-MOF/PDMS nanowire paper is able to efficiently separate oil from water.
Keyword ：
flexible flexible free-standing free-standing metal-organic frameworks metal-organic frameworks nanopaper nanopaper nanowires nanowires
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| GB/T 7714 | Yang, Yong , Yang, Zhe , Zhuang, Guoxin et al. Flexible and Free-Standing Metal-Organic Framework Nanowire Paper [J]. | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (23) : 30306-30313 . |
| MLA | Yang, Yong et al. "Flexible and Free-Standing Metal-Organic Framework Nanowire Paper" . | ACS APPLIED MATERIALS & INTERFACES 16 . 23 (2024) : 30306-30313 . |
| APA | Yang, Yong , Yang, Zhe , Zhuang, Guoxin , Feng, Ya-Nan , Chen, Fei-Fei , Yu, Yan . Flexible and Free-Standing Metal-Organic Framework Nanowire Paper . | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (23) , 30306-30313 . |
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The 3-level features of Latent fingerprints (LFPs) are pivotal in linking suspects with problematic or incomplete fingerprint data, constituting one of the most robust forms of evidence. Aggregation-induced emission (AIE) materials, known for their heightened emissive properties in high aggregation states, provide a robust and powerful approach for developing techniques for 3-level details of LFPs. So far, tremendous efforts have been devoted to solving high background fluorescence interference during the 3-level LFPs visualization process. This review commences with an overview of 3-level features and summarizes the interaction and mechanism of visualizing LFPs involving AIE materials and LFPs secretions. Moreover, it encompasses strategies to enhance the contrast and brightness of 3-level LFPs images. We highlight the mechanism of AIE ' s physicochemical properties and their effects on the visualization of 3-level LFPs. Additionally, we provide insights into potential challenges and opportunities in this emerging field. This paper summarizes the recent development regarding AIE materials for 3-level LFPs visualization, focusing on the visualizing mechanism, engineering strategies, and structure-function relationship. Meanwhile, this review also investigates present challenges and the future directions of AIE materials in this booming research field. image
Keyword ：
3-level features 3-level features Aggregation-induced emission Aggregation-induced emission Background interference Background interference Forensic science Forensic science Latent fingerprints detection Latent fingerprints detection
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| GB/T 7714 | Zhuang, GuoXin , Wen, YongLin , Lai, XiangHui et al. Recent Progress of Advanced AIE Materials for Visualization of 3-Level Latent Fingerprints [J]. | CHEMPHOTOCHEM , 2024 , 8 (10) . |
| MLA | Zhuang, GuoXin et al. "Recent Progress of Advanced AIE Materials for Visualization of 3-Level Latent Fingerprints" . | CHEMPHOTOCHEM 8 . 10 (2024) . |
| APA | Zhuang, GuoXin , Wen, YongLin , Lai, XiangHui , Lin, GuoSong , Zhuang, ZanYong , Chen, Fei-Fei et al. Recent Progress of Advanced AIE Materials for Visualization of 3-Level Latent Fingerprints . | CHEMPHOTOCHEM , 2024 , 8 (10) . |
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