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学者姓名：邵宇
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Abstract ：
Absolute cross sections (ACSs) are needed to estimate cellular damage induced by high-energy radiation (HER). Low-energy electrons (LEEs), which are the most numerous secondary particles generated by HER, can trigger hyperthermal reactions in DNA. ACSs for such reactions are essential input parameters to calculate radiobiological effectiveness, particularly in targeted radiotherapy. Using a mathematical model, we generate ACSs from effective damage yields induced by LEE impact on 3197 base-pair plasmid DNA films. Direct or enzyme-revealed conformational damages, quantified by electrophoresis, provide the first complete set of ACSs for inducing crosslinks, double-strand breaks (DSBs), single-strand breaks, base-damage-related crosslinks, non-DSB clustered damages (NDCDs), and isolated base damages. These ACSs are generated across the 1-20 eV range, at one eV intervals. They exhibit a strong energy dependence with maximum values at 10 eV of 3.7 +/- 0.8, 3.5 +/- 0.6, 45.4 +/- 4.1, 2.9 +/- 1.1, 5.1 +/- 1.4, and 54.0 +/- 16.4 x 10-15 cm2, respectively. ACSs for DSBs, NDCDs, and crosslinks clearly indicate that lesions threatening cell function and genetic stability can be generated by a single LEE. At 5 and 10 eV, total damage ACSs are 63% and 80% larger, respectively, than those previously determined for the same plasmids bound to arginine, a constituent of histones protecting DNA.
Keyword ：
cross sections cross sections DNA lesions DNA lesions low-energy electrons low-energy electrons Monte Carlo Monte Carlo radiation damage radiation damage
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| GB/T 7714 | Dong, Yanfang , Huang, Xin , Zhang, Wenlu et al. Hyperthermal Reactions in DNA Triggered by 1-20 eV Electrons: Absolute Cross Sections for Crosslinks, Strand Breaks, Clustered Damages and Base Modifications [J]. | INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES , 2025 , 26 (9) . |
| MLA | Dong, Yanfang et al. "Hyperthermal Reactions in DNA Triggered by 1-20 eV Electrons: Absolute Cross Sections for Crosslinks, Strand Breaks, Clustered Damages and Base Modifications" . | INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES 26 . 9 (2025) . |
| APA | Dong, Yanfang , Huang, Xin , Zhang, Wenlu , Shao, Yu , Cloutier, Pierre , Zheng, Yi et al. Hyperthermal Reactions in DNA Triggered by 1-20 eV Electrons: Absolute Cross Sections for Crosslinks, Strand Breaks, Clustered Damages and Base Modifications . | INTERNATIONAL JOURNAL OF MOLECULAR SCIENCES , 2025 , 26 (9) . |
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Photocatalysis is a green technology which could sustainably convert CO2 into value-added chemicals by using solar energy. Under xenon light irradiation, Mn2O3/MgTi2O5 nanocomposites synthesized by two-step hydrothermal method greatly increase photocatalytic activity of CO2 reduction. The optimal yield 420.53 mu mol g- 1 h- 1 for CH4 is achieved at a ratio 1:10 (W/W) of Mn2O3 to MgTi2O5, with selectivity of 98.1 %, i.e., 4 and 33 times larger than those of individual MgTi2O5 and Mn2O3, respectively. The superior photocatalytic performance is attributed to the formation of S-type heterojunction, valence change of Mn3+/Mn4+, and the bridging effect of Mg migration, which facilitates the separation and transfer of photogenerated electrons and holes. Mn2O3/ MgTi2O5 constructs an efficient redox photocatalytic system composed of a light trapping component (Mn2O3), electron transport channel (Mg penetrating Mn2O3), mutually separated reduction center (MgTi2O5) and oxidation center (Mn2O3). The potential Mn2O3/MgTi2O5 photocatalyst for CO2 reduction provides new insights to design novel efficient photocatalyst composites akin to biological photosynthesis.
Keyword ：
Carbon dioxide reduction Carbon dioxide reduction High selectivity of CH 4 High selectivity of CH 4 Mn 2 O 3 /MgTi 2 O 5 composite Mn 2 O 3 /MgTi 2 O 5 composite Oxidation-reduction system Oxidation-reduction system Photocatalysis Photocatalysis
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| GB/T 7714 | Shen, Yaru , Cai, Jiasheng , Huang, Xin et al. Enhanced photocatalytic CO2 reduction to CH4 by Mn2O3/ MgTi2O5 nanocomposite [J]. | COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS , 2025 , 708 . |
| MLA | Shen, Yaru et al. "Enhanced photocatalytic CO2 reduction to CH4 by Mn2O3/ MgTi2O5 nanocomposite" . | COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS 708 (2025) . |
| APA | Shen, Yaru , Cai, Jiasheng , Huang, Xin , Zheng, Yi , Shao, Yu . Enhanced photocatalytic CO2 reduction to CH4 by Mn2O3/ MgTi2O5 nanocomposite . | COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS , 2025 , 708 . |
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ZnIn2S4 as a promising material for photocatalytic hydrogen evolution (PHE) has attracted significant attention in recent years. However, its high electron-hole recombination rate and low visible light utilization result in poor photocatalytic activity. Herein, ZnIn2S4 nanosheets were first controlled to assemble over electrospun Ni2GeO4 nanofibers to form core-shell structured Ni2GeO4/ZnIn2S4 composites to address the two issues above. Ni2GeO4 nanofibers, acting as both "dispersant" and "support" have prevented the agglomeration of ZnIn2S4 nanosheets and expanded the light-receiving area, thereby exposing more active sites and promoting solar energy utilization. Scanning electron microscopy (SEM) images confirmed the uniform decoration of ZnIn2S4 nanosheets on the surface of Ni2GeO4 nanofibers. Such a core-shell structure facilitates the formation of heterojunction at their interface, which could significantly improve charge separation efficiency. The optimized NGO/ZIS-2 hybrid showed the best PHE rate as high as 7001 mu mol & sdot;g- 1 & sdot;h- 1 under simulated sunlight, which was 3.19 times higher than that of ZnIn2S4 (2196 mu mol & sdot;g- 1 & sdot;h- 1). The cyclic experiments show excellent stability of Ni2GeO4/ZnIn2S4 composite. Based on the results of photoelectrochemical tests, in-situ X-ray photoelectron spectroscopy (XPS) analysis, and density functional theory (DFT) calculations, a more efficient S-scheme charge transfer mode was proposed.
Keyword ：
Core-shell structure Core-shell structure Electrospun Electrospun H 2 evolution H 2 evolution Photocatalysis Photocatalysis
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| GB/T 7714 | Yu, Ziqing , Sun, Meng , Wang, Li et al. Electrospun core-shell structured Ni2GeO4/ZnIn2S4 nanofibers with efficient charge separation efficiency for boosting photocatalytic hydrogen generation [J]. | FUEL , 2025 , 393 . |
| MLA | Yu, Ziqing et al. "Electrospun core-shell structured Ni2GeO4/ZnIn2S4 nanofibers with efficient charge separation efficiency for boosting photocatalytic hydrogen generation" . | FUEL 393 (2025) . |
| APA | Yu, Ziqing , Sun, Meng , Wang, Li , Sun, Jiayu , Yan, Tao , Liu, Qing et al. Electrospun core-shell structured Ni2GeO4/ZnIn2S4 nanofibers with efficient charge separation efficiency for boosting photocatalytic hydrogen generation . | FUEL , 2025 , 393 . |
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Constructing novel surface microstructures for photocatalytic materials could significantly enhance the photocatalytic hydrogen production rate from water splitting. In this work, novel 2D/3D structured CuCo2S4/CdIn2S4 p-n heterojunction photocatalysts for water splitting were successfully prepared by a solvothermal method. The coupling of a 2D CuCo2S4 nanoplate on the surface of 3D flower-like CdIn2S4 microspheres has strengthened the visible light absorption and promoted the charge separation efficiency due to their tight contacting area. The obtained CuCo2S4/CdIn2S4 (CSCIS-2) photocatalyst exhibited a hydrogen production rate of 1320 mu mol g(-1) h(-1), which was fivefold of that for pure CdIn2S4. Additionally, cyclic tests demonstrated improved photoactivity stability of the samples. A series of photoelectrochemical characterizations confirmed the effective suppression of charge carrier recombination in CuCo2S4/CdIn2S4 composite catalysts. Finally, a rational photocatalytic mechanism was proposed based on the semiconductor band theory. This work contributes to the enrichment of sulfide-based research and applications in photocatalysis.
Keyword ：
CuCo2S4/CdIn2S4 CuCo2S4/CdIn2S4 hydrogen evolution hydrogen evolution photocatalyst photocatalyst p-n heterojunction p-n heterojunction water splitting water splitting
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| GB/T 7714 | Rao, Yansen , Sun, Meng , Zhou, Bingzheng et al. Highly Efficient 2D/3D Structured CuCo2S4/CdIn2S4 Composites with a p-n Heterojunction for Boosting Photocatalytic Hydrogen Evolution [J]. | ACS APPLIED ENERGY MATERIALS , 2024 , 7 (13) : 5457-5466 . |
| MLA | Rao, Yansen et al. "Highly Efficient 2D/3D Structured CuCo2S4/CdIn2S4 Composites with a p-n Heterojunction for Boosting Photocatalytic Hydrogen Evolution" . | ACS APPLIED ENERGY MATERIALS 7 . 13 (2024) : 5457-5466 . |
| APA | Rao, Yansen , Sun, Meng , Zhou, Bingzheng , Wang, Zhongpeng , Yan, Tao , Shao, Yu . Highly Efficient 2D/3D Structured CuCo2S4/CdIn2S4 Composites with a p-n Heterojunction for Boosting Photocatalytic Hydrogen Evolution . | ACS APPLIED ENERGY MATERIALS , 2024 , 7 (13) , 5457-5466 . |
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Photocatalytic organic synthesis has attracted much attention in recent years. Herein, a N and C co-decorated mesoporous TiO2 (mp-NCT) photocatalyst was synthesized for selective oxidation of alcohols. Notably, the asprepared mp-NCT composites possess large specific surface areas and mesoporous structures, which could provide sufficient active sites and improve mass transfer. Furthermore, the co-doping of N and C species could not only extend the light absorption, but also tune the valence band of TiO2. Meanwhile, numerous oxygen vacancies and intra-band could be introduced, which helps to reduce the combination of the photogenerated carriers. As a result, the mp-NCT composites show excellent photocatalytic performance towards selective oxidation of benzyl alcohol and its derivatives to corresponding aldehydes under simulated sunlight irradiation. Mechanism studies revealed that the photogenerated electrons, holes and high dynamic equilibrium concentration of O2 center dot- radicals were responsible for the efficient conversion of alcohols to aldehydes.
Keyword ：
functionalized TiO 2 functionalized TiO 2 Mesoporous Mesoporous N -doping N -doping Photocatalysis Photocatalysis Selective oxidation Selective oxidation
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| GB/T 7714 | Cao, Changsheng , Shen, Yaru , Shao, Yu . Rational design of nitrogen and carbon co-decorated mesoporous TiO2 composites for photocatalytic selective oxidation of alcohols [J]. | MOLECULAR CATALYSIS , 2024 , 567 . |
| MLA | Cao, Changsheng et al. "Rational design of nitrogen and carbon co-decorated mesoporous TiO2 composites for photocatalytic selective oxidation of alcohols" . | MOLECULAR CATALYSIS 567 (2024) . |
| APA | Cao, Changsheng , Shen, Yaru , Shao, Yu . Rational design of nitrogen and carbon co-decorated mesoporous TiO2 composites for photocatalytic selective oxidation of alcohols . | MOLECULAR CATALYSIS , 2024 , 567 . |
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ZnIn2S4 has been extensively studied in the field of photocatalytic hydrogen evolution (PHE), but its bulky structure often results in high charge carrier recombination and low light harvesting capability. Herein, efficient hierarchical MGa2O4/ZnIn2S4 (M = Ni, Co) hollow nanofiber photocatalysts with p-n heterojunction were fabricated by an electrospinning-solvothermal method. The hierarchical structure of MGa2O4/ZnIn2S4 composites has facilitated p-n heterojunction formation, promoted the charge separation efficiency, enhanced light harvesting capability, and provided abundant reactive sites. The synergistic effects of MGa2O4 and ZnIn2S4 accelerated the PHE rate by reducing the *H reaction intermediates energy barrier. Under simulated solar light, the NiGa2O4/ZnIn2S4 and CoGa2O4/ZnIn2S4 with optimal proportions delivered outstanding PHE rate of 9292 and 6283 mu mol center dot g(-1)center dot h(- 1), which was 5 and 3 times higher than that of pure ZnIn2S4, respectively. This work opens up an efficient electrospinning-mediated solvothermal strategy for constructing hierarchical ZnIn2S4-based nanofiber composites with excellent PHE performance.
Keyword ：
Electrospinning Electrospinning Photocatalytic H-2 evolution Photocatalytic H-2 evolution P-n heterojunction P-n heterojunction
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| GB/T 7714 | Wang, Li , Sun, Meng , Zhou, Bingzheng et al. Electrospinning mediated solvothermal preparation of hierarchical MGa2O4/ZnIn2S4 (M = Ni, Co) hollow nanofibers with p-n heterojunction for boosting photocatalytic H2 evolution [J]. | FUEL , 2024 , 374 . |
| MLA | Wang, Li et al. "Electrospinning mediated solvothermal preparation of hierarchical MGa2O4/ZnIn2S4 (M = Ni, Co) hollow nanofibers with p-n heterojunction for boosting photocatalytic H2 evolution" . | FUEL 374 (2024) . |
| APA | Wang, Li , Sun, Meng , Zhou, Bingzheng , Rao, Yansen , Yan, Tao , Du, Bin et al. Electrospinning mediated solvothermal preparation of hierarchical MGa2O4/ZnIn2S4 (M = Ni, Co) hollow nanofibers with p-n heterojunction for boosting photocatalytic H2 evolution . | FUEL , 2024 , 374 . |
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Chemoradiation therapy (CRT), which combines a chemotherapeutic drug with ionizing radiation (IR), is the most common cancer treatment. At the molecular level, the binding of Pt-drugs to DNA sensitizes cancer cells to IR, mostly by increasing the damage induced by secondary low-energy (0-20 eV) electrons (LEEs). We investigate such enhancements by binding terpyridine-platinum (Tpy-Pt) to supercoiled plasmid DNA. Fifteen nanometer thick films of Tpy-Pt-DNA complexes in a molar ratio of 5 : 1 were irradiated with monoenergetic electrons of 5 and 10 eV, which principally attach to the DNA bases to form transient anions (TAs) decaying into a multitude of bond-breaking channels. At both energies, the effective yields of crosslinks (CLs), base damage (BD) related CLs, single and double strand breaks (SSBs and DSBs), non-DSB-cluster lesions, loss of supercoiled configuration and base lesions are 6.5 +/- 1.5, 8.8 +/- 3.0, 88 +/- 11, 5.3 +/- 1.3, 9.6 +/- 2.2, 106 +/- 17, 189 +/- 31 x 10(-15) per electron per molecule, and 11.9 +/- 2.6, 19.9 +/- 4.4, 128 +/- 18, 7.7 +/- 3.0, 13.4 +/- 3.9, 144 +/- 19, 229 +/- 42 x 10(-15) per electron per molecule, respectively. DNA damage increased 1.2-4.2-fold due to Tpy-Pt, the highest being for BD-related CLs. These enhancements are slightly higher than those obtained by the conventional Pt-drugs cisplatin, carboplatin and oxaliplatin, apart from BD-related CLs, which are about 3 times higher. Enhancements are related to the strong perturbation of the DNA helix by Tpy-Pt, its high dipole moment and its favorable binding to guanine (G), all of which increase bond-breaking via TA formation. In CRT, Tpy-Pt could considerably enhance crosslinking within genomic DNA and between DNA and other components of the nucleus, causing roadblocks to replication and transcription, particularly within telomeres, where it binds preferentially within G-quadruplexes.
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| GB/T 7714 | Ouyang, Liangde , Lin, Hong , Zhuang, Puxiang et al. DNA radiosensitization by terpyridine-platinum: damage induced by 5 and 10 eV transient anions [J]. | NANOSCALE , 2023 , 15 (7) : 3230-3242 . |
| MLA | Ouyang, Liangde et al. "DNA radiosensitization by terpyridine-platinum: damage induced by 5 and 10 eV transient anions" . | NANOSCALE 15 . 7 (2023) : 3230-3242 . |
| APA | Ouyang, Liangde , Lin, Hong , Zhuang, Puxiang , Shao, Yu , Khosravifarsani, Meysam , Guerin, Brigitte et al. DNA radiosensitization by terpyridine-platinum: damage induced by 5 and 10 eV transient anions . | NANOSCALE , 2023 , 15 (7) , 3230-3242 . |
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Histone proteins protect cellular DNA from radiationdamage. Wefind that arginine, a major component of histone proteins, protectsDNA from lesions induced by low-energy secondary electrons generatedby radiation. Thin films of 7 +/- 2, 12 +/- 4, and 17 +/- 4 nm thicknesses containing arginine-plasmid-DNA complexesin molar ratio of [Arg(2+)]/[PO4 (-)] = 16 are irradiated in vacuum with 5 and 10 eV electrons. Damageyields are measured for base damages, cross-links, single-strand breaks(SSBs), double-strand breaks, and other clustered lesions. Most damageresults from dissociative electron attachment. Absolute cross sections(ACSs) for all damage types are extracted from yields at differentfilm thicknesses. Compared with bare DNA, these ACSs are reduced byfactors of up to 4.4 in Arg-DNA complexes. SSB protection isthe highest. Potentially lethal cluster lesions decrease by factorsof up to 2.2. ACSs are critical input parameters in modeling radiation-induceddamage and assessing protection factors under simulated cellular conditions.
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| GB/T 7714 | Wang, Xuran , Liao, Hong , Liu, Wenhui et al. DNA Protection against Damages Induced by Low-Energy Electrons: Absolute Cross Sections for Arginine-DNA Complexes [J]. | JOURNAL OF PHYSICAL CHEMISTRY LETTERS , 2023 , 14 (24) : 5674-5680 . |
| MLA | Wang, Xuran et al. "DNA Protection against Damages Induced by Low-Energy Electrons: Absolute Cross Sections for Arginine-DNA Complexes" . | JOURNAL OF PHYSICAL CHEMISTRY LETTERS 14 . 24 (2023) : 5674-5680 . |
| APA | Wang, Xuran , Liao, Hong , Liu, Wenhui , Shao, Yu , Zheng, Yi , Sanche, Leon . DNA Protection against Damages Induced by Low-Energy Electrons: Absolute Cross Sections for Arginine-DNA Complexes . | JOURNAL OF PHYSICAL CHEMISTRY LETTERS , 2023 , 14 (24) , 5674-5680 . |
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Constructing heterojunction is an efficient strategy to boost the charge carrier separation rate and promote the catalytic performance for photocatalysts. In this paper, amorphous CoMoS4 was first deposited on the surface of the flower-like microspheres of CdIn2S4 to fabricate CoMoS4/CdIn2S4 composites for accelerating the photocatalytic hydrogen evolution (PHE) rate under simulated sunlight irradiation. The compositions, morphologies, and photoelectrochemical properties of the obtained samples were examined. SEM images show that a great number of CoMoS4 nanoparticles were filled into the gaps of CdIn2S4 microspheres. Optical characterization shows that the combination of CoMoS4 and CdIn2S4 strongly strengthened their light absorption capability. The remarkably promoted PHE rate of the optimum 5%-CCIS catalyst (2196 mmol g-1 h-1) was 8.4 folds larger than that for CdIn2S4. More importantly, the heterostructured 5%-CCIS composite also exhibited good activity stability in the three-cycled experiments. Photoelectrochemical measurements provided the energy band potentials and demonstrated the efficient charge separation efficiency, consistent with the photocatalytic activity of CoMoS4/CdIn2S4 composites for hydrogen production. This study will provide a new strategy to fabricate CoMoS4-based heterostructures for boosting the hydrogen evolution under visible light.(c) 2023 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
Keyword ：
Co-catalyst Co-catalyst Heterojunction Heterojunction Hydrogen evolution Hydrogen evolution Photocatalysis Photocatalysis
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| GB/T 7714 | Rao, Yansen , Sun, Meng , Zhou, Bingzheng et al. Facile deposition of CoMoS4 on flower-like CdIn2S4 microspheres: Enhanced charge separation and efficient photocatalytic hydrogen evolution [J]. | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2023 , 51 : 133-144 . |
| MLA | Rao, Yansen et al. "Facile deposition of CoMoS4 on flower-like CdIn2S4 microspheres: Enhanced charge separation and efficient photocatalytic hydrogen evolution" . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY 51 (2023) : 133-144 . |
| APA | Rao, Yansen , Sun, Meng , Zhou, Bingzheng , Wang, Li , Wang, Zhongpeng , Yan, Tao et al. Facile deposition of CoMoS4 on flower-like CdIn2S4 microspheres: Enhanced charge separation and efficient photocatalytic hydrogen evolution . | INTERNATIONAL JOURNAL OF HYDROGEN ENERGY , 2023 , 51 , 133-144 . |
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Constructing heterojunctions with transition metal sulfides is an excellent strategy to reduce the dependency on noble metals in photocatalytic water splitting. Herein, 0D CoMoS4 nanoparticles were first deposited in-situ on the surface of 3D ZnIn2S4 microflowers for constructing heterostructured CoMoS4-ZnIn2S4 (CMS-ZIS) compos-ites. The CMS-ZIS composites showed strengthened absorption capabilities in the visible light region compared with pure ZnIn2S4. The electron microscopy scanning images indicate that countless CoMoS4 particles were loaded into the gaps on the surface of ZnIn2S4 microflowers, resulting in a close interface contact between the materials. The photocatalytic hydrogen evolution (PHE) rate of the optimized CMS-ZIS-3 product is 6.43 folds that of pure ZnIn2S4, which is approximately 3942.1 mu mol g(-1) h(-1). The enhanced activity should be attributed to the promoted carrier transfer rate and reduced recombination efficiency. We inferred the possible mechanism for photocatalytic hydrogen production over CMS-ZIS-3 based on the band potential and photoelectrochemical testing results. This study provides a feasible strategy for designing efficient and cost-effective 0D/3D heterostructures.
Keyword ：
0D/3d heterostructure 0D/3d heterostructure CoMoS4-ZnIn2S4 CoMoS4-ZnIn2S4 Hydrogen evolution Hydrogen evolution Photocatalysis Photocatalysis Solar light Solar light
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| GB/T 7714 | Zhou, Bingzheng , Sun, Meng , Wang, Li et al. Constructing 0D CoMoS4-3D ZnIn2S4 heterostructure: Strengthened visible light absorption and efficient charge separation for boosting photocatalytic hydrogen evolution [J]. | SOLID STATE SCIENCES , 2023 , 145 . |
| MLA | Zhou, Bingzheng et al. "Constructing 0D CoMoS4-3D ZnIn2S4 heterostructure: Strengthened visible light absorption and efficient charge separation for boosting photocatalytic hydrogen evolution" . | SOLID STATE SCIENCES 145 (2023) . |
| APA | Zhou, Bingzheng , Sun, Meng , Wang, Li , Rao, Yansen , Yan, Tao , Du, Bin et al. Constructing 0D CoMoS4-3D ZnIn2S4 heterostructure: Strengthened visible light absorption and efficient charge separation for boosting photocatalytic hydrogen evolution . | SOLID STATE SCIENCES , 2023 , 145 . |
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