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学者姓名：张焱焱
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Abstract ：
Aqueous zinc-iodine (Zn-I2) batteries have attracted considerable research interest as an alternative energy storage system due to their high specific capacity, intrinsic safety, and low cost. However, the notorious shuttle effect of soluble polyiodides causes severe capacity loss and poor electrochemical reversibility, restricting their practical usage. Herein, this study reports a bifunctional binder (polyacrylonitrile copolymer, as known as LA133) with strong iodine-chemisorption capability for aqueous Zn-I2 batteries to suppress polyiodide shuttling. From both calculation and experimental data, this study reveals that the amide and carboxyl groups in LA133 binder can strongly bond to polyiodides, significantly immobilizing them at cathode side. As a result, fewer byproducts, slower hydrogen evolution, and lesser Zn dendrite in the Zn-I2 battery are observed. Consequently, the battery shows high specific capacity (202.8 mAh g-1) with high iodine utilization efficiency (96.1%), and long cycling lifespan (2700 cycles). At the high mass loading of 7.82 mg cm-2, the battery can still retain 83.3% of its initial capacity after 1000 cycles. The specific capacity based on total cathode slurry mass reaches 71.2 mAh g-1, higher than most of the recent works. The strategy opens a new avenue to address the shuttling challenge of Zn-I2 batteries through bifunctional binder. A new bifunctional LA133 binder with strong iodine-chemisorption capability is reported for high-loading and shuttle-free Zn-I2 batteries. The oxygen-containing groups in LA133 binder can generate strong interactions with I2 and polyiodides, thus significantly enhancing the iodine immobilization performance. This work provides a new strategy to address the shuttling challenge of Zn-I2 batteries from functional binder design. image
Keyword ：
bifunctional binder bifunctional binder chemical confinement chemical confinement shuttle effect shuttle effect zinc-iodine batteries zinc-iodine batteries Zn corrosion Zn corrosion
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| GB/T 7714 | Wang, Kexuan , Li, Heng , Xu, Zhu et al. An Iodine-Chemisorption Binder for High-Loading and Shuttle-Free Zn-Iodine Batteries [J]. | ADVANCED ENERGY MATERIALS , 2024 , 14 (17) . |
| MLA | Wang, Kexuan et al. "An Iodine-Chemisorption Binder for High-Loading and Shuttle-Free Zn-Iodine Batteries" . | ADVANCED ENERGY MATERIALS 14 . 17 (2024) . |
| APA | Wang, Kexuan , Li, Heng , Xu, Zhu , Liu, Yupeng , Ge, Mingzheng , Wang, Huibo et al. An Iodine-Chemisorption Binder for High-Loading and Shuttle-Free Zn-Iodine Batteries . | ADVANCED ENERGY MATERIALS , 2024 , 14 (17) . |
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Sodium-ion batteries (SIBs) with low cost and high safety are considered as an electrochemical energy storage technology suitable for large-scale energy storage. Hard carbon, which is inexpensive and has both high capacity and low sodium storage potential, is regarded as the most promising anode for commercial SIBs. However, the commercialization of hard carbon still faces technical issues of low initial Coulombic efficiency, poor rate performance, and insufficient cycling stability, due to the intrinsically irregular microstructure of hard carbon. To address these challenges, the rational design of the hard carbon microstructure is crucial for achieving high-performance SIBs, via gaining an in-depth understanding of its structure–performance correlations. In this context, our review firstly describes the sodium storage mechanism from the perspective of the hard carbon microstructure's formation. We then summarize the state-of-art development of hard carbon, providing a critical overview of emergence of hard carbon in terms of precursor selection, microstructure design, and electrolyte regulation to optimize strategies for addressing practical problems. Finally, we highlight directions for the future development of hard carbon to achieve the commercialization of high-performance SIBs. We believe this review will serve as basic guidance for the rational design of hard carbon and stimulate more exciting research into other types of energy storage devices. © 2023 The Authors
Keyword ：
Controllable microstructure Controllable microstructure Coulombic efficiency Coulombic efficiency Electrolyte regulation Electrolyte regulation Hard carbon Hard carbon Sodium-ion batteries Sodium-ion batteries Sodium storage mechanism Sodium storage mechanism
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| GB/T 7714 | Wang, F. , Jiang, Z. , Zhang, Y. et al. Revitalizing sodium-ion batteries via controllable microstructures and advanced electrolytes for hard carbon [J]. | eScience , 2024 , 4 (3) . |
| MLA | Wang, F. et al. "Revitalizing sodium-ion batteries via controllable microstructures and advanced electrolytes for hard carbon" . | eScience 4 . 3 (2024) . |
| APA | Wang, F. , Jiang, Z. , Zhang, Y. , Li, J. , Wang, H. , Jiang, Y. et al. Revitalizing sodium-ion batteries via controllable microstructures and advanced electrolytes for hard carbon . | eScience , 2024 , 4 (3) . |
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Aqueous zinc-ion batteries (AZIBs) are promising large-scale energy storage devices due to their costeffectiveness and high safety. However, the rampant dendrite growth and notorious side reactions resulting from the decomposition of active water molecules hinder its practical application. Herein, the zincophilic polyoltype surfactant of alkyl polyglycoside (APG) is introduced to induce the rearrangement of the H-bonds network to diminish the free water activity, facilitating the zinc-ion solvation structure transition from [Zn2+(H2O)6 & sdot;SO42-] (solvent separated ion pair, SSIP) to [Zn2+(H2O)5 & sdot;OSO32-] (contact ion pair, CIP) with less Zn2+-solvated H2O. Meanwhile, the APG molecular preferentially adsorb on the Zn surface to form a dehydrated layer, which can suppress the hydrogen evolution reaction (HER) and hinder the two-dimensional (2D) diffusion of Zn2+ ions. Consequently, the Zn//Zn symmetric cell using our designed electrolyte demonstrates an ultralong cycle life of 5250 h at 1.0 mA cm-2/1.0 mAh cm-2. Furthermore, the as-prepared Zn//Na2V6O16 & sdot;3H2O full cell also delivers a high-capacity retention rate of 80.8% even after 1000 cycles at 2.0 A g-1, superior to that of the full cell using pure ZnSO4 electrolyte. This study offers an effective strategy to modulate the cation solvation structure by rearranging the H-bonds network for a highly reversible Zn anode.
Keyword ：
Alkyl polyglycoside Alkyl polyglycoside H -bonds network H -bonds network Hydrogen evolution reaction Hydrogen evolution reaction Solvation structure Solvation structure Zn anodes Zn anodes
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| GB/T 7714 | Wang, Huicai , Zhu, Mengyu , Wang, Huibo et al. Rearrangement of H-bonds network of solvation structure via a zincophilic polyol-type surfactant to stabilize zinc anode in aqueous zinc-ion batteries [J]. | ENERGY STORAGE MATERIALS , 2024 , 67 . |
| MLA | Wang, Huicai et al. "Rearrangement of H-bonds network of solvation structure via a zincophilic polyol-type surfactant to stabilize zinc anode in aqueous zinc-ion batteries" . | ENERGY STORAGE MATERIALS 67 (2024) . |
| APA | Wang, Huicai , Zhu, Mengyu , Wang, Huibo , Li, Chunxin , Ren, Zejia , Zhang, Yanlei et al. Rearrangement of H-bonds network of solvation structure via a zincophilic polyol-type surfactant to stabilize zinc anode in aqueous zinc-ion batteries . | ENERGY STORAGE MATERIALS , 2024 , 67 . |
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Ionic liquid electrolytes (ILEs) are promising to develop high-safety and high-energy-density lithium-metal batteries (LMBs). Unfortunately, ILEs normally face the challenge of sluggish Li+ transport due to increased ions' clustering caused by Coulombic interactions. Here a type of anion-reinforced solvating ILEs (ASILEs) is discovered, which reduce ions' clustering by enhancing the anion-cation coordination and promoting more anions to enter the internal solvation sheath of Li+ to address this concern. The designed ASILEs, incorporating chlorinated hydrocarbons and two anions, bis(fluorosulfonyl) imide (FSI-) and bis(trifluoromethanesulfonyl) imide (TFSI-), aim to enhance Li+ transport ability, stabilize the interface of the high-nickel cathode material (LiNi0.8Co0.1Mn0.1O2, NCM811), and retain fire-retardant properties. With these ASILEs, the Li/NCM811 cell exhibits high initial specific capacity (203 mAh g-1 at 0.1 C), outstanding capacity retention (81.6% over 500 cycles at 1.0 C), and excellent average Coulombic efficiency (99.9% over 500 cycles at 1.0 C). Furthermore, an Ah-level Li/NCM811 pouch cell achieves a notable energy density of 386 Wh kg-1, indicating the practical feasibility of this electrolyte. This research offers a practical solution and fundamental guidance for the rational design of advanced ILEs, enabling the development of high-safety and high-energy-density LMBs. An anion-reinforced solvating ionic liquid electrolyte is developed to enhance the anion-cation coordination and promote more anions to enter the internal solvation sheath of Li+. This new type of ionic liquid electrolyte improves Li+ transport ability and stabilizes the interface between the electrolyte and high-nickel cathode, rendering the practical application toward high-safety and high-energy-density lithium-metal batteries. image
Keyword ：
anion reinforced anion reinforced high energy density high energy density ionic liquids ionic liquids lithium-metal batteries lithium-metal batteries
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| GB/T 7714 | Zou, Wenhong , Zhang, Jun , Liu, Mengying et al. Anion-Reinforced Solvating Ionic Liquid Electrolytes Enabling Stable High-Nickel Cathode in Lithium-Metal Batteries [J]. | ADVANCED MATERIALS , 2024 , 36 (23) . |
| MLA | Zou, Wenhong et al. "Anion-Reinforced Solvating Ionic Liquid Electrolytes Enabling Stable High-Nickel Cathode in Lithium-Metal Batteries" . | ADVANCED MATERIALS 36 . 23 (2024) . |
| APA | Zou, Wenhong , Zhang, Jun , Liu, Mengying , Li, Jidao , Ren, Zejia , Zhao, Wenlong et al. Anion-Reinforced Solvating Ionic Liquid Electrolytes Enabling Stable High-Nickel Cathode in Lithium-Metal Batteries . | ADVANCED MATERIALS , 2024 , 36 (23) . |
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Layered structure Na2Ti3O7 with a suitable sodiation plateau potential (similar to 0.3 V vs Na+/Na) is a promising anode for highly safe sodium-ion batteries (SIBs). However, the practical use of Na2Ti3O7 is hindered by the unstable interface that forms between the anode and electrolyte leading to issues such as low initial coulombic efficiency (ICE) and cycling instability. Herein, we introduce tetraethyl orthosilicate (TEOS) as an electrolyte additive that can spontaneously and effectively react with the main component of the detrimental surface corrosion layer (sodium hydroxide, etc.) to form a protective film on the Na2Ti3O7 anode. The Na2Ti3O7 anode exhibits an enhanced capacity from 134.8 to 167.1 mAh g(-1) at 0.1 A g(-1), along with an increase in capacity retention from 56.1 to 83.9% after 250 cycles at 0.2 A g(-1). This work provides a straightforward protection strategy to address the unstable interface issues, rendering sodium titanate as a promising anode material to achieve practical application in the future.
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| GB/T 7714 | Jiang, Zhenming , Ke, Haifeng , Zhang, Yanlei et al. Building a Stable Plateau-Type Na2Ti3O7 Anode Interface toward Advanced Sodium-Ion Batteries [J]. | ENERGY & FUELS , 2024 , 38 (3) : 2472-2479 . |
| MLA | Jiang, Zhenming et al. "Building a Stable Plateau-Type Na2Ti3O7 Anode Interface toward Advanced Sodium-Ion Batteries" . | ENERGY & FUELS 38 . 3 (2024) : 2472-2479 . |
| APA | Jiang, Zhenming , Ke, Haifeng , Zhang, Yanlei , Li, Linwei , Wang, Feng , Li, Jidao et al. Building a Stable Plateau-Type Na2Ti3O7 Anode Interface toward Advanced Sodium-Ion Batteries . | ENERGY & FUELS , 2024 , 38 (3) , 2472-2479 . |
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Rechargeable metal batteries have received widespread attention due to their high energy density by using pure metal as the anode. However, there are still many fundamental problems that need to be solved before approaching practical applications. The critical ones are low charge/discharge current due to slow ion transport, short cycle lifetime due to poor anode/cathode stability, and unsatisfied battery safety. To tackle these problems, various strategies have been suggested. Among them, electrolyte additive is one of the most widely used strategies. Most of the additives currently studied are soluble, but their reliability is questionable, and they can easily affect the electrochemical process, causing unwanted battery performance decline. On the contrary, insoluble additives with excellent chemical stability, high mechanical strength, and dimensional tunability have attracted considerable research exploration recently. However, there is no timely review on insoluble additives in metal batteries yet. This review summarizes various functions of insoluble additives: ion transport modulation, metal anode protection, cathode amelioration, as well as battery safety enhancement. Future research directions and challenges for insoluble solid additives are also proposed. It is expected this review will stimulate inspiration and arouse extensive studies on further improvement in the overall performance of metal batteries. Highly stable insoluble additives in metal batteries provide a feasible approach to counteract additive depletion as well as its accompanying side reactions. This review summarizes recent advances in insoluble additives for metal batteries with a unique focus on the following aspects: modulation of ion transport, protection of metal anodes, amelioration of cathodes, and enhancement of battery safety. image
Keyword ：
battery safety battery safety electrode stability electrode stability insoluble additives insoluble additives ion transport ion transport metal batteries metal batteries
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| GB/T 7714 | Xu, Zhu , Wang, Kexuan , Li, Heng et al. Critical Effects of Insoluble Additives in Liquid Electrolytes for Metal Batteries [J]. | SMALL , 2024 , 20 (37) . |
| MLA | Xu, Zhu et al. "Critical Effects of Insoluble Additives in Liquid Electrolytes for Metal Batteries" . | SMALL 20 . 37 (2024) . |
| APA | Xu, Zhu , Wang, Kexuan , Li, Heng , Wang, Huibo , Ge, Mingzheng , Zhang, Yanyan et al. Critical Effects of Insoluble Additives in Liquid Electrolytes for Metal Batteries . | SMALL , 2024 , 20 (37) . |
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The plateau-type sodium titanate with suitable sodiation potential is a promising anode candidate for high safe and high energy density of sodium-ion batteries (SIBs). However, the poor initial Coulombic efficiency (ICE) and cyclic instability of sodium titanate are attributed to the unstable interfacial structure along with the decomposition of electrolytes, resulting in the continuous formation of solid electrolyte interface (SEI) film. To address this issue, a chemical grafting method is developed to fabricate a highly stable interface layer of inert Al2O3 on the sodium titanate anode, rendering the high ICE and excellent cycling stability. Based on theoretical calculations, NaPF6 are more likely adsorption on the Al2O3 surface and produce sodium fluoride. The formation of a thin and dense SEI film with rich sodium fluoride achieves the low interfacial resistances and charge-transfer resistances. Benefitting from our design, the obtained sodium titanate exhibits a high ICE from 67.7 % to 79.4 % and an enhanced reversible capacity from 151 mAh g-1 to 181 mAh g-1 at 20 mA g-1, along with an increase in capacity retention from 56.5 % to 80.6 % after 500 cycles. This work heralds a promising paradigm for rational regulation of interfacial stability to achieve high-performance anodes for SIBs. A chemical grafting method is developed to fabricate a highly stable interface layer of inert Al2O3 on the sodium titanate anode, rendering the high initial Coulombic efficiency (ICE) and excellent cycling stability. This is due to the formation of a thin and dense solid-electrolyte interface (SEI) film with rich sodium fluoride, leading to the lower interfacial resistances and charge-transfer resistances.+ image
Keyword ：
heterostructure-layer heterostructure-layer initial Coulombic efficiency initial Coulombic efficiency Plateau-type sodium titanate Plateau-type sodium titanate sodium-ion batteries sodium-ion batteries
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| GB/T 7714 | Zhang, Yanlei , Li, Linwei , Wang, Feng et al. Achieving High Initial Coulombic Efficiency and Capacity in a Surface Chemical Grafting Layer of Plateau-type Sodium Titanate [J]. | CHEMSUSCHEM , 2024 , 17 (11) . |
| MLA | Zhang, Yanlei et al. "Achieving High Initial Coulombic Efficiency and Capacity in a Surface Chemical Grafting Layer of Plateau-type Sodium Titanate" . | CHEMSUSCHEM 17 . 11 (2024) . |
| APA | Zhang, Yanlei , Li, Linwei , Wang, Feng , Wang, Huicai , Jiang, Zhenming , Lin, Zhimin et al. Achieving High Initial Coulombic Efficiency and Capacity in a Surface Chemical Grafting Layer of Plateau-type Sodium Titanate . | CHEMSUSCHEM , 2024 , 17 (11) . |
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Hard carbon with abundant resources, low-cost, and high specific capacity, is a promising anode material for large-scale sodium-ion batteries. However, the poor rate performance of hard carbon suffers from serious challenges due to sluggish ion transport dynamic behavior, especially at low potential, in high power density of sodium-ion batteries. To address this issue, we introduce an ionic-conductive sodium-titanate into hard carbon to boost its sodium-ion transport kinetics via constructing a dual ionic-electronic conducting network in hard carbon anode. Benefiting from our design, the optimized hard carbon-sodium titanate electrode achieves high specific capacity of 137 mAh g(-1) at a high current density of 10 A g(-1), compared to that of hard carbon of 25 mAh g(-1) at 10 A g(-1). Remarkably, it also exhibits an excellent capacity retention of 71.4% at the current density of 2.0 A g(-1) after 800 cycles. This work presents a practical strategy for high-rate hard carbon design and provides valuable insights into the construction of high-rate anode for advanced sodium-ion batteries.
Keyword ：
Hard carbon Hard carbon High rate High rate Ionic conductivity Ionic conductivity Sodium ion batteries Sodium ion batteries Sodium titanate Sodium titanate
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| GB/T 7714 | Li, Fan , Gong, Hao , Zhang, Yanlei et al. Ionic-conductive sodium titanate to boost sodium-ion transport kinetics of hard carbon anode in sodium-ion batteries [J]. | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 981 . |
| MLA | Li, Fan et al. "Ionic-conductive sodium titanate to boost sodium-ion transport kinetics of hard carbon anode in sodium-ion batteries" . | JOURNAL OF ALLOYS AND COMPOUNDS 981 (2024) . |
| APA | Li, Fan , Gong, Hao , Zhang, Yanlei , Liu, Xinyu , Jiang, Zhenming , Chen, Lian et al. Ionic-conductive sodium titanate to boost sodium-ion transport kinetics of hard carbon anode in sodium-ion batteries . | JOURNAL OF ALLOYS AND COMPOUNDS , 2024 , 981 . |
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Separators or electrolyte membranes are recognized as the key components to guarantee ion transport in rechargeable batteries. However, the ever-growing applications of the battery systems for diverse working environments bring new challenges, which require advanced battery membranes with high thermal stability, excellent mechanical strength, high voltage tolerance, etc. Therefore, it is highly desirable to design novel methods/concepts to solve the current challenges for battery membranes through understanding the mechanism of novel phenomena and electrochemical reactions in battery systems working under unconventional conditions. Recently, the new emerging Janus separators or electrolyte membranes with two or more distinct chemical/physical properties arising from their asymmetric structure and composition, are promising to address the above challenges via rational design of their targeted functionalities. To this end, in this review, we first briefly cover the current challenges of the traditional battery membrane for battery devices working in unconventional conditions. Then, the state-of-art developments of the rational design of Janus membranes to overcome the above challenges for diverse battery applications are summarized. Finally, we outline these latest developments, challenges, and future potential directions of the Janus membrane. Our review is aimed to provide basic guidance for developing functional separators or electrolyte membranes for advanced batteries.
Keyword ：
batteries batteries Janus membranes Janus membranes separators separators solid-state electrolytes solid-state electrolytes
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| GB/T 7714 | Chan, Dan , Liu, Yunfei , Fan, You et al. Functional Janus Membranes: Promising Platform for Advanced Lithium Batteries and Beyond [J]. | ENERGY & ENVIRONMENTAL MATERIALS , 2023 , 6 (5) . |
| MLA | Chan, Dan et al. "Functional Janus Membranes: Promising Platform for Advanced Lithium Batteries and Beyond" . | ENERGY & ENVIRONMENTAL MATERIALS 6 . 5 (2023) . |
| APA | Chan, Dan , Liu, Yunfei , Fan, You , Wang, Huibo , Chen, Shi , Hao, Tianwei et al. Functional Janus Membranes: Promising Platform for Advanced Lithium Batteries and Beyond . | ENERGY & ENVIRONMENTAL MATERIALS , 2023 , 6 (5) . |
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Prussian blue analogues (PBAs) with the 3D open framework are regarded as promising cathode candidates for aqueous Zinc ion batteries (ZIBs). Among various PBAs, nickel hexacyanoferrate (NiHCF) has attracted considerable attention because of its high operating voltage and economic merit. However, the cyclability of NiHCF is unsatisfactory due to poor structural stability during Zn 2 + ions insertion/deinsertion. Moreover, the ion storage mechanism of NiHCF in aqueous electrolytes has not been fully revealed yet. Herein, high-crystallinity NiHCF (HC-NiHCF) microcubes with improved structural stability and larger crystal plane spacing are synthesized. For the first time, highly reversible Zn 2 + ions and Na + ions coinsertion/extraction are achieved for the HC-NiHCF microcubes in mixed aqueous electrolyte, as evidenced by various observations including two separated discharge plateaus and sequential changes of Na 1s and Zn 2p signals in ex-situ X-ray photoelectron spectroscopy (XPS). As a result, a high specific capacity of 73.9 mAh g -1 is obtained for the HC-NiHCF microcubes at 0.1 A g -1 , combined with enhanced cycle stability (75% vs. 16.4%) over 10 0 0 cycles at 2 A g -1 . The reversible Zn 2 + ions and Na + ions coinsertion in HC-NiHCF microcubes reveals a new ion storage mechanism of Ni-based PBAs in aqueous electrolytes.& COPY; 2023 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology.
Keyword ：
Aqueous zinc -ion batteries Aqueous zinc -ion batteries Dual ions storage Dual ions storage High crystallinity High crystallinity Ion storage mechanism Ion storage mechanism Prussian blue analogues Prussian blue analogues
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| GB/T 7714 | Wang, Kexuan , Xu, Zhu , Li, Heng et al. Realizing the highly reversible Zn2+and Na+ dual ions storage in high-crystallinity nickel hexacyanoferrate microcubes for aqueous zinc-ion batteries [J]. | JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY , 2023 , 164 : 102-110 . |
| MLA | Wang, Kexuan et al. "Realizing the highly reversible Zn2+and Na+ dual ions storage in high-crystallinity nickel hexacyanoferrate microcubes for aqueous zinc-ion batteries" . | JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 164 (2023) : 102-110 . |
| APA | Wang, Kexuan , Xu, Zhu , Li, Heng , Wang, Huibo , Ge, Mingzheng , Liu, Jilei et al. Realizing the highly reversible Zn2+and Na+ dual ions storage in high-crystallinity nickel hexacyanoferrate microcubes for aqueous zinc-ion batteries . | JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY , 2023 , 164 , 102-110 . |
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