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学者姓名：陈孔发
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Abstract ：
La0.9Sr0.1Ga0.8Mg0.2O3 (LSGM) with an extraordinary oxygen-ion conductivity has been extensively studied as an electrolyte material for intermediate temperature solid oxide cells (SOCs). However, the conventional hightemperature sintering process of electrodes results in detrimental reaction between LSGM and Ni-based hydrogen electrode and microstructural coarsening of the electrode. Herein, a buffer-layer-free LSGM electrolyte-supported single cell with a nanostructured Ni-Gd0.1Ce0.9O1.95 (GDC) electrode is developed using a sintering-free fabrication approach. The cell exhibits a peak power density of 1.23 W cm-2 at 800 degrees C and an electrolysis current density of 1.85 A cm-2 at 1.5 V with excellent operating stability. The good performance and durability is owing to the synergistic effects of the elimination of elemental interdiffusion at the electrode/ electrolyte interface, polarization induced in situ formation of hetero-interfaces between Ni-GDC and LSGM, and remarkable structural stability of Ni-GDC. This study provides an innovative means for the development of efficient and durable buffer-layer-free LSGM-supported SOCs.
Keyword ：
Buffer -layer -free Buffer -layer -free Elemental interdiffusion Elemental interdiffusion Interface formation Interface formation Nanostructure Nanostructure Sintering -free Sintering -free
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| GB/T 7714 | Qian, Jiaqi , Lin, Changgen , Chen, Zhiyi et al. High-performance, stable buffer-layer-free La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported solid oxide cell with a nanostructured nickel-based hydrogen electrode [J]. | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2024 , 346 . |
| MLA | Qian, Jiaqi et al. "High-performance, stable buffer-layer-free La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported solid oxide cell with a nanostructured nickel-based hydrogen electrode" . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY 346 (2024) . |
| APA | Qian, Jiaqi , Lin, Changgen , Chen, Zhiyi , Huang, Jiongyuan , Ai, Na , Jiang, San Ping et al. High-performance, stable buffer-layer-free La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte-supported solid oxide cell with a nanostructured nickel-based hydrogen electrode . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2024 , 346 . |
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Abstract ：
Perovskite oxide La0.9Sr0.1Ga0.8Mg0.2O3 (LSGM) is an intermedium-temperature solid oxide cell electrolyte material with extraordinary oxygen-ion conductivity. However, the manufacturing procedures of LSGM discs are complex involving multiple steps of powder preparation, forming, and sintering at high temperatures. Herein, thin LSGM electrolyte discs are prepared by coupling of tape casting and in situ solid-state reaction using oxides/carbonates as the feedstock. A pure-phase LSGM electrolyte disc with uniform elemental distribution is obtained by sintering at 1450 degrees C, and it possesses an ionic conductivity of 0.105 S cm(1) at 800 degrees C, a thermal expansion coefficient of 12.2 x 10(6) K-1, and a bending strength of 156 MPa A 170 mu m thick LSGM electrolyte-supported single cell delivers a peak power density of 0.96 W cm(2) at 800 degrees C and an electrolysis current density of 1.82 A cm(2) at 1.5 V with no noticeable degradation for 200 h. The findings of this research provide a cost-effective approach for manufacturing the LSGM electrolytes of efficient and durable solid oxide cells.
Keyword ：
Electrolyte-support Electrolyte-support LSGM LSGM Solid oxide cells Solid oxide cells Solid-state reaction Solid-state reaction Tape casting Tape casting
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| GB/T 7714 | Lin, Changgen , Zhang, Yongmei , Qian, Jiaqi et al. Coupling of tape casting and in situ solid-state reaction for manufacturing La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte of efficient solid oxide cells [J]. | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY , 2024 , 44 (6) : 3818-3823 . |
| MLA | Lin, Changgen et al. "Coupling of tape casting and in situ solid-state reaction for manufacturing La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte of efficient solid oxide cells" . | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY 44 . 6 (2024) : 3818-3823 . |
| APA | Lin, Changgen , Zhang, Yongmei , Qian, Jiaqi , Chen, Zhiyi , Huang, Jiongyuan , Ai, Na et al. Coupling of tape casting and in situ solid-state reaction for manufacturing La0.9Sr0.1Ga0.8Mg0.2O3 electrolyte of efficient solid oxide cells . | JOURNAL OF THE EUROPEAN CERAMIC SOCIETY , 2024 , 44 (6) , 3818-3823 . |
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The photon-assisted electron transport properties through a parallel-coupled tri-quantum-dot system are studied using the time-dependent non-equilibrium Green's function theory. When a time-dependent external field irradiates a parallel-coupled three-quantum-dot system, the interaction between photons and electrons provides more novel transport characteristics. The average current can be switched between zero and non-zero by controlling the level of the time-dependent external field, indicating that an optically-controlled quantum switch can be realized. The time-dependent external field makes it more advantageous for the system to be designed as a magnetic-controlled quantum switch. If the magnetic flux and Rashba spin orbit coupling interaction are simultaneously considered, the average current exhibits a spin polarization phenomenon. For the spin down current, the bound states are formed as the magnetic flux takes an appropriate value, which greatly enhances the spin polarization. These research results are expected to contribute to the design of future quantum function devices.
Keyword ：
Average current Average current Electron transport Electron transport Green 's function Green 's function Parallel -coupled tri-quantum-dot Parallel -coupled tri-quantum-dot
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| GB/T 7714 | He, Zelong , Li, Qiang , Aslam, Muhammad et al. Electron transport properties of a parallel-coupled tri-quantum-dot system irradiated by a time-dependent external field [J]. | PHYSICA B-CONDENSED MATTER , 2024 , 679 . |
| MLA | He, Zelong et al. "Electron transport properties of a parallel-coupled tri-quantum-dot system irradiated by a time-dependent external field" . | PHYSICA B-CONDENSED MATTER 679 (2024) . |
| APA | He, Zelong , Li, Qiang , Aslam, Muhammad , Ran, Du , Chen, Kongfa , Zhao, Xinwei . Electron transport properties of a parallel-coupled tri-quantum-dot system irradiated by a time-dependent external field . | PHYSICA B-CONDENSED MATTER , 2024 , 679 . |
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A challenge hindering the development of durable solid oxide fuel cells (SOFCs) is the significant performance degradation of cathodes owing to poisoning by volatile Cr originating from the FeCr alloy interconnect. Herein, a heterogeneous catalyst coating, composed of Ba1-xCe0.8Gd0.2O3-delta and BaCO3, remarkably improves the oxygen adsorption, dissociation capability, and Cr resistance of a La0.6Sr0.4Co0.2Fe0.8O3-delta (LSCF) cathode is demonstrated. The coherent heterointerface interactions formed between the catalyst coating and LSCF result in varied levels of surface strain and electrostatic interactions, significantly suppressing Sr surface segregation on LSCF. A single cell with the catalyst coating-decorated LSCF (CC-LSCF) achieves a peak power density of 1.73 W cm-2 at 750 degrees C, with no noticeable performance degradation for 100 h. The CC-LSCF cathode also exhibits outstanding durability under accelerated Cr poisoning conditions, compared with the tremendous degradation rate of 0.42% h-1 for the bare LSCF cathode. The enhanced Cr resistance is attributed to synergy induced by the stabilization of the lattice Sr cations by heterointerface interactions and the remarkable structural stability of the catalyst coating under Cr poisoning conditions. The novel heterointerface engineering strategy in this study provides insight into the design and development of active and Cr-tolerant cathodes. A heterogeneous catalyst coating composed of Ba1-xCe0.8Gd0.2O3-delta and BaCO3 remarkably improves the oxygen adsorption, dissociation capability, and Cr tolerance of La0.6Sr0.4Co0.2Fe0.8O3-delta cathode. The enhanced Cr tolerance is attributed to synergy induced by the stabilization of the lattice Sr cations by heterointerface interactions and the remarkable structural stability of the catalyst coating under Cr poisoning conditions. image
Keyword ：
chromium tolerance chromium tolerance heterointerfaces heterointerfaces solid oxide fuel cells solid oxide fuel cells Sr surface segregation Sr surface segregation strain strain
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| GB/T 7714 | Huang, Jiongyuan , Liang, Fujun , Zhao, Sunce et al. Heterogeneous Catalyst Coating for Boosting the Activity and Chromium Tolerance of Cathodes for Solid Oxide Fuel Cells [J]. | ADVANCED FUNCTIONAL MATERIALS , 2024 , 34 (26) . |
| MLA | Huang, Jiongyuan et al. "Heterogeneous Catalyst Coating for Boosting the Activity and Chromium Tolerance of Cathodes for Solid Oxide Fuel Cells" . | ADVANCED FUNCTIONAL MATERIALS 34 . 26 (2024) . |
| APA | Huang, Jiongyuan , Liang, Fujun , Zhao, Sunce , Zhao, Ling , Ai, Na , Jiang, San Ping et al. Heterogeneous Catalyst Coating for Boosting the Activity and Chromium Tolerance of Cathodes for Solid Oxide Fuel Cells . | ADVANCED FUNCTIONAL MATERIALS , 2024 , 34 (26) . |
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Transition metal sulfides are used in the field of supercapacitors due to their remarkable electrical conductivity and superior energy density. However, few research has been conducted on how the sulfidation process affects the structure and electrochemical properties of electrodes. The nanoneedle array Zn-Mn-Co sulfide (ZMC-S/NF) electrode is prepared by directly growing on nickel foam (NF) via a two-step hydrothermal technique. During the first step, the Zn-Mn-Co carbonate hydroxide nanoneedle skeleton can be obtained. During the second step, the nanoneedle skeletons are etched, and rough nanoneedle arrays are created by the introduced sulfur ions,i.e., the sulfidation process. The ZMC-S/NF electrode exhibits a specific capacity of 1401.0 C g−1 at 2 A g−1. It still has excellent rate performance with a specific capacity of 1015.3 C g−1 at 20 A g−1. Moreover, it exhibits excellent cycling stability with 81.9% capacity retention after 10,000 cycles. ZMC-S/NF as the cathode and activated carbon (AC) as the anode are assembled to be a hybrid supercapacitor (HSC), which has an energy density of 43.4 Wh kg−1 at a power density of 700.4 W kg−1. The effect of adding Zn and Mn to the Co3S4 on energy band structure and density of states during the sulfidation process is calculated by the DFT. The HSC devices constructed by two series-connected ZMC-S/NF//AC can light a star made by ten 1.8 V-red Light Emitting Diodes (LEDs) for 10 minutes. © 2024
Keyword ：
Activated carbon Activated carbon Cobalt compounds Cobalt compounds Density functional theory Density functional theory Electrochemical electrodes Electrochemical electrodes Manganese compounds Manganese compounds Musculoskeletal system Musculoskeletal system Nanoneedles Nanoneedles Supercapacitor Supercapacitor Ternary alloys Ternary alloys Transition metals Transition metals Zinc sulfide Zinc sulfide
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| GB/T 7714 | Wang, Hongtao , Zhao, Kun , Shao, Yanqun et al. ZnMnCo-S nanoneedle arrays as battery-type eletrodes for high-performance hybrid supercapacitors [J]. | Materials Today Communications , 2024 , 39 . |
| MLA | Wang, Hongtao et al. "ZnMnCo-S nanoneedle arrays as battery-type eletrodes for high-performance hybrid supercapacitors" . | Materials Today Communications 39 (2024) . |
| APA | Wang, Hongtao , Zhao, Kun , Shao, Yanqun , Xiao, Shengtao , Yang, Zhiguang , Chen, Zhe et al. ZnMnCo-S nanoneedle arrays as battery-type eletrodes for high-performance hybrid supercapacitors . | Materials Today Communications , 2024 , 39 . |
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Phosphates are a kind of promising electrode materials because they can provide numerous cavities and several reaction sites to be favored for storing anions and cations. However, the widespread application of phosphates are limited by their intrinsically low electronic conductivity. RuO 2 /hydrated RuO 2 exhibits high conductivity and excellent electrochemical properties. Reducing its dosage and increasing its specific surface area are the research concerns. Combining less RuO 2 to Nickel phosphate (NiP) is expected to improve the electrochemical performance. RuO 2 -modified NiP (NiP-RuO 2 ) electrode material is synthesized by a one-step hydrothermal reaction and its structural morphology and capacitive properties are investigated. The results indicate that NiPRuO 2 electrode consists of hydrated RuO 2 and Ni 11 (HPO 3 ) 8 (OH) 6 , and exhibits excellent battery -type electrochemical supercapacitor performance with a specific capacity of 878.06 C/g at 1 A/g. According to density functional theory (DFT) analysis, Ru-doped Ni 11 (HPO 3 ) 8 (OH) 6 has a narrower forbidden band width and higher conductivity than Ni 11 (HPO 3 ) 8 (OH) 6 . Furthermore, the asymmetric supercapacitor (ASC) assembled by NiPRuO 2 /NF and activated carbon (AC) electrode achieves a high energy density (43.58 Wh/kg) at a power density of 923.47 W/kg. When two ASC devices are connected in series, ten light -emitting diodes (LEDs) can be illuminated for ten minutes.
Keyword ：
Asymmetric supercapacitors Asymmetric supercapacitors DFT DFT HydratedRuO2 HydratedRuO2 Ni11(HPO3)8(OH)6 Ni11(HPO3)8(OH)6
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| GB/T 7714 | Zhao, Kun , Wang, Hongtao , Shao, Yanqun et al. A battery-type cathode with RuO2 modified Ni11 (HPO3 )8(OH)6 for asymmetric supercapacitors [J]. | ELECTROCHIMICA ACTA , 2024 , 488 . |
| MLA | Zhao, Kun et al. "A battery-type cathode with RuO2 modified Ni11 (HPO3 )8(OH)6 for asymmetric supercapacitors" . | ELECTROCHIMICA ACTA 488 (2024) . |
| APA | Zhao, Kun , Wang, Hongtao , Shao, Yanqun , Yang, Zhiguang , Chen, Zhe , Chen, Kongfa et al. A battery-type cathode with RuO2 modified Ni11 (HPO3 )8(OH)6 for asymmetric supercapacitors . | ELECTROCHIMICA ACTA , 2024 , 488 . |
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Modulation of the surface chemistry of air electrodes makes it possible to significantly improve the electrocatalytic performance of solid oxide cells (SOCs). Here, the surface chemistry of BaGd0.8La0.2Co2O6-delta (BGLC) double perovskite is modulated by treatment in an acidic citric acid solution. The treatment leads to corrosion on the surface of BGLC particles, and the effect is dependent on the acidity of the solution. As the acidity of solution is low, Ba cations are selectively dissolved out of the BGLC surface, while as the acidity increases, the corrosion becomes more homogeneous. The Ba surface deficiency remarkably increases the concentration of surface oxygen vacancies and electrocatalytic activity of BGLC. To avoid the loss of Ba-deficient surface during the conventional high temperature sintering process, a sintering-free fabrication route is utilized to directly assemble the Ba-deficient BGLC powder into an air electrode. A single cell with the surface Ba-deficient BGLC electrode shows a peak power density of 1.04 W cm(-2) at 750 degrees C and an electrolysis current density of 1.48 A cm(-2) at 1.3 V, much greater than 0.64 W cm(-2) and 1.02 A cm(-2) of the cell with the pristine BGLC, respectively. This work provides a simple and effective surface chemistry modulation strategy for the development of an efficient air electrode for SOCs.
Keyword ：
A-sitedeficiency A-sitedeficiency double perovskite double perovskite selectivecorrosion selectivecorrosion solid oxide cells solid oxide cells surface chemistry modulation surface chemistry modulation
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| GB/T 7714 | Chen, Kongfa , Weng, Qiaohang , Yue, Zhongwei et al. Surface Chemistry Modulation of BaGd0.8La0.2Co2O6-δ As Active Air Electrode for Solid Oxide Cells [J]. | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (24) : 31181-31190 . |
| MLA | Chen, Kongfa et al. "Surface Chemistry Modulation of BaGd0.8La0.2Co2O6-δ As Active Air Electrode for Solid Oxide Cells" . | ACS APPLIED MATERIALS & INTERFACES 16 . 24 (2024) : 31181-31190 . |
| APA | Chen, Kongfa , Weng, Qiaohang , Yue, Zhongwei , Huang, Jiongyuan , Qian, Jiaqi , Chen, Zhiyi et al. Surface Chemistry Modulation of BaGd0.8La0.2Co2O6-δ As Active Air Electrode for Solid Oxide Cells . | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (24) , 31181-31190 . |
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In the development of nanoscale oxygen electrodes of high-temperature solid oxide cells (SOCs), the interface formed between the nanoelectrode particles and the electrolyte or electrolyte scaffolds is the most critical. In this work, a new synthesis technique for the fabrication of nanostructured electrodes via in situ electrochemical polarization treatment is reported. The lanthanum strontium cobalt ferrite (LSCF) precursor solution is infiltrated into a gadolinia-doped ceria (GDC) scaffold presintered on a yttria-stabilized zirconia (YSZ) electrolyte, followed by in situ polarization current treatment at SOC operation temperatures. Electrode ohmic and polarization resistances decrease with an increase in the polarization current treatment. Detailed microstructure analysis indicates the formation of a convex-shaped interface between the LSCF nanoparticles (NPs) and the GDC scaffold, very different from the flat contact between LSCF and GDC observed after heating at 800 degrees C with no polarization current treatment. The embedded LSCF NPs on the GDC scaffold contribute to the superior stability under both fuel cell and electrolysis operation conditions at 750 degrees C and a high peak power density of 1.58 W cm(-2) at 750 degrees C. This work highlights a novel and facile route to in situ construct a stable and high-performing nanostructured electrode for SOCs.
Keyword ：
convex-shapedinterface convex-shapedinterface embedded LSCF nanoparticles embedded LSCF nanoparticles in situ polarization treatment in situ polarization treatment nanostructured LSCF/GDC compositeelectrodes nanostructured LSCF/GDC compositeelectrodes solid oxide cells solid oxide cells stable electrodenanostructure stable electrodenanostructure
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| GB/T 7714 | Sun, Yi , He, Shuai , Li, Zhishan et al. Development of Nanostructured Lanthanum Strontium Cobalt Ferrite/Gadolinian-Doped Ceria Composite Electrodes of Solid Oxide Cells Formed by In Situ Polarization [J]. | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (17) : 21818-21827 . |
| MLA | Sun, Yi et al. "Development of Nanostructured Lanthanum Strontium Cobalt Ferrite/Gadolinian-Doped Ceria Composite Electrodes of Solid Oxide Cells Formed by In Situ Polarization" . | ACS APPLIED MATERIALS & INTERFACES 16 . 17 (2024) : 21818-21827 . |
| APA | Sun, Yi , He, Shuai , Li, Zhishan , Mclaughlin, Abbie C. , Chen, Kongfa , Shao, Zongping et al. Development of Nanostructured Lanthanum Strontium Cobalt Ferrite/Gadolinian-Doped Ceria Composite Electrodes of Solid Oxide Cells Formed by In Situ Polarization . | ACS APPLIED MATERIALS & INTERFACES , 2024 , 16 (17) , 21818-21827 . |
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Protonic ceramic fuel cells (PCFCs) are characterized by a low activation energy for proton conduction and a high fuel utilization efficiency at low -to -intermediate temperatures. However, the sluggish oxygen reduction reaction kinetics on the cathodes drastically limit the power output performance of PCFCs. Herein, multiphase Gd 0.1 Ce 0.9 O 1.95 - BaGd 0.8 La 0.2 Co 2 O 6- delta (GDC-BGLC) nanocomposite cathodes are prepared by coupling selfassembly and sintering -free electrode construction methods. The nanocomposite cathode comprises mixed H + /e - conducting BGLC and O 2- conducting GDC and BaCoO 3 nanoparticles, and these phases are homogeneously mixed with coherent heterointerfaces. The nanocomposite cathode exhibits a significant increase in surface oxygen vacancies and three-phase boundaries, enhanced catalytic activity, and reduced activation energy for the oxygen reduction and water formation reactions. The results imply that the oxygen reduction and water formation reactions on the multiphase GDC-BGLC nanocomposite electrodes are most likely the dissociation, reduction and diffusion of oxygen species, which in turn is affected by the water vapor formed. An anodesupported single cell with the GDC-BGLC cathode exhibits a peak power density of 810 mW cm -2 at 700 degrees C with excellent operating stability at 650 degrees C for 110 h. This study provides a new strategy for the preparation of a high-performance and durable nanocomposite cathode for PCFCs.
Keyword ：
Heterointerface Heterointerface Nanocomposite cathode Nanocomposite cathode Protonic ceramic fuel cells (PCFCs) Protonic ceramic fuel cells (PCFCs) Reaction mechanism Reaction mechanism Self -assembly Self -assembly
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| GB/T 7714 | Liao, Dan , Jia, Lichao , Xu, Jianghui et al. Self-assembled Gd 0.1 Ce 0.9 O 1.95-BaGd 0.8 La 0.2 Co 2 O 6-δ nanocomposite cathode for efficient protonic ceramic fuel cells [J]. | CERAMICS INTERNATIONAL , 2024 , 50 (13) : 22574-22582 . |
| MLA | Liao, Dan et al. "Self-assembled Gd 0.1 Ce 0.9 O 1.95-BaGd 0.8 La 0.2 Co 2 O 6-δ nanocomposite cathode for efficient protonic ceramic fuel cells" . | CERAMICS INTERNATIONAL 50 . 13 (2024) : 22574-22582 . |
| APA | Liao, Dan , Jia, Lichao , Xu, Jianghui , Chen, Zhiyi , Huang, Jiongyuan , Ai, Na et al. Self-assembled Gd 0.1 Ce 0.9 O 1.95-BaGd 0.8 La 0.2 Co 2 O 6-δ nanocomposite cathode for efficient protonic ceramic fuel cells . | CERAMICS INTERNATIONAL , 2024 , 50 (13) , 22574-22582 . |
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Metal-supported solid oxide fuel cells (SOFCs) have the merits of quick startup, low cost, and excellent robustness, however, there is a lack of understanding on the effect of thermally driven elemental diffusion. Herein, we investigate the role of elemental diffusion on the evolution of morphologies and electrochemical performance of Ni-Fe alloy supported Ni-yttria stabilized zirconia (YSZ) anode and YSZ electrolyte film. The results show that during the co-sintering process at high temperatures, there is significant diffusion of Fe element from the Ni-Fe oxide substrate to the anode and electrolyte. The elemental diffusion leads to the formation of a NiO core/NiFe2O4 shell structure in the anode and dissolution of Fe cations in the YSZ lattices of anode and electrolyte, but also significantly enhances the sinterability of both layers. The negative effect of Fe diffusion induced microstructure coarsening is largely compensated by the formation of an electrocatalytically active Ni-Fe alloy in the reduced anode. The present work provides insights into the design and development of effi-cient metal-supported SOFCs by taking advantage of elemental diffusion.
Keyword ：
Elemental diffusion Elemental diffusion Metallic substrate Metallic substrate Microstructure coarsening Microstructure coarsening Solid oxide fuel cells Solid oxide fuel cells
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| GB/T 7714 | Lin, Xu , Xu, Jianghui , Chen, Zhiyi et al. Thermally driven long-distance elemental diffusion enhances the sinterability of anode and electrolyte of metal-supported solid oxide fuel cells [J]. | JOURNAL OF POWER SOURCES , 2023 , 555 . |
| MLA | Lin, Xu et al. "Thermally driven long-distance elemental diffusion enhances the sinterability of anode and electrolyte of metal-supported solid oxide fuel cells" . | JOURNAL OF POWER SOURCES 555 (2023) . |
| APA | Lin, Xu , Xu, Jianghui , Chen, Zhiyi , Ai, Na , Lue, Zhe , Jiang, San Ping et al. Thermally driven long-distance elemental diffusion enhances the sinterability of anode and electrolyte of metal-supported solid oxide fuel cells . | JOURNAL OF POWER SOURCES , 2023 , 555 . |
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