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学者姓名：徐胜
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Abstract ：
Inorganic metal halide perovskite quantum dots (PQDs) have recently emerged as promising candidates for color conversion materials in Micro-LED displays, due to their outstanding color purity, high absorption coefficient, tunable emission wavelength. However the inferior stability and undesirable photoluminescence quantum yield (PLQY) restrict their particle applications. Herein, CsPbX3/PMMA (X = Br, I) composites with improved stability and optical performance were successfully prepared by a general and mild in-situ polymerization strategy. The ester carbonyl (C--O) group in MMA formed complexes with Pb2+, leading to the in-situ thermal polymerization of polymethyl methacrylate (PMMA) under the action of the initiator. The multifunctional PMMA can efficiently passivate halogen vacancies while acting as a barrier against the degradation caused by heat, water, and oxygen. As a result, the PLQYs and stability of PMMA-coated CsPbX3 PQDs have been significantly improved. When implementing CsPbX3/PMMA/PDMS composites as color conversion layers in Micro-LEDs, they achieve an impressive color gamut of 127.23% with excellent stability. We believe our work will stimulate the exploration of perovskite/polymer composites for industrial Micro-LED applications.
Keyword ：
dots dots Inorganic metal halide perovskite quantum Inorganic metal halide perovskite quantum In-situ polymerization In-situ polymerization Micro-LED Micro-LED Photoluminescence Photoluminescence PMMA PMMA
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| GB/T 7714 | Cai, Junhu , Zhang, Xiang , Chen, Yu et al. Highly luminescent CsPbX3/PMMA (X=Br, I) composites with improved stability for full-color Micro-LED displays [J]. | JOURNAL OF LUMINESCENCE , 2024 , 269 . |
| MLA | Cai, Junhu et al. "Highly luminescent CsPbX3/PMMA (X=Br, I) composites with improved stability for full-color Micro-LED displays" . | JOURNAL OF LUMINESCENCE 269 (2024) . |
| APA | Cai, Junhu , Zhang, Xiang , Chen, Yu , Lai, Wenzong , Zhang, Wenyan , Lin, Zexi et al. Highly luminescent CsPbX3/PMMA (X=Br, I) composites with improved stability for full-color Micro-LED displays . | JOURNAL OF LUMINESCENCE , 2024 , 269 . |
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When quantum dot diffusion plates (QDDPs) are used as phosphor conversion materials for high-power lighting, transparent ceramics (TCs) can be used to prevent thermal damage of QDDPs. The spectral, suitable for diverse lighting environments, can be precisely calibrated by modifying their ratio. The temperature dependent photoluminescence spectra, fluorescence lifetime, Huang Rhys factor and activation energy of TCs were studied in detail. It was evident from the results that the intensity of TCs remained above 89% even at 423 K, while fluorescence lifetime remained stable, nearly 64 ns. Huang-Rhys factor and activation energy were consistently measured at 1.81 and 0.13 eV, respectively. The extraordinary luminescent stability of TCs revealed their integral role in providing reliable protection for QDDPs. The spectra of LEDs/LDs were successfully predicted using Monte Carlo ray tracing method. The service condition under high-energy laser was studied using finite element method. White light with Commission Internationale de l'Eclairage (CIE) of (0.38, 0.39) and (0.31, 0.34) and luminous efficiency of 58 and 150 lm/W were prepared by combining QDDPs/TCs with LEDs/LDs, and the Color Rendering Index (CRI) reached a remarkable 88.4 and 78.8. A detailed exploration of the proficient thermal management was accomplished using finite element analysis, with the simulated outcomes matching closely with the experimental results. © 2024 Elsevier Ltd and Techna Group S.r.l.
Keyword ：
Activation energy Activation energy Finite element method Finite element method Fluorescence Fluorescence High energy lasers High energy lasers Light emitting diodes Light emitting diodes Monte Carlo methods Monte Carlo methods Nanocrystals Nanocrystals Photoluminescence Photoluminescence Quantum dot lasers Quantum dot lasers Ray tracing Ray tracing Semiconductor quantum dots Semiconductor quantum dots Yttrium aluminum garnet Yttrium aluminum garnet
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| GB/T 7714 | Du, Aochen , Xie, Hongxing , Zheng, Xingke et al. Exploring potential of quantum dots for high power solid-state lighting protected by transparent ceramics [J]. | Ceramics International , 2024 , 50 (11) : 20275-20284 . |
| MLA | Du, Aochen et al. "Exploring potential of quantum dots for high power solid-state lighting protected by transparent ceramics" . | Ceramics International 50 . 11 (2024) : 20275-20284 . |
| APA | Du, Aochen , Xie, Hongxing , Zheng, Xingke , Gao, Jiaqi , Lin, Xinyu , Ye, Yun et al. Exploring potential of quantum dots for high power solid-state lighting protected by transparent ceramics . | Ceramics International , 2024 , 50 (11) , 20275-20284 . |
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Quantum dots（QDs）are widely used in luminescence and display，solar cells，photocatalysis and other fields due to their excellent photovoltaic properties，and its discovery and synthesis won the 2023 Nobel Prize in Chemistry. Micro-LED full-color display technology using quantum dot color conversion does not require mass transfer technology and is expected to achieve large-scale mass production. However，there are still limitations to the performance and lifespan of quantum dots under intense Micro-LED light excitation. Based on，this paper studies the Micro-LED color conversion technology and its characteristics based on quantum dot@ordered mesoporous（QDs@SBA-15）composite materials. The unique pore structure of the ordered mesoporous materials not only can effectively improve the Micro-LED color conversion and light extraction efficiency，but also the dense ordered mesoporous material guarantees the stability of the quantum dots to a certain extent. Firstly，we established a Micro-LED simulation model through the Finite-difference time-domain（FDTD）method to investigate the effects of the particle size of the quantum dots and the pore size of the ordered mesoporous materials on the light extraction efficiency. Based on the guidance of simulation results，QDs@SBA-15 composites were further prepared by physical blending method，characterized by transmission spectroscopy，fluorescence excitation spectroscopy and UV-Vis absorption spectroscopy，and the concentration ratios were determined. Finally，we combined this composite material with polydimethylsiloxane （PDMS）to solidify it into a film and studied its photoluminescence performance. The experimental results showed that the matching degree of the quantum dot particle size and the pore diameter of the mesoporous material，as well as the concentration ratio of quantum dots and ordered mesoporous materials，is crucial to the luminous efficiency of QDs@SBA-15 composite materials and the color conversion performance of Micro-LED. Through the optimization，the resulting composites can obtain excellent luminescence performance and good environmental stability，compared with the pure quantum dots color conversion layer，the light extraction efficiency of the composite material has been improved by 81. 73%，and the environmental stability of the composite material has been improved by 14. 33%. The color gamut of tri-color devices obtained with Micro-LED as the blue light source reached 104. 52% NTSC. This research provides theoretical guidance for quantum dot color conversion Micro-LED display technology，and opens up a new path to realize the full-color Micro-LED. © 2024 Chines Academy of Sciences. All rights reserved.
Keyword ：
Absorption spectroscopy Absorption spectroscopy Color Color Composite materials Composite materials Extraction Extraction Finite difference time domain method Finite difference time domain method Light emitting diodes Light emitting diodes Luminescence Luminescence Mass transfer Mass transfer Nanocrystals Nanocrystals Particle size Particle size Pore size Pore size Quantum efficiency Quantum efficiency Semiconductor quantum dots Semiconductor quantum dots Silicones Silicones Solar power generation Solar power generation
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| GB/T 7714 | Chen, Xiaogang , Zhao, Mengyun , Cai, Junhu et al. Color Conversion Characteristics of Micro-LED Based on Quantum Dot@Ordered Mesoporous Composite Materials [J]. | Chinese Journal of Luminescence , 2024 , 45 (1) . |
| MLA | Chen, Xiaogang et al. "Color Conversion Characteristics of Micro-LED Based on Quantum Dot@Ordered Mesoporous Composite Materials" . | Chinese Journal of Luminescence 45 . 1 (2024) . |
| APA | Chen, Xiaogang , Zhao, Mengyun , Cai, Junhu , Li, Gongming , Zha, Nan , Ye, Yun et al. Color Conversion Characteristics of Micro-LED Based on Quantum Dot@Ordered Mesoporous Composite Materials . | Chinese Journal of Luminescence , 2024 , 45 (1) . |
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光波导组合器在增强现实显示的出瞳扩展和外观薄化方面颇具优势。出瞳扩展技术是通过在耦出区域诱导多次衍射，将光线引导至人眼。然而，这种多次衍射可能导致出瞳亮度在沿光路径的空间分布上逐渐减弱，从而造成亮度不均。特别是当使用液晶制备而成的偏振体全息光栅作为耦合元件时，由于光栅仅对一种圆偏振光敏感，与之正交的圆偏振光会被直接透射，导致波导系统的能量利用率并不高。针对这一挑战，本文提出了一种实现左旋和右旋圆偏振光复用的偏振体全息光栅光波导AR显示光学系统，同时实现了大出瞳尺寸和良好入眼均匀性。在理论设计和仿真方面，首先通过k空间理论设计了大视场角下的光栅结构，再以微型发光二极管（Micro-LED，μLED）作为微显示屏，设计了一套与之匹配的投影镜头，并对整个波导系统进行了成像仿真。在实验部分，制备了中心波长为532 nm、出瞳尺寸为45 mm×25 mm的偏振体全息光栅波导。实验结果显示，该波导系统在基板折射率为1.51下的对角线视场角达到了预期的32.86°。相比于仅响应单一圆偏振光的方案，采用九点法测得的均匀性提升了48.8%，整体均匀性提升了34.1%，波导组合器的光学效率也实现了1.2倍的提升。本文工作为偏振体全息光栅波导的设计提供了宝贵的指导和参考。
Keyword ：
增强现实 增强现实 微型发光二极管显示 微型发光二极管显示 波导 波导 液晶偏振体光栅 液晶偏振体光栅 衍射光栅 衍射光栅
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| GB/T 7714 | 林子健 , 姚立胜 , 金华健 et al. 偏振光复用的液晶体光栅波导AR近眼显示系统 [J]. | 液晶与显示 , 2024 , 39 (05) : 646-655 . |
| MLA | 林子健 et al. "偏振光复用的液晶体光栅波导AR近眼显示系统" . | 液晶与显示 39 . 05 (2024) : 646-655 . |
| APA | 林子健 , 姚立胜 , 金华健 , 邱健滨 , 叶芸 , 徐胜 et al. 偏振光复用的液晶体光栅波导AR近眼显示系统 . | 液晶与显示 , 2024 , 39 (05) , 646-655 . |
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A carbon layer usually covers the outside of SnS/MoS2 nanosheets produced by a traditional C-layer cladding process, resulting in a material with a lower specific surface area and fewer active sites. Therefore, it is difficult for these as-obtained SnS and MoS2 materials to be directly employed as electrode materials. There is a great need to develop a new C-layer coating process that can effectively coat active materials and simultaneously increase the specific surface area. In this study, novel SnS@C/MoS2 nanotubes were designed and synthesized by a self-sacrificing template method (SSTM). Specifically, MoO3 nanoribbons were first coated with Sn to produce Sn-MOF, and SnS@C/MoS2 nanotubes with a particular nanosheet architecture preserved were achieved via an elegant SSTM vulcanization strategy. This SSTM preparation method not only retains the nanosheet microstructure of the surface but also leaves a thin layer of amorphous carbon on the surface, which greatly improves the conductivity and effectively improves the cycling stability. In addition to above-mentioned advantages, there is a synergistic effect between the various components of the SnS@C/MoS2 nanotubes, which has a positive effect on the electrochemical performance. When used as the anode of a lithium-ion battery (LIB), the SnS@C/MoS2 composite can maintain a specific discharge capacity of 970.9 mAh g(-1) after 500 cycles at a current density of 1 A g(-1), and a specific discharge capacity of 778.1 mAh g(-1) even after 1000 cycles at a current density of 2 A g(-1). This method provides a reference for the synthesis of other nanostructured materials.
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| GB/T 7714 | Ye, Songwei , Yang, Zunxian , Ye, Yuliang et al. Forming SnS@C/MoS2 nanotubes with high specific surface area via self-sacrificing template method as superior performance anode for lithium-ion batteries [J]. | CRYSTENGCOMM , 2024 , 26 (12) : 1779-1788 . |
| MLA | Ye, Songwei et al. "Forming SnS@C/MoS2 nanotubes with high specific surface area via self-sacrificing template method as superior performance anode for lithium-ion batteries" . | CRYSTENGCOMM 26 . 12 (2024) : 1779-1788 . |
| APA | Ye, Songwei , Yang, Zunxian , Ye, Yuliang , Cheng, Zhiming , Hong, Hongyi , Zeng, Zhiwei et al. Forming SnS@C/MoS2 nanotubes with high specific surface area via self-sacrificing template method as superior performance anode for lithium-ion batteries . | CRYSTENGCOMM , 2024 , 26 (12) , 1779-1788 . |
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Augmented reality (AR) near-eye displays seamlessly integrate virtual information with real world, in which the optical waveguide is the key component functioned as a coupler. Due to strong chromatic aberration, independent waveguides are always indispensable to separate the three primary colors that inevitably brings larger and thicker appearance. To address this, this paper proposes a new chromatic-aberration-free single-layer waveguide for AR displays by integrating a double-layer grating metasurface (MS) and the covered cylindrical MSs. The double-layer grating MS breaks through the limitations on a narrow wavelength band, enabling high diffraction efficiency for incident light deflection across the entire visible spectrum. Further, the cylindrical MSs provide accurate control over incident angles, not only overcoming the challenge of total reflection but also effectively eliminating chromatic aberration. Design results show that the proposed structure achieves an impressive diffraction efficiency of over 80 % for blue and green light and over 90 % for red light with an outstanding diffraction angular difference lower than 2.5 deg. Real-time ray tracing simulation demonstrates the capability of the designed AR engine to achieve high-resolution full-color imaging. The compound MSs enable precise light and color control for a single-layer waveguide coupler with exceptional diffraction efficiency and minimal chromatic aberration, which show great potential for cutting-edge AR applications.
Keyword ：
Augmented reality Augmented reality Chromatic-aberration-free Chromatic-aberration-free Compound metasurfaces Compound metasurfaces Full-color imaging Full-color imaging High diffraction efficiency High diffraction efficiency Near-eye displays Near-eye displays
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| GB/T 7714 | Sun, Zhilin , Yan, Shuzhan , Chen, Kangkang et al. Single-layer waveguide with compound metasurfaces for highly efficient and chromatic-aberration-free augmented reality near-eye displays [J]. | OPTICS AND LASERS IN ENGINEERING , 2024 , 178 . |
| MLA | Sun, Zhilin et al. "Single-layer waveguide with compound metasurfaces for highly efficient and chromatic-aberration-free augmented reality near-eye displays" . | OPTICS AND LASERS IN ENGINEERING 178 (2024) . |
| APA | Sun, Zhilin , Yan, Shuzhan , Chen, Kangkang , Lin, Zijian , Ye, Yun , Xu, Sheng et al. Single-layer waveguide with compound metasurfaces for highly efficient and chromatic-aberration-free augmented reality near-eye displays . | OPTICS AND LASERS IN ENGINEERING , 2024 , 178 . |
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Alloyed quantum dots (QDs) show great potential for photoluminescence (PL) applications. However, the oxidative decay of QDs during photoexcitation has been a major hurdle to the application of QDs. Blocking water-oxygen erosion by coating oxides on the surface of QDs is a common technique. Even though, this approach often leads to alterations in the optical properties of QDs and reduced compatibility with polymers. In this paper, hindered phenol was utilized to treat QDs to form QD/Hindered phenol complexes. Using the reduction of phenolic hydroxyl group in the hindered phenol, the hindered phenol was used as an exhausted substance to protect QDs from oxidation. After 450 h of aging, the obtained QD/Hindered phenol complex kept the photoluminescence quantum yield (PLQY) at 48 %. The luminance of the QD diffusion plate prepared by the QD/Hindered phenol complexes maintained above 98 % of the initial value after aging 1032 h. The introduction of phosphite ester further improved the photostability of QD/Hindered phenol complex under blue-light excitation. This technique promotes the application of QDs in polymers and offers a new reference for improving the stability of QDs under photoexcitation.
Keyword ：
Hindered phenol Hindered phenol Optical stability Optical stability Photo -oxidation Photo -oxidation QD diffusion plate QD diffusion plate Quantum dots Quantum dots
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| GB/T 7714 | Zeng, Zhenyu , Xie, Hongxing , Ye, Yun et al. Enhancement of photo-oxidation resistance of quantum dots by hindered phenol and its application in diffusion plate [J]. | OPTICAL MATERIALS , 2024 , 148 . |
| MLA | Zeng, Zhenyu et al. "Enhancement of photo-oxidation resistance of quantum dots by hindered phenol and its application in diffusion plate" . | OPTICAL MATERIALS 148 (2024) . |
| APA | Zeng, Zhenyu , Xie, Hongxing , Ye, Yun , Zheng, Xingke , Lin, Qizhong , Chen, Enguo et al. Enhancement of photo-oxidation resistance of quantum dots by hindered phenol and its application in diffusion plate . | OPTICAL MATERIALS , 2024 , 148 . |
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量子点(Quantum dots)由于具有优异的光电特性,广泛应用于发光与显示、太阳能电池、光催化等领域,它的发现和合成获得了2023年诺贝尔化学奖.采用量子点色转换的Micro-LED全彩化显示技术无需巨量转移,有望实现大规模量产,然而,量子点在高强度Micro-LED出光激发下的性能和寿命仍存在局限.基于此,本文研究了基于量子点@有序介孔(QDs@SBA-15)复合材料的Micro-LED色转换技术及其特性,有序介孔分子筛载体独特的孔道结构不仅能够有效提升Micro-LED色转换和光提取效率,且致密的有序介孔材料也一定程度上保障了量子点的稳定性.首先,通过时域有限差分方法(FDTD)建立了Micro-LED仿真模型,探究量子点粒径和有序介孔材料的孔径对光提取效率的影响;基于仿真结果指导,进一步采用物理共混法制备了QDs@SBA-15复合材料,通过透射光谱、荧光激发光谱、紫外-可见光吸收谱等手段对其进行表征并确定浓度配比;最后,将该复合材料与聚二甲基硅氧烷(PDMS)混合固化成膜,并研究了其光致发光性能.实验结果发现,量子点粒径和介孔材料孔径的匹配度以及量子点和有序介孔材料的比例浓度是影响QDs@SBA-15复合材料发光效率及Micro-LED色转换性能的关键因素;通过优化,所得复合材料可获得优异的发光性能以及良好的环境稳定性,相比于纯量子点色转换层,复合材料的光提取效率提升了81.73％,复合材料的环境稳定性提升了14.33％,以Micro-LED作为蓝光光源组成的三基色发光器件工作色域达到了104.52％NTSC.本研究为量子点色转换Micro-LED显示技术提供了理论指导,为实现Micro-LED全彩化开辟了新路径.
Keyword ：
Micro-LED Micro-LED 有序介孔材料 有序介孔材料 色转换 色转换 量子点 量子点
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| GB/T 7714 | 陈晓钢 , 赵梦云 , 蔡俊虎 et al. 基于量子点@有序介孔复合材料的Micro-LED色转换特性 [J]. | 发光学报 , 2024 , 45 (1) : 59-68 . |
| MLA | 陈晓钢 et al. "基于量子点@有序介孔复合材料的Micro-LED色转换特性" . | 发光学报 45 . 1 (2024) : 59-68 . |
| APA | 陈晓钢 , 赵梦云 , 蔡俊虎 , 李恭明 , 查楠 , 叶芸 et al. 基于量子点@有序介孔复合材料的Micro-LED色转换特性 . | 发光学报 , 2024 , 45 (1) , 59-68 . |
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Over the past few years, light-emitting diodes (LEDs) have emerged as an efficient replacement for standard incandescent and fluorescent lamps, due to their superior efficiency, energy conservation, service longevity, reliability, and affordability. However, identifying a red emitter for white LEDs has presented significant challenges. This study seeks to synthesize and analyze a novel red emitter, investigating its potential use in white LEDs and indoor plant growth lighting. The Sr2Lu(Nb,Mn)O6 is manufactured employing the traditional high-temperature solid-phase method. The internal and external quantum efficiencies (IQE and EQE) of double perovskites reached 32.39% and 21.67%. The g value calculates to 2.146, which corroborates that the magnetic dipolar transitions of Mn4+ ions inhabit symmetric octahedral sites. First-principles investigations are utilized to unveil local electronic structures. Emission spectra reveal a substantial broad red emission peak at 688 nm. The Tanabe-Sugano diagram is applied to understand the luminescence mechanism. Additionally, the evaluation of parameters such as the internal UV emission ratio, crystal field strength, and Racah parameters is conducted. The luminescent intensity of the Sr2Lu(Nb,Mn)O6 can still be maintained at 60% upon reaching a temperature of 423 K. The findings suggest that Sr2Lu(Nb,Mn)O6 offers a novel alternative for white LEDs and indoor plant growth lighting. This paper unveils the local electronic structure of manganese-doped Sr2LuNbO6 double perovskite red emitter, and elaborates on its crystal structures, luminescence properties, crystal field properties, thermal stability, and energy transfer mechanisms. Based upon first principles calculations, reveals the superior photoelectric performance of it, positioning it as a potential solution for the red-deficiency in white LED and indoor lighting technologies. image
Keyword ：
double perovskite double perovskite first-principles first-principles solid-state lighting solid-state lighting thermometry thermometry white LEDs white LEDs
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| GB/T 7714 | Zheng, Xingke , Du, Aochen , Ye, Yun et al. Unveiling Local Electronic Structures of Manganese-Doped Double Perovskites Red Emitters [J]. | LASER & PHOTONICS REVIEWS , 2024 , 18 (5) . |
| MLA | Zheng, Xingke et al. "Unveiling Local Electronic Structures of Manganese-Doped Double Perovskites Red Emitters" . | LASER & PHOTONICS REVIEWS 18 . 5 (2024) . |
| APA | Zheng, Xingke , Du, Aochen , Ye, Yun , Chen, Enguo , Xu, Sheng , Guo, Tailiang . Unveiling Local Electronic Structures of Manganese-Doped Double Perovskites Red Emitters . | LASER & PHOTONICS REVIEWS , 2024 , 18 (5) . |
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The potential of organic-inorganic hybrid perovskites, owing to their distinct photoelectric attributes and boosted photoluminescence stability, has garnered substantial attention. Despite comprehensive examinations of the synthesis and optical characteristics of FAPbBr(3) crystals, the understanding of their microstructure's implication on photoelectric applications, their electronic configuration, and electron-phonon interplay remains vague. In this study, we detailed the electronic configuration, phonon dispersion, and vibrational properties using density functional theory. We further calculated the formation enthalpy stability diagram. Characterization and calculation of the crystalline structure were accomplished via Rietveld refinement. Phonon dispersion curves, as well as total and partial phonon densities of states, were also calculated. The theoretical results align well with experimental Fourier infrared and Raman spectra. Beyond elementary characterization, we explored the photoelectric qualities of FAPbBr(3) crystals, thereby reaffirming the outstanding photoelectric attributes and extensive application potential. A non-contact fixed-point lighting device was designed based on the principle of electromagnetic induction coils, which proved the uniformity of crystal luminescence. According to the first principle, FAPbBr(3) possesses a Poisson ratio of 0.32, indicative of high flexibility, emphasizing their superb photoelectric characteristics and vast application scope.
Keyword ：
Contactless Contactless Crystal Crystal First-principle First-principle Perovskites Perovskites Photoelectric Photoelectric
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| GB/T 7714 | Du, Aochen , Zheng, Xingke , Li, Genzhuang et al. Uncovering the structural and photoelectric properties of perovskite crystals by joint multifaceted characterization and theoretical analysis [J]. | JOURNAL OF MATERIALS RESEARCH AND TECHNOLOGY-JMR&T , 2024 , 28 : 3988-4000 . |
| MLA | Du, Aochen et al. "Uncovering the structural and photoelectric properties of perovskite crystals by joint multifaceted characterization and theoretical analysis" . | JOURNAL OF MATERIALS RESEARCH AND TECHNOLOGY-JMR&T 28 (2024) : 3988-4000 . |
| APA | Du, Aochen , Zheng, Xingke , Li, Genzhuang , Ye, Yun , Chen, Enguo , Xu, Sheng et al. Uncovering the structural and photoelectric properties of perovskite crystals by joint multifaceted characterization and theoretical analysis . | JOURNAL OF MATERIALS RESEARCH AND TECHNOLOGY-JMR&T , 2024 , 28 , 3988-4000 . |
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