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学者姓名：李浩宏
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Abstract ：
Purpose: To investigate the inhibition of Streptococcus mutans (S.mutans) and its biofilm by AgBr-nanoparticles (NP) @CTMAB (cetyltrimethyl-ammonium bromide) and evaluate the changes in Polymethyl methacrylate (PMMA)'s surface roughness (Ra), microhardness, and flexural strength during prolonged immersion in AgBr-NP@CTMAB for application in the denture cleaning industry. Patients and Methods: The antibacterial activity of AgBr-NP@CTMAB against S.mutans was measured colony formation assay, OD600 and laser confocal microscopy. Changes in the specimens' values for surface roughness, microhardness, and flexural strength (MPa) were measured after immersion solutions for 180 or 360 days. Results: The AgBr-NP@CTMAB solution exhibited a robust antibacterial effect on planktonic S. mutans, with a minimum bactericidal concentration of 5 mu g/mL. The 10 mu g/mL AgBr-NP@CTMAB solution efficiently inhibited S. mutans biofilm formation. (2) No significant difference in surface roughness after immersion in AgBr-NP@CTMAB (10 mu g/mL and 20 mu g/mL) comparing with distilled water (P > 0.05) and Polident had significantly higher than distilled water (P < 0.05). There was a significant decrease in the surface hardness of the PMMA specimens that were immersed in the Polident compared with those in distilled water (P < 0.05). While, no significant differences in surface hardness after immersion in the AgBr-NP@CTMAB (P > 0.05). The result of flexural strength suggested that there was no statistically significant difference (P < 0.05) between AgBr-NP@CTMAB as well as Polident and water. Conclusion: AgBrNP@CTMAB can efficiently inhibit the growth of plankton S.mutans and biofilm formation, without affecting the flexural strength, microhardness, or surface roughness of PMMA. Therefore, AgBrNP@CTMAB holds promise as a new denture cleaning agent.
Keyword ：
AgBr-NP@CTMAB AgBr-NP@CTMAB biofilm biofilm denture cleanser denture cleanser polymethyl methacrylate polymethyl methacrylate S.mutans S.mutans
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| GB/T 7714 | Huang, Jing-Jing , Jia, Lin , Zhang, Qiao-Jun et al. Anti-Microbial Effect of AgBr-NP@CTMAB on Streptococcus Mutans and Assessment of Surface Roughness Hardness and Flexural Strength of PMMA [J]. | INTERNATIONAL JOURNAL OF NANOMEDICINE , 2024 , 19 : 1273-1285 . |
| MLA | Huang, Jing-Jing et al. "Anti-Microbial Effect of AgBr-NP@CTMAB on Streptococcus Mutans and Assessment of Surface Roughness Hardness and Flexural Strength of PMMA" . | INTERNATIONAL JOURNAL OF NANOMEDICINE 19 (2024) : 1273-1285 . |
| APA | Huang, Jing-Jing , Jia, Lin , Zhang, Qiao-Jun , Li, Hao-Hong , Zheng, Da-Li , Zheng, Ming . Anti-Microbial Effect of AgBr-NP@CTMAB on Streptococcus Mutans and Assessment of Surface Roughness Hardness and Flexural Strength of PMMA . | INTERNATIONAL JOURNAL OF NANOMEDICINE , 2024 , 19 , 1273-1285 . |
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The development of green memorizers with distinct mechanism is significant. In this work, renewable polyphenol ellagic acid (EA) and environmentally friendly calcium were used to construct a unique 3D interpenetrated bio-metal-organic framework (BioMOF), i.e. {[Ca2(EA)3(4H2O)]2H2O}n. Its high chemical stability stems from the twofold interpenetrated (6,3) bi-layers and versatile strong pi-pi stacking interactions. The memorizer FTO/{[Ca2(EA)3(4H2O)]2H2O}n/Ag exhibits good bipolar resistive switching performance with an ON/OFF ratio of 5.40 x 103 and a tolerant temperature of 300 degrees C. In particular, the local conjugated EA ligand and strong pi-pi stacking interactions in the interpenetrated 3D network are responsible for a carrier trapping/de-trapping process, rendering the excellent binary resistive switching performance. This work demonstrates a new way for the construction of green electrons by adopting renewable natural products as organic linkers. Natural product ellagic acid was used to construct a stable 3D BioMOF with twofold interpenetrated (6,3) bi-layers, which was fabricated as a biomemorizer with an ON/OFF ratio of 5.40 x 103 bearing a high working temperature of 300 degrees C.
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| GB/T 7714 | Liu, Ting-Bo , Deng, Jing-Wen , Li, Yi et al. Stable calcium ellagate metal-organic frameworks as high-performance green memorizers bearing high working temperatures [J]. | INORGANIC CHEMISTRY FRONTIERS , 2024 , 11 (10) : 3056-3062 . |
| MLA | Liu, Ting-Bo et al. "Stable calcium ellagate metal-organic frameworks as high-performance green memorizers bearing high working temperatures" . | INORGANIC CHEMISTRY FRONTIERS 11 . 10 (2024) : 3056-3062 . |
| APA | Liu, Ting-Bo , Deng, Jing-Wen , Li, Yi , Fu, Hai-Ying , Shi, Liang-Wen , Lin, Shi-Ying et al. Stable calcium ellagate metal-organic frameworks as high-performance green memorizers bearing high working temperatures . | INORGANIC CHEMISTRY FRONTIERS , 2024 , 11 (10) , 3056-3062 . |
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The low efficiency of growing single-walled carbon nanotubes (SWCNT) poses a barrier to their application in high-performance electronic devices. However, it is difficult to control the uniform growth of SWCNT in a floating catalytic reactor due to the complex parameter control. Therefore, it is essential to enhance the growth of SWCNT in the floating catalyst chemical vapor deposition (FCCVD) process. In the present work, the influence of the reactive flow field on the growth of SWCNT, which is often neglected, is revealed. To address this issue, this work combines experiments and simulations to obtain the characteristics of the field distribution within the reactor and the trend of the products. The results of the flow field analysis indicate that thermal buoyancy is the cause of SWCNT growth limitation in FCCVD. By weakening the thermal buoyancy, a homogeneous reaction field is obtained; vortices in the flow field are reduced or even disappear; the temperature field is more homogeneous, and, importantly, the crystallinity of SWCNT is enhanced (IG/ID up to 20-fold). In addition, the decomposition process of the carbon source is also enhanced, thus suppressing the generation of by-products. Based on the results of the small tube experiments, both the increase in temperature and the decrease in residence time increased the IG/ID. Furthermore, the distributions of the maximum and minimum diameters in SWCNT imply variations in the growth modes of SWCNT at different temperatures. © 2024 Elsevier B.V.
Keyword ：
Buoyancy Buoyancy Catalysts Catalysts Chemical vapor deposition Chemical vapor deposition Crystallinity Crystallinity Flow fields Flow fields Residence time distribution Residence time distribution Single-walled carbon nanotubes (SWCN) Single-walled carbon nanotubes (SWCN)
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| GB/T 7714 | Yu, Guo , Han, Peilin , Yi, Hongmei et al. Study of field distribution characteristics in CVD reactors and enhanced growth of SWNCT [J]. | Diamond and Related Materials , 2024 , 145 . |
| MLA | Yu, Guo et al. "Study of field distribution characteristics in CVD reactors and enhanced growth of SWNCT" . | Diamond and Related Materials 145 (2024) . |
| APA | Yu, Guo , Han, Peilin , Yi, Hongmei , Zhao, Jiaxiang , Hou, Songjia , Yan, Zuoyi et al. Study of field distribution characteristics in CVD reactors and enhanced growth of SWNCT . | Diamond and Related Materials , 2024 , 145 . |
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Dehydroxylation of biomass-based platform molecules is critical for obtaining building blocks for use in the chemical industry. Acid catalytic dehydration has provided a feasible route. However, simultaneously pursuing high product-selective and ultra-stable catalysts for the dehydroxylation of polyols remains an open challenge. In this study, a strategy for in-situ Bronsted acid sites (BAS) with chemo-adsorption selectivity is proposed. The construction of defect sites B[3] and P[4] species has been proved to be a prerequisite for the dynamic acid site formation at hydrothermal conditions. The BPO4 catalyst with in-situ BAS can achieve the high selectivity of acrolein (similar to 80%) and robust stability of catalyst (over 425 h) using glycerol dehydration as a model reaction. In addition, in-situ BAS is highly selective for secondary hydroxyl groups and has been extended to other substrate applications. This catalytic strategy provides a green, efficient, and economical approach for converting biomassderived polyols to high-value-added chemicals.
Keyword ：
Acrolein Acrolein Biomass Biomass Dehydration Dehydration Glycerol Glycerol In -situ Br onsted acid In -situ Br onsted acid
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| GB/T 7714 | Su, Chenxin , Zhou, Shouquan , Wu, Shaoyun et al. Highly efficient dehydration of polyols: In-situ Brempty setnsted acid from boron phosphate catalyst [J]. | CHEMICAL ENGINEERING JOURNAL , 2024 , 483 . |
| MLA | Su, Chenxin et al. "Highly efficient dehydration of polyols: In-situ Brempty setnsted acid from boron phosphate catalyst" . | CHEMICAL ENGINEERING JOURNAL 483 (2024) . |
| APA | Su, Chenxin , Zhou, Shouquan , Wu, Shaoyun , Gao, Mingbin , Zhang, Weiling , Ma, Zhuang et al. Highly efficient dehydration of polyols: In-situ Brempty setnsted acid from boron phosphate catalyst . | CHEMICAL ENGINEERING JOURNAL , 2024 , 483 . |
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Polyoxometalate (POM)-based materials are ideal candidates for implementing molecular memories, and rational POM molecule design is key to higher resistive switching (RS) performance. In this work, in order to obtain a deep structure-property correlation of POM-based memristors, three Anderson-based hybrids, i.e. two-component hybrids (MV)3(MnMo6O18L2)2·4DMF (1) and (MV)2[Cu(DMF)2](MnMo6O18L1)2·6DMF (2), and the three-component one (MV)2(Cu2I3)(MnMo6O18L2)·4CH3CN (3) (L = 2-(hydroxymethyl)-2-(pyridine-4-yl)-1,3-propanediol) have been structurally determined. These hybrids together with the precursors (methyl viologen (MV2+), CuI, and (MnMo6O18L2)) were further fabricated as memristors with the structure of ITO/active layer/Ag. Interestingly, three precursors are RS silent or have bad RS performance, but the incorporation of MV2+ in 1 and 2 can trigger the RS performances, and the further decoration of iodocuprate in 3 can render enhanced RS behavior (ON/OFF ratio: 2.32 × 102) with high thermal-tolerance temperature (240 °C) and extremely long-term stability. The RS mechanism could be assigned to the valence change (VC) induced by oxygen vacancy migrations. The presence of air-stable (MnMo6O18L2)3−-MV2+ donor-acceptor couples can stabilize the oxygen vacancies, which not only trigger the RS behaviors in ITO/1/Ag and ITO/2/Ag, but also result in extremely long-term stability in ITO/3/Ag. Besides, the oxygen vacancies can also be stabilized by Cu2I3 with intense cuprophilic interactions, which corresponds to enhanced RS properties in ITO/3/Ag. This mechanism could be validated by the following structural characters in 3: the stronger POM-MV2+ interactions, the better planarity of MV2+, the very short Cu⋯Cu distances and the ABAB-type packing fashion. The structure-property correlation in this work can provide a new strategy for the development of highly efficient and reliable memristors. © 2024 The Royal Society of Chemistry.
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| GB/T 7714 | Chen, H.-B. , He, M.-Y. , Li, T. et al. Exploring the role of viologen and iodocuprate in the enhanced resistive switching performance of Anderson polyoxometalate-based three-component hybrids [J]. | Journal of Materials Chemistry C , 2024 , 12 (34) : 13555-13561 . |
| MLA | Chen, H.-B. et al. "Exploring the role of viologen and iodocuprate in the enhanced resistive switching performance of Anderson polyoxometalate-based three-component hybrids" . | Journal of Materials Chemistry C 12 . 34 (2024) : 13555-13561 . |
| APA | Chen, H.-B. , He, M.-Y. , Li, T. , Deng, C.-C. , Xiao, H.-P. , Qi, M.-Q. et al. Exploring the role of viologen and iodocuprate in the enhanced resistive switching performance of Anderson polyoxometalate-based three-component hybrids . | Journal of Materials Chemistry C , 2024 , 12 (34) , 13555-13561 . |
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In the field of biomemorizers, the simultaneous enhancement of resistive switching (RS) performance and environmental robustness, and the understanding the RS mechanism involving interfacial interaction is still challengeable. Herein, the bio-composites by encapsulating graphene (GR), graphene oxide (GO) and reduced graphene oxide (RGO) into chitosan (CS) have been fabricated as memory devices with the structure of FTO/biocomposite/Ag. Among them, FTO/GO@CS(12 %)/Ag biomemorizer exhibits the best RS performance with high ON/OFF ratio (10 5.92 ), and it possesses good thermal (170 degrees C) and irradiation stabilities (UV exposure for 96 h). The RS mechanism is due to the migration of oxygen vacancies accompanied by formation of Ag conducting filaments in the bio-composite films. Therefore, the enhanced resistive switching performance after encapsulating into CS can be explained as the increment of defects, the higher current densities and quenched radicals. Specially, for the first time we find the presence of voltage -induced packing mode changes in GO@CS composite, which can facilitate the migration of oxygen vacancies and render its best RS performance. In all, the more carboxyl groups can strengthen the GO -CS interfacial interactions through the formation of stable hydrogen bonding network and covalent bonds, which can enhance the stabilities and makes the composites be more sensitive to electrical stimulus. The rules drawn in this work will be significant for the construction of new biomemorizers with good environmental robustness.
Keyword ：
Biomemorizer Biomemorizer Chitosan Chitosan Environmental robustness Environmental robustness Graphene derivant Graphene derivant Resistive switching mechanism Resistive switching mechanism
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| GB/T 7714 | Zheng, Mei -Qin , Yi, Hong -Mei , Yu, Guo et al. Graphene derivant@chitosan composite-based biomemorizers: The effect of functional groups on the resistive switching performances and their thermal/irradiative stabilities [J]. | DIAMOND AND RELATED MATERIALS , 2024 , 146 . |
| MLA | Zheng, Mei -Qin et al. "Graphene derivant@chitosan composite-based biomemorizers: The effect of functional groups on the resistive switching performances and their thermal/irradiative stabilities" . | DIAMOND AND RELATED MATERIALS 146 (2024) . |
| APA | Zheng, Mei -Qin , Yi, Hong -Mei , Yu, Guo , Wang, Jia-Wei , Lv, Zhou -Lin , Li, Hui -Fang et al. Graphene derivant@chitosan composite-based biomemorizers: The effect of functional groups on the resistive switching performances and their thermal/irradiative stabilities . | DIAMOND AND RELATED MATERIALS , 2024 , 146 . |
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The Microscale Oscillatory Flow Reactor (MOFR) can achieve good plug flow and micromixing performance simultaneously at laminar net flow conditions. An unbaffled U-shaped microreactor coupled with oscillating flow technology was designed to study the macro and micromixing performance. Firstly, the influence of oscillations on the flow performance was studied to reveal the formation rule of vortex. The simulation results showed that the continuous formation and destruction of periodic vortexes occurred in the microreactor with oscillation. With the increase of oscillation intensity, the vortex size in the radial direction first gradually increased and then becomes stable, and gradually moved axially, resulting in axial diffusion. Secondly, the effect of oscillation on the macromixing and micromixing performance were investigated. The results showed that the coupling oscillation could greatly improve the macromixing and micromixing performance. The macromixing and micromixing performance were promoted simultaneously at lower oscillation intensity and then tended to be flat due to the axial diffusion at high oscillation intensity. When φ>6.05, the minimum micromixing time and the maximum number of tanks can be achieved at the same time. At a velocity ratio of about 23, FoM reached a maximum of about 3.5. © 2024
Keyword ：
Computational fluid dynamics Computational fluid dynamics Diffusion Diffusion Laminar flow Laminar flow Oscillating flow Oscillating flow Vortex flow Vortex flow
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| GB/T 7714 | Yu, Liping , Zheng, Meiqin , Wang, Jiawei et al. Enhanced mixing characteristics of unbaffled U-shaped microreactor coupled oscillatory flow [J]. | Chemical Engineering and Processing - Process Intensification , 2024 , 205 . |
| MLA | Yu, Liping et al. "Enhanced mixing characteristics of unbaffled U-shaped microreactor coupled oscillatory flow" . | Chemical Engineering and Processing - Process Intensification 205 (2024) . |
| APA | Yu, Liping , Zheng, Meiqin , Wang, Jiawei , Yan, Zuoyi , Yao, Wei , Li, Haohong et al. Enhanced mixing characteristics of unbaffled U-shaped microreactor coupled oscillatory flow . | Chemical Engineering and Processing - Process Intensification , 2024 , 205 . |
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The low ternary yield and expensive organic active materials hinder the potential industrialization of organic multi-level resistive memories. Here, facile melamine (M)-cyanuric acid (C) hydrogen-bonded organic frame-work (M -C HOF) was firstly fabricated as a new type of ternary memorizer. In the M -C HOF, the robust graphite-like planar 2D sheet along ab-plane containing a rosette motif is constructed from nine hydrogen bonds among M and C, and the 2D sheets are stacked into a 3D network through strong pi-pi stacking interactions. The FTO/M-C/Ag device exhibits a typical ternary memory performance with considerable OFF/ON1/ON2 current ratio of 1:103.1:104.6, relatively low set voltages (1.14 and 1.70 V), good reliability, and high ternary device yield of 74 %. The ternary resistive switching behavior could be ascribed to the filled traps in 2D layer (for ON1 state) and the carriers flowing in 3D network (for ON2 state), which have been verified by quenched fluorescence of isolated M and C, increased (201) lattice plane distance upon external voltages. Besides, this ternary memorizer has superior thermal stability (300 degrees C) and irradiative tolerance. This attempt of HOF-based ternary memorizer presents a new choice for efficient and facial multi-level resistive material.
Keyword ：
Hydrogen-bonded organic framework Hydrogen-bonded organic framework Memorizers in harsh environment Memorizers in harsh environment Ternary resistive memorizer Ternary resistive memorizer Ternary resistive switching mechanism Ternary resistive switching mechanism
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| GB/T 7714 | Song, Kaiyue , Yang, Hailong , Chen, Binjun et al. The facile implementing ternary resistive memory in graphite-like melamine-cyanuric acid hydrogen-bonded organic framework with high ternary yield and environmental tolerance [J]. | APPLIED SURFACE SCIENCE , 2023 , 608 . |
| MLA | Song, Kaiyue et al. "The facile implementing ternary resistive memory in graphite-like melamine-cyanuric acid hydrogen-bonded organic framework with high ternary yield and environmental tolerance" . | APPLIED SURFACE SCIENCE 608 (2023) . |
| APA | Song, Kaiyue , Yang, Hailong , Chen, Binjun , Lin, Xiaoli , Liu, Yue , Liu, Yuanzheng et al. The facile implementing ternary resistive memory in graphite-like melamine-cyanuric acid hydrogen-bonded organic framework with high ternary yield and environmental tolerance . | APPLIED SURFACE SCIENCE , 2023 , 608 . |
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Two new heterometallic uranyl-organic frameworks (UOFs), [Cd(phen)(2)(H2O)(2)][(UO2)(2)(BDC)(3)]center dot 2H(2)O (1) and [Ni(phen)(3)][(UO2)(2)(BDC)(3)]center dot 2H(2)O (2), were obtained under hydrothermal conditions. Both crystal structures were characterized by single-crystal X-ray diffraction analyses and the results indicate that both complexes feature a similar 2D honeycomb framework that is connected by rigid benzenedicarboxylate (BDC) ligands and uranyl units. BDC works as a linker to bridge neighboring UO22+ units, where UO22+ is tris-chelated. Different guest molecules guided the stacking of 2D layers and lead into their 3D supramolecular crystal structures with different space groups. As a result, 1 crystallized in a polar space group Cc, whereas 2 belongs to a chiral space group P6(1)22. Thermogravimetric measurements were performed to study their thermal stability. UV-visible diffuse reflectance spectroscopy measurements indicate an experimental optical bandgap of 3.87 eV and 3.63 eV, respectively, for 1 and 2. Luminescent studies of both samples show strong green light emissions.
Keyword ：
crystal structure crystal structure Heterometallic Heterometallic luminescence luminescence uranyl complexes uranyl complexes
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| GB/T 7714 | Wu, Hong-Yan , Luo, Ju-Xiang , Li, Hao-Hong et al. Guest molecular guided syntheses of 2-dimensional uranyl complexes with rigid benzenedicarboxylate ligands [J]. | JOURNAL OF COORDINATION CHEMISTRY , 2023 , 76 (2) : 292-306 . |
| MLA | Wu, Hong-Yan et al. "Guest molecular guided syntheses of 2-dimensional uranyl complexes with rigid benzenedicarboxylate ligands" . | JOURNAL OF COORDINATION CHEMISTRY 76 . 2 (2023) : 292-306 . |
| APA | Wu, Hong-Yan , Luo, Ju-Xiang , Li, Hao-Hong , Zhang, Jian-Han . Guest molecular guided syntheses of 2-dimensional uranyl complexes with rigid benzenedicarboxylate ligands . | JOURNAL OF COORDINATION CHEMISTRY , 2023 , 76 (2) , 292-306 . |
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Background: Drug-resistant microbes pose a global health concern, requiring the urgent development of effective antibacterial agents and strategies in clinical practice. Therefore, there is an urgent need to explore novel antibacterial materials to effectively eliminate bacteria. The synthesis of quaternary phosphonium salt in haloargentate systems, wherein the phosphorus atom is represented in a cationic form, is a possible strategy for the development of antibacterial materials.Methods: Using (triphenyl)phosphonium-based quaternary phosphorus salts with different spacer lengths (n=2, 4, 6) as a template, we designed three kinds of quaternary phosphorus salts as effective antibacterial agents against drug-resistant bacteria.Results: The synthesized quaternary phosphorus salt of (1,4-DBTPP)Br2 effectively prevented the formation of the bacterial biofilms, and degraded bacterial membranes and cell walls by promoting the production of reactive oxygen species, which exhibited effective therapeutic effects in a rat model of a superficial wound infected with methicillin-resistant Staphylococcus aureus. Conclusion: The quaternary phosphorus salt (1,4-DBTPP)Br2 demonstrated hemocompatibility and low toxicity, revealing its potential in the treatment of clinical infections.
Keyword ：
antibacterial antibacterial biocompatible biocompatible quaternary phosphorus salts quaternary phosphorus salts reactive oxygen species reactive oxygen species wound infection therapy wound infection therapy
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| GB/T 7714 | Shi, Liang-Wen , Zhuang, Quan-Quan , Wang, Tai-Qin et al. Synthetic Antibacterial Quaternary Phosphorus Salts Promote Methicillin-Resistant Staphylococcus aureus-Infected Wound Healing [J]. | INTERNATIONAL JOURNAL OF NANOMEDICINE , 2023 , 18 : 1145-1158 . |
| MLA | Shi, Liang-Wen et al. "Synthetic Antibacterial Quaternary Phosphorus Salts Promote Methicillin-Resistant Staphylococcus aureus-Infected Wound Healing" . | INTERNATIONAL JOURNAL OF NANOMEDICINE 18 (2023) : 1145-1158 . |
| APA | Shi, Liang-Wen , Zhuang, Quan-Quan , Wang, Tai-Qin , Jiang, Xian-Dong , Liu, Yue , Deng, Jing-Wen et al. Synthetic Antibacterial Quaternary Phosphorus Salts Promote Methicillin-Resistant Staphylococcus aureus-Infected Wound Healing . | INTERNATIONAL JOURNAL OF NANOMEDICINE , 2023 , 18 , 1145-1158 . |
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