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学者姓名：谭文
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Abstract ：
We present a novel design of a ferroelectric fast reactive tuner (FE-FRT) capable of modulating megaVAR reactive power on a submicrosecond timescale. The high reactive power capability of our design extends the range of applications of reactive tuners to numerous applications. We present a detailed analytical model of the performance of a megawatt-class reactive power device and benchmark it against finite-element method eigenmode and frequency domain electromagnetic simulations. We introduce new features, including an annulus design for the ferroelectric capacitors and capacitive window coupling to the cavity. We consider thermal design issues and nonlinear effects in the ferroelectric. The model covers several configurations, allowing control of the frequency of superconducting and normal-conducting cavities in a variety of applications and frequencies. We calculate that the FE-FRT designed should be capable of handling around 0.45 MVAR of reactive power with around 3 kW of resistive losses, providing a frequency tuning range of 8 kHz in an example of 400 MHz cavity geometry.
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| GB/T 7714 | Zhong, Shuiping , Xu, Tingyu , Chen, Hang et al. Conceptual design of a high reactive-power ferroelectric fast reactive tuner [J]. | JOURNAL OF ENVIRONMENTAL SCIENCES , 2025 , 151 . |
| MLA | Zhong, Shuiping et al. "Conceptual design of a high reactive-power ferroelectric fast reactive tuner" . | JOURNAL OF ENVIRONMENTAL SCIENCES 151 (2025) . |
| APA | Zhong, Shuiping , Xu, Tingyu , Chen, Hang , Tang, Ding , Tan, Wen , Weng, Wei et al. Conceptual design of a high reactive-power ferroelectric fast reactive tuner . | JOURNAL OF ENVIRONMENTAL SCIENCES , 2025 , 151 . |
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电解锰行业面临电效低、SeO_2添加剂剧毒且沉积产物形貌难控制等问题.为了提高电流效率以降低能耗、改善锰电沉积形貌及降低添加剂SeO_2的使用量，本文根据电解锰行业标准，配制MnSO_4–(NH_4)_2SO_4电解液体系，通过添加聚丙烯酸、甘氨酸、乙二胺四乙酸(EDTA)、葡萄糖酸等分别作辅助添加剂，探究其对锰沉积的影响以降低剧毒性主添加剂SeO_2的用量.采用场发射扫描电子显微镜(SEM)、X射线衍射分析(XRD)、恒电流阴极极化曲线测试方法 (LSV)等表征手段，研究金属锰沉积形貌、晶体结构、阴极电化学极化行为与添加剂之间的关系.结果表明：四种添加剂均可以促进α-Mn的形成，且最优晶型取向为(330)晶面，其中葡萄糖酸最适宜作为辅助添加剂.当以葡萄糖酸为辅助添加剂，质量浓度为1.84 g·L~(-1)时，阴极电流密度明显提高，降低了阴极极化，产品形貌更加致密光滑.最优条件下，SeO_2的质量浓度可由工业上常规用量0.03～0.06 g?L~(-1)降低至0.015 g?L~(-1)，电流效率可由70%提高至89.73%，能耗由6500 kW·h·t~(-1)降至4990.58 kW·h·t~(-1).研究结果有望为电解锰行业绿色生产和高效电沉积提供借鉴，有助于推动电解锰行业的可持续发展.
Keyword ：
有机物 有机物 极化行为 极化行为 添加剂 添加剂 电流效率 电流效率 电解锰 电解锰
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| GB/T 7714 | 迟晓鹏 , 张瑞莹 , 翁威 et al. 有机添加剂对电解锰的影响 [J]. | 工程科学学报 , 2024 , 46 (05) : 835-843 . |
| MLA | 迟晓鹏 et al. "有机添加剂对电解锰的影响" . | 工程科学学报 46 . 05 (2024) : 835-843 . |
| APA | 迟晓鹏 , 张瑞莹 , 翁威 , 苏国晖 , 谭文 , 衷水平 . 有机添加剂对电解锰的影响 . | 工程科学学报 , 2024 , 46 (05) , 835-843 . |
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Electrolytic manganese is an important metal material that is widely employed in batteries, electronics, steel, and other fields. However, there are many issues regarding the production process of electrolytic manganese, such as low current efficiency, high-content toxic SeO2 additives in the electrolyte, and difficulty in controlling the product morphology. These issues not only impact the production efficiency and quality of electrolytic manganese but also result in severe environmental pollution. To address these issues, a MnSO4-(NH4)2SO4 electrolyte system was prepared based on the electrolytic manganese industry standard. The effects of polyacrylic acid, glycine, ethylenediaminetetraacetic acid (EDTA), and gluconic acid were explored as auxiliary additives under neutral electrolysis conditions to lower the SeO2 content, which is a highly toxic main additive. The effects of the different additives on the metal manganese morphology, crystal structure, and cathodic electrochemical polarization behavior were examined by field-emission scanning electron microscopy, X-ray diffraction, and constant current cathodic polarization curve tests. The findings reveal that the main orientation of the metal manganese crystal form deposited by the four auxiliary additives is the (330) crystal plane, and all of them can promote the formation of α-Mn, enhance the electrolysis efficiency, and lower the energy consumption. In particular, the optimized amount of polyacrylic acid of 0.08 g·L−1 contributes to an energy consumption of 5735.34 kW·h·t−1. Correspondingly, the addition of 10 g·L−1 glycine is the most favorable amount, leading to an energy consumption of 5518.56 kW·h·t−1. For EDTA, the lowest energy consumption of 5168.26 kW·h·t−1 is measured at an added amount of 0.5 g·L−1. Note that among the four investigated candidates, gluconic acid is the most favorable auxiliary additive, contributing to the increased cathode current density and reduced cathodic polarization as well as denser metal manganese products. Moreover, gluconic acid addition can lower the concentration of toxic SeO2 from 0.03-0.06 to 0.015 g·L−1, significantly increase the cathode current density, reduce the cathodic polarization, and result in a more dense and smooth product morphology, with the current efficiency being increased from approximately 70% to 89.73% and energy consumption being reduced from 6500 to 4990.58 kW·h·t−1 at the same time. Gluconic acid, as the auxiliary additive, not only contributes to the best electrolysis indexes for electrolytic manganese but also facilitates the formation of metal manganese with the most desirable crystal structure. This work offers novel insights into the environmentally friendly production and cheap electrodeposition of metal manganese for the electrolytic manganese industry. © 2024 Science Press. All rights reserved.
Keyword ：
Additives Additives Amino acids Amino acids Cathodic polarization Cathodic polarization Crystal orientation Crystal orientation Current density Current density Electrolysis Electrolysis Electrolytes Electrolytes Energy efficiency Energy efficiency Energy utilization Energy utilization Ethylenediaminetetraacetic acid Ethylenediaminetetraacetic acid Field emission cathodes Field emission cathodes Field emission microscopes Field emission microscopes Manganese Manganese Manganese compounds Manganese compounds Morphology Morphology Nitrogen compounds Nitrogen compounds Scanning electron microscopy Scanning electron microscopy Selenium compounds Selenium compounds
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| GB/T 7714 | Chi, Xiaopeng , Zhang, Ruiying , Weng, Wei et al. Effect of organic additives on manganese electrolysis [J]. | Chinese Journal of Engineering , 2024 , 46 (5) : 835-843 . |
| MLA | Chi, Xiaopeng et al. "Effect of organic additives on manganese electrolysis" . | Chinese Journal of Engineering 46 . 5 (2024) : 835-843 . |
| APA | Chi, Xiaopeng , Zhang, Ruiying , Weng, Wei , Su, Guohui , Tan, Wen , Zhong, Shuiping . Effect of organic additives on manganese electrolysis . | Chinese Journal of Engineering , 2024 , 46 (5) , 835-843 . |
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无氰亚硫酸盐电沉积金体系面临电流效率低、镀液稳定性差、循环周期短、镀层性能难以满足工业发展需求等问题。为了提高电流效率、镀液稳定性和镀层表面光泽度，改善电沉积金形貌及提高镀层性能，配制了亚硫酸金钠电镀液体系，通过添加不同质量浓度乙二胺（EDA）作为辅助添加剂，研究了EDA对镀液稳定性、电沉积产物表面形貌、元素组成和晶体晶面取向，以及金镀层光泽度、硬度和粗糙度的影响。采用电化学测试进一步研究EDA对溶液中Au~+行为的影响。结果表明：EDA使吸附Au~+的活性位点增加了2.8倍，同时增加了阴极表面的极化并促进晶粒细化，增强了Au(111）晶面的峰强度。EDA质量浓度为15 g/L时，电镀液能保存6个月以上，电流效率从54%提高到98%，金镀层表面均匀性、光泽度和硬度明显提高，镀层表面粗糙度、腐蚀速率明显降低，镀层综合性能最优。本研究有望为亚硫酸盐电镀体系开发新型高效添加剂提供借鉴，有助于推动电镀金行业的可持续发展。
Keyword ：
乙二胺 乙二胺 亚硫酸盐 亚硫酸盐 无氰电沉积金 无氰电沉积金 电化学 电化学 硬度 硬度 耐腐蚀性 耐腐蚀性
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| GB/T 7714 | 衷水平 , 徐婷钰 , 陈江濠 et al. 乙二胺添加剂对无氰亚硫酸盐体系电沉积金的影响 [J]. | 铜业工程 , 2024 , PageCount-页数: 11 (04) : 44-54 . |
| MLA | 衷水平 et al. "乙二胺添加剂对无氰亚硫酸盐体系电沉积金的影响" . | 铜业工程 PageCount-页数: 11 . 04 (2024) : 44-54 . |
| APA | 衷水平 , 徐婷钰 , 陈江濠 , 迟晓鹏 , 谭文 , 翁威 et al. 乙二胺添加剂对无氰亚硫酸盐体系电沉积金的影响 . | 铜业工程 , 2024 , PageCount-页数: 11 (04) , 44-54 . |
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锂云母酸法浸出液含有大量杂质金属，使用传统化学沉淀法会引起大量产物损失。为了降低浸出液除杂过程中的产物损失，使用溶剂萃取法进行萃取除杂工艺研究。通过对不同萃取剂组合萃取除杂效果的研究，确定使用P204作为萃取剂。考察了萃取过程中不同因素的影响，并使用H_2O_2预氧化水相里的Fe~(2+),强化萃取效果。结果表明：在有机相组成为30%P204+70%磺化煤油、料液初始pH为2.4、相比O/A=1、萃取时间10min和振荡频率300 r/min的单级萃取最佳条件下，铁除杂率为99.89%、铝除杂率为31.23%、锂和铷的萃取率分别为7.63%和14.85%。相比于化学沉淀法，锂和铷的回收率得到了30%左右的提高。
Keyword ：
P204 P204 化学沉淀法 化学沉淀法 溶剂萃取法 溶剂萃取法 硫酸浸出 硫酸浸出 锂云母 锂云母
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| GB/T 7714 | 梁东辉 , 谭文 , 翁威 et al. 锂云母酸浸液萃取除杂 [J]. | 有色金属(冶炼部分) , 2024 , (07) : 76-84 . |
| MLA | 梁东辉 et al. "锂云母酸浸液萃取除杂" . | 有色金属(冶炼部分) 07 (2024) : 76-84 . |
| APA | 梁东辉 , 谭文 , 翁威 , 迟晓鹏 , 衷水平 . 锂云母酸浸液萃取除杂 . | 有色金属(冶炼部分) , 2024 , (07) , 76-84 . |
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Lithium and its associated rubidium are regarded as the strategic metal resource, which have a wide use in many commercial products. Nowadays, the continuing growth in demand for Li resources, propelling the object of industrial exploitation will focus on low-grade, complex minerals composition and unwieldy ores. Zinnwaldite has received increasing attention as a potential lithium-containing resource in recent years. However, there are a lack of effective extraction processes for zinnwaldite. Hence, this paper proposes an effective method to extract metal cleanly and efficiently from zinnwaldite by using CaO and B2O3 2 O 3 as thermal activation additives and H2SO4 2 SO 4 as the leaching agent. The results showed that the destruction of Fe-O and Si-O-Si bonds led to increased extraction efficiency. The breathing vibrations of oxygen atoms symmetric in 4- and 3-membered rings and Si-O symmetric stretch could influence the Li separation from silica skeleton. Ultimately, the 91.32 % Li, 93.09% Rb, 81.14 % Fe, 95.00 % Al and 71.12 % K were recovered under the optimal conditions. Meanwhile, about 10 % F escaped into the air during thermal activation and the concentration of F in the leaching solution was lower than 2 mg/L. The use of B2O3 2 O 3 provides a valuable reference for the efficient and clean treatment of lepidolite using the salt roasting method.
Keyword ：
Acid leaching Acid leaching Boron oxide Boron oxide Calcium oxide Calcium oxide Thermal activation Thermal activation Zinnwaldite Zinnwaldite
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| GB/T 7714 | Zhong, Shuiping , Liang, Donghui , Weng, Wei et al. Efficient extraction of Li and Rb from zinnwaldite via thermal activation and acid leaching [J]. | MINERALS ENGINEERING , 2024 , 216 . |
| MLA | Zhong, Shuiping et al. "Efficient extraction of Li and Rb from zinnwaldite via thermal activation and acid leaching" . | MINERALS ENGINEERING 216 (2024) . |
| APA | Zhong, Shuiping , Liang, Donghui , Weng, Wei , Chi, Xiaopeng , Zhang, Wengze , Tan, Wen . Efficient extraction of Li and Rb from zinnwaldite via thermal activation and acid leaching . | MINERALS ENGINEERING , 2024 , 216 . |
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Surface engineering of both morphology and composition is appealing strategy for further boosting the hydrogen evolution reaction (HER) performances of commercial bulk nickel electrode in alkaline media. However, modified surface structure with long-term stability is still in desperate need, especially at industrial-scale current density. Herein, by grafting the commercial nickel electrode with well-aligned nickel-rhenium (Ni–Re) alloy particles, the electrode surface turns to be highly hydrophilic, thus propelling the detachment of hydrogen (H2) bubbles from the electrode surface. In addition, the synergy within the dual Ni–Re atom optimizes the electronic structure of electrode surface, lowering the energy barriers for water dissociation. Resultantly, the NiRe-modified nickel bulk electrode shows fascinating HER performance in both activity and long-term stability, namely overpotential of 191 mV@100 mA cm−2, stable operation for 2000 h at 200 mA cm−2 in H-type cell, and steady running for >1000 h at 1000 mA cm−2 using the configuration of Ni||Ni-60 %Re in the membrane electrode assembly, outperforming that of the benchmark Pt/C catalysts. The results can provide new insights for the tradeoff between activity and cost towards high-performance alkaline water electrolysis. © 2024 Elsevier B.V.
Keyword ：
Benchmarking Benchmarking Electrodes Electrodes Electronic structure Electronic structure Grafting (chemical) Grafting (chemical) Hydrogen Hydrogen Morphology Morphology Nickel Nickel Surface reactions Surface reactions Surface structure Surface structure
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| GB/T 7714 | Weng, Wei , Zhang, Wenze , Lei, Tianhan et al. Grafting nickel electrode with self-supporting semispherical NiRe particles for stably large-current alkaline hydrogen evolution reaction [J]. | Journal of Power Sources , 2024 , 614 . |
| MLA | Weng, Wei et al. "Grafting nickel electrode with self-supporting semispherical NiRe particles for stably large-current alkaline hydrogen evolution reaction" . | Journal of Power Sources 614 (2024) . |
| APA | Weng, Wei , Zhang, Wenze , Lei, Tianhan , Tan, Wen , Chi, Xiaopeng , Zhong, Shuiping . Grafting nickel electrode with self-supporting semispherical NiRe particles for stably large-current alkaline hydrogen evolution reaction . | Journal of Power Sources , 2024 , 614 . |
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为了实现铜冶炼含砷烟尘中有价金属的回收和砷元素的无害化处理，采用电沉积法对含砷烟尘的浸出液进行脱砷处理，研究了电流密度、As(Ⅲ)浓度、pH和添加剂对脱砷效果的影响，并用循环伏安法分析了电化学行为。结果表明，最佳工艺条件下，砷单质、H_2和AsH_3的电流效率分别为91.41%、7.06%和1.99%,实现了高效脱砷。添加柠檬酸钠可降低电沉积的还原电位，促进金属放电。本文提出的工艺可回收有价金属，无害化处置砷元素。
Keyword ：
含砷烟尘 含砷烟尘 柠檬酸钠 柠檬酸钠 电沉积 电沉积 砷 砷 铜冶炼 铜冶炼
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| GB/T 7714 | 罗子健 , 许佳妍 , 翁威 et al. 电沉积脱砷工艺研究及添加剂对电沉积的影响 [J]. | 有色金属(冶炼部分) , 2023 , (10) : 7-16 . |
| MLA | 罗子健 et al. "电沉积脱砷工艺研究及添加剂对电沉积的影响" . | 有色金属(冶炼部分) 10 (2023) : 7-16 . |
| APA | 罗子健 , 许佳妍 , 翁威 , 谭文 , 迟晓鹏 , 衷水平 . 电沉积脱砷工艺研究及添加剂对电沉积的影响 . | 有色金属(冶炼部分) , 2023 , (10) , 7-16 . |
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采用“富铼渣浸出—浸出液预处理—萃取—反萃—结晶”工艺流程，研究了铜冶炼富铼渣提铼工艺，着重考察浸出工序中H_2O_2用量、硫酸浓度、浸出时间和浸出温度等对铼浸出率的影响，以及预处理工序中CaO用量对铼、砷回收率的影响。结果表明：在50 g富铼渣、H_2O_2用量150 mL、初始液固比2、初始硫酸浓度20 g/L、室温(20～25℃)搅拌浸出2 h的最优条件下，铼浸出率可达92.2%,砷浸出率达到96.6%;浸出液经过CaO预处理后，“预处理—萃取—反萃”工序铼总回收率超过98%,砷总回收率不到1.8%,实现了铼与砷的有效分离；一次结晶所得铼酸铵的纯度约为95%,铼结晶率为66%。
Keyword ：
富铼渣 富铼渣 浸出 浸出 萃取 萃取 铼酸铵 铼酸铵
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| GB/T 7714 | 衷水平 , 涂宾 , 翁威 et al. 铜冶炼富铼渣提铼工艺 [J]. | 有色金属(冶炼部分) , 2023 , (07) : 57-62 . |
| MLA | 衷水平 et al. "铜冶炼富铼渣提铼工艺" . | 有色金属(冶炼部分) 07 (2023) : 57-62 . |
| APA | 衷水平 , 涂宾 , 翁威 , 迟晓鹏 , 谭文 . 铜冶炼富铼渣提铼工艺 . | 有色金属(冶炼部分) , 2023 , (07) , 57-62 . |
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Real-time and rapid determination of trace copper ion (Cu2+) in the electrolyte of zinc smelting process is urgently needed. However, the complicated composition of the electrolyte, especially the extremely high-concentration of zinc ion (Zn2+) may cause severe interference to the detection of Cu2+. This work describes a facile electrochemical sensor for Cu2+ determination in the electrolyte of zinc smelting plants based on a fluorine-doped tin oxide (FTO) electrode with silver nanowires (AgNWs) and Nafion modification. The AgNWs/Nafion-FTO electrode showed good detection ability with the linear detection range of 0.2-2 mg l-1 Cu2+ in 45 g l-1 Zn2+ solution using differential pulse anodic stripping voltammetry (DPASV) technique. With DPASV technique, Cu2+ can be first reduced and pre-concentrated on the working electrode surface at -0.6 V vs Ag/AgCl for 500 s, after which the deposited Cu metal is oxidized around 0 V vs Ag/AgCl during the stripping step. It has been proved by transmission electron microscopy (TEM) and X-ray photoelectron spectra (XPS) that trace Cu2+ can be adsorbed and reduced on AgNWs in solutions with Zn/Cu ratio up to (2.25-22.5) x 104. The results extend AgNWs modified electrode to the industrial solution, providing a new strategy for detection of trace metal ions in industrial solutions.
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| GB/T 7714 | Xiao, Ni , Chen, Yinan , Tan, Wen et al. Extending Silver Nanowire Modified Electrodes to Industrial Zinc Electrolyte for Copper Ion Detection [J]. | JOURNAL OF THE ELECTROCHEMICAL SOCIETY , 2023 , 170 (9) . |
| MLA | Xiao, Ni et al. "Extending Silver Nanowire Modified Electrodes to Industrial Zinc Electrolyte for Copper Ion Detection" . | JOURNAL OF THE ELECTROCHEMICAL SOCIETY 170 . 9 (2023) . |
| APA | Xiao, Ni , Chen, Yinan , Tan, Wen , Ku, Jiangang , Wang, Qiang , Chen, Hang et al. Extending Silver Nanowire Modified Electrodes to Industrial Zinc Electrolyte for Copper Ion Detection . | JOURNAL OF THE ELECTROCHEMICAL SOCIETY , 2023 , 170 (9) . |
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