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author:

Liao, S. (Liao, S..) [1] | Dong, G. (Dong, G..) [2] | Han, B. (Han, B..) [3] | Wei, J. (Wei, J..) [4] | Zhang, Y. (Zhang, Y..) [5] | Guo, Y. (Guo, Y..) [6] | Lin, T. (Lin, T..) [7] | Lin, C. (Lin, C..) [8] | Zhao, C. (Zhao, C..) [9] | Gao, M. (Gao, M..) [10] | Wu, X. (Wu, X..) [11] | Wen, N. (Wen, N..) [12] | Fan, H. (Fan, H..) [13] | Zheng, Y. (Zheng, Y..) [14] | Gao, F. (Gao, F..) [15] | Zheng, X. (Zheng, X..) [16]

Indexed by:

Scopus

Abstract:

The bioluminescence mechanisms of deep-sea organisms provide innovative ideas for biomimetic design. To meet the detection needs in low-light deep-sea environments, the development of soft robots with high-brightness luminescence is crucial for long-term in situ observation. Directly incorporating high-performance fluorescent molecules into hydrogel matrices presents challenges: fluorescent molecules tend to dissociate in physically crosslinked systems, and complex aqueous environments may lead to instability in the material structure. These issues limit the fluorescence stability and service life of underwater devices. Inspired by the behaviors of marine organisms, this study proposes a biomimetic soft actuator with high fluorescence intensity. The actuator adopts a bilayer hydrogel structure, where the luminescent layer (PT4B-N), covalently crosslinked with fluorescent molecules, achieves a high photoluminescence quantum yield (PLQY > 60%), and the pH-responsive driving layer (PNPC) enables motion control (strip-shaped hydrogel: maximum bending angle ≈360°, cycle time ≈20 min). The experimental results demonstrate that the actuator can realize biological-like synergic fluorescence and shape change (SFSC) behavior. © 2025 Wiley-VCH GmbH.

Keyword:

aggregation-induced emission biomimetic soft actuator fluorescent hydrogel

Community:

  • [ 1 ] [Liao S.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 2 ] [Dong G.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 3 ] [Han B.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 4 ] [Wei J.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 5 ] [Zhang Y.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 6 ] [Guo Y.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 7 ] [Lin T.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 8 ] [Lin C.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 9 ] [Zhao C.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 10 ] [Gao M.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 11 ] [Wu X.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 12 ] [Wen N.]College of Materials Science and Engineering, Fuzhou University, Fuzhou, 350108, China
  • [ 13 ] [Fan H.]Department of Anesthesiology, Fuzhou University Affiliated Provincial Hospital, Fuzhou, 350001, China
  • [ 14 ] [Zheng Y.]Shengli Clinical Medical College of Fujian Medical University, Fuzhou, 350122, China
  • [ 15 ] [Gao F.]Department of Anesthesiology, Fuzhou University Affiliated Provincial Hospital, Fuzhou, 350001, China
  • [ 16 ] [Gao F.]Shengli Clinical Medical College of Fujian Medical University, Fuzhou, 350122, China
  • [ 17 ] [Gao F.]Fujian Provincial Key Laboratory of Emergency Medicine, Fujian Provincial Key Laboratory of Critical Care Medicine, Fujian Provincial Co-Constructed Laboratory of “belt and Road”, Fujian Emergency Medical Center, Fuzhou, 350001, China
  • [ 18 ] [Zheng X.]Department of Anesthesiology, Fuzhou University Affiliated Provincial Hospital, Fuzhou, 350001, China
  • [ 19 ] [Zheng X.]Shengli Clinical Medical College of Fujian Medical University, Fuzhou, 350122, China
  • [ 20 ] [Zheng X.]Fujian Provincial Key Laboratory of Emergency Medicine, Fujian Provincial Key Laboratory of Critical Care Medicine, Fujian Provincial Co-Constructed Laboratory of “belt and Road”, Fujian Emergency Medical Center, Fuzhou, 350001, China

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Small

ISSN: 1613-6810

Year: 2025

1 3 . 0 0 0

JCR@2023

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ESI Highly Cited Papers on the List: 0 Unfold All

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30 Days PV: 0

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