Phosphate　and　fluoride　ions　are　common　water　pollutants　whose　presence　and　excessive　discharge　cause　potential　hazards　to　the　environment　and　human　health.　MOF　materials　commonly　used　to　remove　phosphate　and　fluoride　ions　are　usually　in　powder　form,　with　low　recovery　during　regeneration.　Herein,　to　address　these　issues,　Fe3O4@La-Zr-MOFs　magnetic　composites　for　phosphate　and　fluoride　removal　were　fabricated　by　means　of　the　hydrothermal　method.　The　adsorption　properties　of　the　adsorbent　were　systematically　assessed　by　means　of　adsorption　experiments.　The　magnetic　Fe3O4@La-Zr-MOFs　exhibited　a　magnetic　recovery　efficiency　of　93%,　and　they　could　maintain　outstanding　adsorption　performance　at　a　broad　range　of　pH　values　and　superior　selectivity　for　phosphate　and　fluoride　ions.　The　adsorption　process　conformed　to　the　Langmuir　isotherm　and　pseudo-second-order　models,　indicating　that　it　was　dominated　by　monomolecular　chemisorption.　Further　characterization　of　the　Fe3O4@La-Zr-MOFs　before　and　after　adsorption　and　kinetic　thermodynamic　investigation　revealed　that　the　elimination　mechanism　of　phosphate　and　fluoride　ions　by　Fe3O4@La-Zr-MOFs　includes　ion　exchange,　electrostatic　interactions,　and　surface　complexation.　This　study　demonstrates　that　magnetic　reusable　Fe3O4@La-Zr-MOFs　composites　have　great　promise　for　phosphate　and　fluoride　removal　and　recovery.