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author:

You, K. (You, K..) [1] | Lin, J. (Lin, J..) [2] | Wang, Z. (Wang, Z..) [3] | Jiang, Y. (Jiang, Y..) [4] | Sun, J. (Sun, J..) [5] | Lin, Q. (Lin, Q..) [6] | Hu, X. (Hu, X..) [7] | Fu, H. (Fu, H..) [8] | Guo, X. (Guo, X..) [9] | Zhao, Y. (Zhao, Y..) [10] | Lin, L. (Lin, L..) [11] | Liu, Y. (Liu, Y..) [12] | Li, F. (Li, F..) [13]

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Scopus

Abstract:

Anticounterfeiting technologies meet challenges in the Internet of Things era due to the rapidly growing volume of objects, their frequent connection with humans, and the accelerated advance of counterfeiting/cracking techniques. Here, we, inspired by biological fingerprints, present a simple anticounterfeiting system based on perovskite quantum dot (PQD) fingerprint physical unclonable function (FPUF) by cooperatively utilizing the spontaneous-phase separation of polymers and selective in situ synthesis PQDs as an entropy source. The FPUFs offer red, green, and blue full-color fingerprint identifiers and random three-dimensional (3D) morphology, which extends binary to multivalued encoding by tuning the perovskite and polymer components, enabling a high encoding capacity (about 108570000, far surpassing that of biometric fingerprints). The strategy is compatible with mainstream production techniques that are widely used in traditional low-cost printed anticounterfeiting labels including spray printing, stamping, writing, and laser printing, avoiding complicated fabrication. Macrographical patterns and micro/nanofingerprint patterns with multiscale-tailorable inter-ridge sizes can be fused into a single FPUF label, satisfying different levels of anticounterfeiting requirements. Furthermore, a smart fused scheme of enhanced deep learning and fingerprint characteristic comparison is leveraged, by which high-efficiency, high-accuracy authentication of our FPUFs is achieved even for the increasingly huge FPUF databases and imperfectly captured images from users. © 2025 American Chemical Society.

Keyword:

anticounterfeiting labels biomimetic fingerprint perovskite quantum dot physical unclonable function smart authentication system

Community:

  • [ 1 ] [You K.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 2 ] [Lin J.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 3 ] [Wang Z.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 4 ] [Jiang Y.]Key Laboratory of Optoelectronic Science and Technology for Medicine of Ministry of Education, Fujian Provincial Key Laboratory of Photonics Technology, Fujian Normal University, Fuzhou, 350007, China
  • [ 5 ] [Sun J.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 6 ] [Lin Q.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 7 ] [Hu X.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 8 ] [Fu H.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 9 ] [Guo X.]Key Laboratory of Optoelectronic Science and Technology for Medicine of Ministry of Education, Fujian Provincial Key Laboratory of Photonics Technology, Fujian Normal University, Fuzhou, 350007, China
  • [ 10 ] [Zhao Y.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 11 ] [Lin L.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 12 ] [Liu Y.]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou, 350117, China
  • [ 13 ] [Li F.]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou, 350116, China

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Source :

ACS Applied Materials and Interfaces

ISSN: 1944-8244

Year: 2025

Issue: 3

Volume: 17

Page: 5254-5267

8 . 5 0 0

JCR@2023

CAS Journal Grade:2

Cited Count:

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SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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