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author:

Li, Li (Li, Li.) [1] | Pan, Lili (Pan, Lili.) [2] | Wang, Jiahui (Wang, Jiahui.) [3] | Zheng, Xiuzhen (Zheng, Xiuzhen.) [4] | Kuang, Kaixuan (Kuang, Kaixuan.) [5] | Zhang, Sujuan (Zhang, Sujuan.) [6] | Chen, Shifu (Chen, Shifu.) [7]

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EI

Abstract:

Improving catalytic performance by controlling the microstructure of materials has become a hot topic in the field of photocatalysis, such as the surface defect site, multistage layered morphology, and exposed crystal surface. Due to the differences in the metal atomic radius (Mn and Cd) and solubility product constant (MnS and CdS), Mn defect easily occurred in the S/Mn0.4Cd0.6S (S/0.4MCS) composite. To optimize the photocatalytic performance in N2 fixation, the effects of the synthesis conditions and reaction conditions for S/0.4MCS were explored and systematically studied. Combined with the experimental characterization and theoretical calculation, not only the photocatalytic reaction pathway but also the key steps of N2 reduction were explored. Moreover, the transfer mechanism of photogenerated charge carriers (PCCs) formed between S and 0.4MCS was studied, which enhanced the utilization rate of photogenerated electrons (e-) and holes (h+). This work detailedly discusses the relationship between microstructure and photocatalytic performance, which is beneficial for the design of efficient photocatalyst. © 2025 American Chemical Society.

Keyword:

Cadmium alloys Cadmium sulfide Crystal defects Layered semiconductors Manganese compounds Photocatalytic activity Rate constants Selenium compounds

Community:

  • [ 1 ] [Li, Li]Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 2 ] [Pan, Lili]Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 3 ] [Wang, Jiahui]Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 4 ] [Zheng, Xiuzhen]Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 5 ] [Zheng, Xiuzhen]State Key Laboratory of Photocatalysis on Energy and Environment, Fuzhou University, Fuzhou; 350116, China
  • [ 6 ] [Zheng, Xiuzhen]Anhui Provincial Key Laboratory of Synthetic Chemistry and Applications, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 7 ] [Kuang, Kaixuan]Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 8 ] [Zhang, Sujuan]Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 9 ] [Chen, Shifu]Key Laboratory of Green and Precise Synthetic Chemistry and Applications, Ministry of Education, Huaibei Normal University, Anhui, Huaibei; 235000, China
  • [ 10 ] [Chen, Shifu]Anhui Provincial Key Laboratory of Synthetic Chemistry and Applications, Huaibei Normal University, Anhui, Huaibei; 235000, China

Reprint 's Address:

  • [zheng, xiuzhen]key laboratory of green and precise synthetic chemistry and applications, ministry of education, huaibei normal university, anhui, huaibei; 235000, china;;[zheng, xiuzhen]state key laboratory of photocatalysis on energy and environment, fuzhou university, fuzhou; 350116, china;;[zheng, xiuzhen]anhui provincial key laboratory of synthetic chemistry and applications, huaibei normal university, anhui, huaibei; 235000, china;;

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Source :

Inorganic Chemistry

ISSN: 0020-1669

Year: 2025

Issue: 3

Volume: 64

Page: 1476-1487

4 . 3 0 0

JCR@2023

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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