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author:

You, Kejia (You, Kejia.) [1] | Lin, Jiasong (Lin, Jiasong.) [2] | Wang, Zhen (Wang, Zhen.) [3] | Jiang, Yi (Jiang, Yi.) [4] | Sun, Jiayu (Sun, Jiayu.) [5] | Lin, Qinghong (Lin, Qinghong.) [6] | Hu, Xin (Hu, Xin.) [7] | Fu, Hongyang (Fu, Hongyang.) [8] | Guo, Xuan (Guo, Xuan.) [9] | Zhao, Yi (Zhao, Yi.) [10] | Lin, Liangxu (Lin, Liangxu.) [11] | Liu, Yang (Liu, Yang.) [12] | Li, Fushan (Li, Fushan.) [13]

Indexed by:

EI

Abstract:

Anticounterfeiting technologies meet challenges in the Internet of Things era due to the rapidly growing volume of objects, their frequent connection with humans, and the accelerated advance of counterfeiting/cracking techniques. Here, we, inspired by biological fingerprints, present a simple anticounterfeiting system based on perovskite quantum dot (PQD) fingerprint physical unclonable function (FPUF) by cooperatively utilizing the spontaneous-phase separation of polymers and selective in situ synthesis PQDs as an entropy source. The FPUFs offer red, green, and blue full-color fingerprint identifiers and random three-dimensional (3D) morphology, which extends binary to multivalued encoding by tuning the perovskite and polymer components, enabling a high encoding capacity (about 108570000, far surpassing that of biometric fingerprints). The strategy is compatible with mainstream production techniques that are widely used in traditional low-cost printed anticounterfeiting labels including spray printing, stamping, writing, and laser printing, avoiding complicated fabrication. Macrographical patterns and micro/nanofingerprint patterns with multiscale-tailorable inter-ridge sizes can be fused into a single FPUF label, satisfying different levels of anticounterfeiting requirements. Furthermore, a smart fused scheme of enhanced deep learning and fingerprint characteristic comparison is leveraged, by which high-efficiency, high-accuracy authentication of our FPUFs is achieved even for the increasingly huge FPUF databases and imperfectly captured images from users. © 2025 American Chemical Society.

Keyword:

Authentication Elastomers Graphene quantum dots Ionomers Layered manufacturing Palmprint recognition

Community:

  • [ 1 ] [You, Kejia]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 2 ] [Lin, Jiasong]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 3 ] [Wang, Zhen]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 4 ] [Jiang, Yi]Key Laboratory of Optoelectronic Science and Technology for Medicine of Ministry of Education, Fujian Provincial Key Laboratory of Photonics Technology, Fujian Normal University, Fuzhou; 350007, China
  • [ 5 ] [Sun, Jiayu]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 6 ] [Lin, Qinghong]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 7 ] [Hu, Xin]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 8 ] [Fu, Hongyang]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 9 ] [Guo, Xuan]Key Laboratory of Optoelectronic Science and Technology for Medicine of Ministry of Education, Fujian Provincial Key Laboratory of Photonics Technology, Fujian Normal University, Fuzhou; 350007, China
  • [ 10 ] [Zhao, Yi]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 11 ] [Lin, Liangxu]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 12 ] [Liu, Yang]Strait Institute of Flexible Electronics (SIFE, Future Technologies), Fujian Key Laboratory of Flexible Electronics, Fujian Normal University and Strait Laboratory of Flexible Electronics (SLoFE), Fuzhou; 350117, China
  • [ 13 ] [Li, Fushan]Institute of Optoelectronic Technology, Fuzhou University, Fuzhou; 350116, China

Reprint 's Address:

  • [liu, yang]strait institute of flexible electronics (sife, future technologies), fujian key laboratory of flexible electronics, fujian normal university and strait laboratory of flexible electronics (slofe), fuzhou; 350117, china;;

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Source :

ACS Applied Materials and Interfaces

ISSN: 1944-8244

Year: 2025

Issue: 3

Volume: 17

Page: 5254-5267

8 . 5 0 0

JCR@2023

CAS Journal Grade:2

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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