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[期刊论文]

Tough and elastic hydrogel thermocells for heat energy utilization

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author:

Lyu, Xiaolin (Lyu, Xiaolin.) [1] (Scholars:吕晓林) | Lin, Ziqing (Lin, Ziqing.) [2] | Huang, Chunzhi (Huang, Chunzhi.) [3] | Unfold

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EI Scopus SCIE

Abstract:

Hydrogel thermocells possess great potential in the energy conversion field as they directly absorb waste heat from the environment to drive redox reactions for continuous electricity generation. However, achieving high toughness and good elasticity simultaneously in hydrogel thermocells remains a challenge because of the inherent contradiction of energy dissipation mechanisms, severely limiting their practical applications and lifespan. To address this, a skin-like hydrogel network with a highly dense interwoven network is developed to construct hydrogel thermocells with good elasticity and high toughness. The dense network structure can effectively disperse the stress and hinder crack propagation, thus breaking the contradiction between high toughness and good elasticity. The thermocell realizes a toughness of 460 J m- 2 while reaching an elastic limit strain of 350 %, far exceeding the elasticity of previous stretchable hydrogel thermocells. Meanwhile, it exhibits ultra-low hysteresis and excellent fatigue resistance under tensile and compressive cyclic loads. Moreover, the thermocell can work stably over long periods, enabling stable voltage output even under compression, bending, and stretching. In addition, the thermocell can power the LED lamp and calculator, and can also be connected in series to form large arrays, thus rendering it an ideal power source for wearable devices.

Keyword:

Heat energy utilization Thermocell Thermoelectric conversion Thermogalvanic Wearable device

Community:

  • [ 1 ] [Lyu, Xiaolin]Fuzhou Univ, Coll Mat Sci & Engn, Key Lab Adv Mat Technol, Int HongKong Macao & Taiwan Joint Lab Adv Mat Tech, Fuzhou 350108, Fujian, Peoples R China
  • [ 2 ] [Lin, Ziqing]Fuzhou Univ, Coll Mat Sci & Engn, Key Lab Adv Mat Technol, Int HongKong Macao & Taiwan Joint Lab Adv Mat Tech, Fuzhou 350108, Fujian, Peoples R China
  • [ 3 ] [Huang, Chunzhi]Fuzhou Univ, Coll Mat Sci & Engn, Key Lab Adv Mat Technol, Int HongKong Macao & Taiwan Joint Lab Adv Mat Tech, Fuzhou 350108, Fujian, Peoples R China
  • [ 4 ] [Zhang, Xinyue]Fuzhou Univ, Coll Mat Sci & Engn, Key Lab Adv Mat Technol, Int HongKong Macao & Taiwan Joint Lab Adv Mat Tech, Fuzhou 350108, Fujian, Peoples R China
  • [ 5 ] [Luo, Zhong-Zhen]Fuzhou Univ, Coll Mat Sci & Engn, Key Lab Adv Mat Technol, Int HongKong Macao & Taiwan Joint Lab Adv Mat Tech, Fuzhou 350108, Fujian, Peoples R China
  • [ 6 ] [Zou, Zhigang]Fuzhou Univ, Coll Mat Sci & Engn, Key Lab Adv Mat Technol, Int HongKong Macao & Taiwan Joint Lab Adv Mat Tech, Fuzhou 350108, Fujian, Peoples R China
  • [ 7 ] [Zhou, Piaopiao]Fujian Med Univ, Union Hosp, Dept Crit Care Med, Fuzhou 350108, Fujian, Peoples R China
  • [ 8 ] [Lyu, Xiaolin]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
  • [ 9 ] [Luo, Zhong-Zhen]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
  • [ 10 ] [Zou, Zhigang]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China
  • [ 11 ] [Lu, Yang]Tech Univ Dresden, Ctr Adv Elect Dresden, D-01067 Dresden, Germany
  • [ 12 ] [Zou, Zhigang]Nanjing Univ, Coll Engn & Appl Sci, Ecomat & Renewable Energy Res Ctr, Nanjing 210093, Peoples R China

Reprint 's Address:

  • [Luo, Zhong-Zhen]Fuzhou Univ, Coll Mat Sci & Engn, Key Lab Adv Mat Technol, Int HongKong Macao & Taiwan Joint Lab Adv Mat Tech, Fuzhou 350108, Fujian, Peoples R China;;[Zhou, Piaopiao]Fujian Med Univ, Union Hosp, Dept Crit Care Med, Fuzhou 350108, Fujian, Peoples R China;;[Luo, Zhong-Zhen]Fujian Sci & Technol Innovat Lab Optoelect Informa, Fuzhou 350108, Fujian, Peoples R China;;[Lu, Yang]Tech Univ Dresden, Ctr Adv Elect Dresden, D-01067 Dresden, Germany;;

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Source :

CHEMICAL ENGINEERING JOURNAL

ISSN: 1385-8947

Year: 2024

Volume: 493

1 3 . 4 0 0

JCR@2023

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count:

30 Days PV: 0

Online/Total:177/10268796
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