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author:

Xu, Yuhui (Xu, Yuhui.) [1] | Zhang, Gaini (Zhang, Gaini.) [2] | Wang, Xiaoxue (Wang, Xiaoxue.) [3] | Li, Xiangyang (Li, Xiangyang.) [4] | Zhang, Jianhua (Zhang, Jianhua.) [5] | Wu, Xinyue (Wu, Xinyue.) [6] | Yuan, Yitong (Yuan, Yitong.) [7] | Xi, Yukun (Xi, Yukun.) [8] | Yang, Xuan (Yang, Xuan.) [9] | Li, Ming (Li, Ming.) [10] | Pu, Xiaohua (Pu, Xiaohua.) [11] | Cao, Guiqiang (Cao, Guiqiang.) [12] | Yang, Zihao (Yang, Zihao.) [13] | Sun, Bo (Sun, Bo.) [14] | Wang, Jingjing (Wang, Jingjing.) [15] | Yang, Huijuan (Yang, Huijuan.) [16] | Li, Wenbin (Li, Wenbin.) [17] | Zhang, Jiujun (Zhang, Jiujun.) [18] (Scholars:张久俊) | Li, Xifei (Li, Xifei.) [19]

Indexed by:

EI Scopus SCIE

Abstract:

Birnessite-type MnO 2 ( 6- MnO 2 ) exhibits great potential as a cathode material for aqueous zinc-ion batteries (AZIBs). However, the structural instability and sluggish reaction kinetics restrict its further application. Herein, a unique protons intercalation strategy was utilized to simultaneously modify the interlayer environment and transition metal layers of 6- MnO 2 . The intercalated protons directly form strong O - H bonds with the adjacent oxygens, while the increased H 2 O molecules also establish a hydrogen bond network (O - H & sdot;& sdot;& sdot; O) between H 2 O molecules or bond with adjacent oxygens. Based on the Grotthuss mechanism, these bondings ultimately enhance the stability of layered structures and facilitate the rapid diffusion of protons. Moreover, the introduction of protons induces numerous oxygen vacancies, reduces steric hindrance, and accelerates ion transport kinetics. Consequently, the protons intercalated 8- MnO 2 (H-MnO 2-x ) demonstrates exceptional specific capacity of 401.7 mAh/g at 0.1 A/g and a fast-charging performance over 1000 cycles. Density functional theory analysis confirms the improved electronic conductivity and reduced diffusion energy barrier. Most importantly, electrochemical quartz crystal microbalance tests combining with ex-situ characterizations verify the inhibitory effect of the interlayer proton environment on basic zinc sulfate formation. Protons intercalation behavior provides a promising avenue for the development of MnO 2 as well as other cathodes in AZIBs.

Keyword:

delta-MnO2 cathodes EQCM Protons Transport kinetics Zinc storage mechanism

Community:

  • [ 1 ] [Xu, Yuhui]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 2 ] [Zhang, Gaini]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 3 ] [Wang, Xiaoxue]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 4 ] [Zhang, Jianhua]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 5 ] [Wu, Xinyue]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 6 ] [Yuan, Yitong]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 7 ] [Xi, Yukun]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 8 ] [Yang, Xuan]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 9 ] [Li, Ming]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 10 ] [Pu, Xiaohua]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 11 ] [Cao, Guiqiang]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 12 ] [Yang, Zihao]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 13 ] [Sun, Bo]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 14 ] [Wang, Jingjing]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 15 ] [Yang, Huijuan]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 16 ] [Li, Wenbin]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 17 ] [Li, Xifei]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China
  • [ 18 ] [Xu, Yuhui]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 19 ] [Zhang, Gaini]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 20 ] [Wang, Xiaoxue]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 21 ] [Zhang, Jianhua]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 22 ] [Wu, Xinyue]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 23 ] [Yuan, Yitong]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 24 ] [Xi, Yukun]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 25 ] [Yang, Xuan]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 26 ] [Li, Ming]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 27 ] [Pu, Xiaohua]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 28 ] [Cao, Guiqiang]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 29 ] [Yang, Zihao]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 30 ] [Sun, Bo]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 31 ] [Wang, Jingjing]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 32 ] [Yang, Huijuan]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 33 ] [Li, Wenbin]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 34 ] [Li, Xifei]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China
  • [ 35 ] [Li, Xiangyang]Xian Inst Electromech Informat Technol, Sci & Technol Electromech Dynam Control Lab, Xian 710065, Peoples R China
  • [ 36 ] [Zhang, Jiujun]Fuzhou Univ, Coll Mat Sci & Engn, Fuzhou 350108, Fujian, Peoples R China
  • [ 37 ] [Li, Xifei]Guangdong Yuanneng Technol Co Ltd, Foshan 528223, Guangdong, Peoples R China
  • [ 38 ] [Li, Xifei]Qinghai Minzu Univ, Qinghai Prov Key Lab Nanomat & Nanotechnol, Xining 810007, Peoples R China

Reprint 's Address:

  • [Zhang, Gaini]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China;;[Li, Xifei]Xian Univ Technol, Inst Adv Electrochem Energy, Shaanxi Int Joint Res Ctr Surface Technol Energy S, Xian 710048, Shaanxi, Peoples R China;;[Zhang, Gaini]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China;;[Li, Xifei]Xian Univ Technol, Sch Mat Sci & Engn, Xian 710048, Shaanxi, Peoples R China;;[Li, Xiangyang]Xian Inst Electromech Informat Technol, Sci & Technol Electromech Dynam Control Lab, Xian 710065, Peoples R China;;

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Source :

JOURNAL OF COLLOID AND INTERFACE SCIENCE

ISSN: 0021-9797

Year: 2024

Volume: 675

Page: 1-13

9 . 4 0 0

JCR@2023

Cited Count:

WoS CC Cited Count: 3

SCOPUS Cited Count: 5

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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