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author:

Lin, Xi (Lin, Xi.) [1] | Liu, Runyu (Liu, Runyu.) [2] | Nie, Wenfeng (Nie, Wenfeng.) [3] | Tian, Feng (Tian, Feng.) [4] | Liu, Xinzhong (Liu, Xinzhong.) [5]

Indexed by:

EI Scopus SCIE

Abstract:

Achieving efficient and stable photocatalytic degradation of xylene hinges on the advancement of photocatalytic materials with outstanding visible light activity. This low-carbon strategy serves as a promising solution to combat air pollution effectively. In this study, we synthesized a Z-scheme heterojunction Ag@CuO/UiO-66-NH2 nanocomposite by hydrothermal method to investigate its photodegradation properties for xylene gas under visible light conditions. XRD, XPS, SEM, FTIR, and UV-vis analyses were employed to confirm the presence of the Z-scheme heterojunction. The CuO/UiO-66-NH2 (CuU-2) composite has high photocatalytic activity, which is 2.37 times that of the original UiO-66-NH2. The incorporation of Z-scheme heterojunction facilitates efficient charge transfer and separation, leading to a substantial enhancement in photocatalytic activity. The Ag@CuO/UiO-66-NH2 (Ag-1@CuU) composite has the highest photocatalytic activity with a degradation efficiency of 84.12%, which is 3.36 times and 1.41 times that of UiO-66-NH2 and CuO/UiO-66-NH2, respectively. The silver cocatalyst improves the absorption capacity of the composite material to visible light, makes the ultraviolet visible absorption edge redshift, and significantly improves the photocatalytic performance. This study introduces a novel approach for xylene gas degradation and offers a versatile strategy for designing and synthesizing metal-organic framework (MOF)-based photocatalysts with exceptional performance.

Keyword:

Ag cocatalyst Gas treatment Heterojunction Metal-organic frameworks Photocatalytic degradation

Community:

  • [ 1 ] [Lin, Xi]Fuzhou Univ, Sch Environm & Safety Engn, Fuzhou 350100, Peoples R China
  • [ 2 ] [Liu, Runyu]Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300350, Peoples R China
  • [ 3 ] [Nie, Wenfeng]Fujian Univ Technol, Sch Ecol Environm & Urban Construct, Fuzhou 350100, Peoples R China
  • [ 4 ] [Liu, Xinzhong]Fujian Univ Technol, Sch Ecol Environm & Urban Construct, Fuzhou 350100, Peoples R China
  • [ 5 ] [Tian, Feng]Jiangnan Univ, Sch Chem & Mat Engn, Wuxi 214000, Jiangsu, Peoples R China

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Source :

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH

ISSN: 0944-1344

Year: 2023

Issue: 2

Volume: 31

Page: 2394-2407

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JCR@2023

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JCR@2023

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 2

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