Metal　organic　framework　(MOF)　as　a　template　strategy　to　get　dispersed　metal　particle　with　high　catalytic　activity　is　widely　used　in　the　design　of　electrodes　for　hydrogen　production.　Herein,　we　report　using　carbon　nanotube　(CNT)　as　a　multifunctional　active　binder　that　would　promote　the　growth　of　MOF　arrays　on　carbon　fiber　cloth　(CFC)　substrate　and　the　release　of　hydrogen.　By　modified　CFC　with　this　new　active　binder:　(1)　the　active　material　was　more　firmly　anchored　to　the　carbon　fiber;　(2)　the　overall　electron　transport　efficiency　was　improved;　and　(3)　the　MOF　precursor　grew　more　uniformly　on　the　carbon　fiber,　and　greatly　increased　the　number　of　active　sites.　Benefited　from　the　CNT　modification,　the　obtained　porous　array　with　CoP　nanoparticle　modification　(CFC-CNTCoOx/CoP)　catalyst　displayed　superior　alkaline　hydrogen　evolution　reaction　(HER)　performance　and　excellent　stability　with　an　overpotential　of　108　mV　at　the　current　density　of　10　mA　cm-2　and　a　small　Tafel　slope　of　60　mV　dec-1.　The　excellent　HER　performance　mainly　derived　from　the　structure　optimization　and　enhanced　electron　transfer　brought　by　the　active　binders.　In　addition,　Co(OH)2　appeared　in　the　long-time　HER　process　and　the　synergistic　interaction　of　CoOx,　CoP,　Co(OH)2　and　CNT　maintained　the　good　stability.