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author:

Wang, Ning (Wang, Ning.) [1] | Zhu, Guofeng (Zhu, Guofeng.) [2] | Hu, Zhiqiang (Hu, Zhiqiang.) [3] | Ju, Xuewei (Ju, Xuewei.) [4] | Su, Haobin (Su, Haobin.) [5] | Huang, Feng (Huang, Feng.) [6] | Chen, Qi (Chen, Qi.) [7] | Cao, Yiming (Cao, Yiming.) [8] | Wang, Xiangfeng (Wang, Xiangfeng.) [9]

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Abstract:

In this study, we utilized time-domain terahertz magneto-optical spectroscopy to investigate the spin resonance in a c-cut TmFeO3 single crystal at T = 1.6 K under different magnetic fields and characterized its intricate internal interactions. By selectively exciting the magnetic resonance modes in the crystal, we found that as the magnetic field increases, the quasi-ferromagnetic (q-FM) mode of TmFeO3 single crystal shifts towards higher frequencies, while the quasi-antiferromagnetic (q-AFM) mode transforms into the q-FM mode at low critical magnetic fields (2.2–3.6 T). Through magnetic structure analysis and theoretical calculations, it is confirmed that the magnetic moment of TmFeO3 undergoes a magnetic-field-induced spin reorientation from Γ2 to Γ4 phase. Materials with magnetic moment flipping at low magnetic fields may find applications for antiferromagnetic spintronic devices in the future. © 2023 Elsevier B.V.

Keyword:

Antiferromagnetism Dichroism Electron spin resonance spectroscopy Iron compounds Magnetic fields Magnetic moments Magnetic resonance Single crystals Terahertz spectroscopy Thulium compounds

Community:

  • [ 1 ] [Wang, Ning]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou; 350108, China
  • [ 2 ] [Zhu, Guofeng]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou; 350108, China
  • [ 3 ] [Hu, Zhiqiang]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou; 350108, China
  • [ 4 ] [Ju, Xuewei]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou; 350108, China
  • [ 5 ] [Ju, Xuewei]The Engineering Research Center for CAD/CAM of Fujian Universities, Putian University, Putian; 351100, China
  • [ 6 ] [Ju, Xuewei]Engineering Research Center of Smart Distribution Grid Equipment, Fujian Province University, Fuzhou; 350108, China
  • [ 7 ] [Su, Haobin]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou; 350108, China
  • [ 8 ] [Huang, Feng]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou; 350108, China
  • [ 9 ] [Chen, Qi]School of Physics and Electronic Engineering, Qujing Normal University, Qujing; 655011, China
  • [ 10 ] [Cao, Yiming]School of Physics and Electronic Engineering, Qujing Normal University, Qujing; 655011, China
  • [ 11 ] [Wang, Xiangfeng]School of Mechanical Engineering and Automation, Fuzhou University, Fuzhou; 350108, China

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Source :

Infrared Physics and Technology

ISSN: 1350-4495

Year: 2023

Volume: 135

3 . 1

JCR@2023

3 . 1 0 0

JCR@2023

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count:

SCOPUS Cited Count:

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 3

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