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author：

Liu, Minghui (Liu, Minghui.) [1] | Zhang, Guigang (Zhang, Guigang.) [2] | Liang, Xiaocong (Liang, Xiaocong.) [3] | Pan, Zhiming (Pan, Zhiming.) [4] | Zheng, Dandan (Zheng, Dandan.) [5] | Wang, Sibo (Wang, Sibo.) [6] | Yu, Zhiyang (Yu, Zhiyang.) [7] | Hou, Yidong (Hou, Yidong.) [8] | Wang, Xinchen (Wang, Xinchen.) [9]

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EI

Abstract：

In　situ　photo-deposition　of　both　Pt　and　CoOx　cocatalysts　on　the　facets　of　poly　(triazine　imide)　(PTI)　crystals　has　been　developed　for　photocatalytic　overall　water　splitting.　However,　the　undesired　backward　reaction　(i.e.,　water　formation)　on　the　noble　Pt　surface　is　a　spontaneously　down-hill　process,　which　restricts　their　efficiency　to　run　the　overall　water　splitting　reaction.　Herein,　we　demonstrate　that　the　efficiency　for　photocatalytic　overall　water　splitting　could　be　largely　promoted　by　the　decoration　of　Rh/Cr2O3　and　CoOx　as　H2　and　O2　evolution　cocatalysts,　respectively.　Results　reveal　that　the　dual　cocatalysts　greatly　extract　charges　from　bulk　to　surface,　while　the　Rh/Cr2O3　cocatalyst　dramatically　restrains　the　backward　reaction,　achieving　an　apparent　quantum　efficiency　(AQE)　of　20.2　%　for　the　photocatalytic　overall　water　splitting　reaction.　©　2023　Wiley-VCH　GmbH.

Keyword：

Chromium compounds Crystals Efficiency Platinum Platinum compounds Rhodium compounds

Community：

  • [ 1 ] [Liu, Minghui]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 2 ] [Zhang, Guigang]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 3 ] [Liang, Xiaocong]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 4 ] [Pan, Zhiming]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 5 ] [Zheng, Dandan]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 6 ] [Wang, Sibo]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 7 ] [Yu, Zhiyang]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 8 ] [Hou, Yidong]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 9 ] [Wang, Xinchen]State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China

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Source ：

Angewandte Chemie - International Edition

ISSN： 1433-7851

Year： 2023

Issue： 37

Volume： 62

1 6 . 1

JCR@2023

1 6 . 1 0 0

JCR@2023

JCR Journal Grade：1

CAS Journal Grade：1

Cited Count：

WoS CC Cited Count：

SCOPUS Cited Count： 104

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 1

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