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author:

Yan, Zhen (Yan, Zhen.) [1] | Ding, Yulin (Ding, Yulin.) [2] | Huang, Meirong (Huang, Meirong.) [3] | Li, Junfeng (Li, Junfeng.) [4] | Han, Qinxue (Han, Qinxue.) [5] | Yang, Meiqi (Yang, Meiqi.) [6] | Li, Wenmu (Li, Wenmu.) [7]

Indexed by:

EI

Abstract:

It is a considerable challenge to develop a composite material with ultra-light and high electromagnetic interference (EMI) shielding efficiency for the next generation of electronic equipment. MXenes have received extensive attention in composite aerogel EMI shielding due to their abundant surface groups and ultra-high conductivity. However, the poor mechanical properties make them difficult to apply on a large scale. Here, we demonstrate a simple method to construct ultra-light conductive Ti3C2Tx MXene/aramid nanofibers (ANFs)/carbon nanotubes (CNTs) aerogels with a 'sandwich' structure. CNTs and MXene absorb and reflect electromagnetic waves, while ANF aerogel provides good mechanical strength. Our composite aerogels with an extra-high EMI shielding efficiency of up to 69.0 dB at the X-band, despite their thickness and density being only 2 mm and 0.0428 g/cm3, respectively. At the same time, the composite aerogel with a low 0.0488 W/(m·K) thermal conductivity shows extraordinary flame resistance, heat preservation, and insulation ability. Besides, MXene/ANFs/CNTs aerogel can reach 104 °C in 3 s under an 8 V voltage and shows long-term Joule heating stability. This work provides a forward-looking idea for building multifunctional EMI shielding materials. The obtained aerogels have potential applications in aerospace, portable electronic devices, and defense industries. © 2023 American Chemical Society.

Keyword:

Aerogels Carbon nanotubes Efficiency Electromagnetic pulse Electromagnetic shielding Electromagnetic wave interference Flame resistance Heat resistance Signal interference Thermal conductivity Thermal insulation

Community:

  • [ 1 ] [Yan, Zhen]College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 2 ] [Yan, Zhen]Key Laboratory of Optoelectronic Materials Chemistry and Physics, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350108, China
  • [ 3 ] [Ding, Yulin]Key Laboratory of Optoelectronic Materials Chemistry and Physics, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350108, China
  • [ 4 ] [Huang, Meirong]College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 5 ] [Huang, Meirong]Key Laboratory of Optoelectronic Materials Chemistry and Physics, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350108, China
  • [ 6 ] [Li, Junfeng]Key Laboratory of Optoelectronic Materials Chemistry and Physics, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350108, China
  • [ 7 ] [Han, Qinxue]College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 8 ] [Han, Qinxue]Key Laboratory of Optoelectronic Materials Chemistry and Physics, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350108, China
  • [ 9 ] [Yang, Meiqi]Key Laboratory of Optoelectronic Materials Chemistry and Physics, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350108, China
  • [ 10 ] [Li, Wenmu]Key Laboratory of Optoelectronic Materials Chemistry and Physics, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou; 350108, China

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Source :

ACS Applied Nano Materials

ISSN: 2574-0970

Year: 2023

Issue: 7

Volume: 6

Page: 6141-6150

5 . 3

JCR@2023

5 . 3 0 0

JCR@2023

ESI HC Threshold:49

JCR Journal Grade:2

CAS Journal Grade:3

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 13

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 1

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