Development of soluble UiO-66 to improve photocatalytic CO2 reduction - Details

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The　conversion　of　CO2　to　valuable　chemicals　by　photocatalysis　has　attracted　widespread　interesting.　Owing　to　the　linear　structure　of　CO2　molecule　with　strong　C[dbnd]O　bond,　the　surface　reaction　is　considered　as　one　of　the　main　issues　to　restrict　the　conversion　efficiency.　Herein,　soluble　UiO-66　has　been　developed　as　co-catalyst　to　enhance　the　photocatalytic　performance　for　CO2　reduction.　The　soluble　UiO-66　has　presented　the　performance　ca.　1.5　higher　than　the　insoluble　version,　yielding　30.6　µmol/h　for　CO2　to　CO　conversion　by　using　5.0　mg　sample.　This　improvement　can　be　attributed　to　the　preserved　framework　by　soluble　UiO-66.　Therefore,　the　chemisorption　of　CO2　molecules　can　be　improved,　boosting　the　reduction　reaction　for　CO　production.　This　research　provides　a　new　path　for　a　rational　design　of　metal-organic　framework　(MOF)　for　photoredox　catalysis,　meanwhile　inspiring　advanced　application　of　MOF　catalysis　with　the　soluble　manner.　©　2022　Elsevier　B.V.

Keyword：

Carbon dioxide Metal-Organic Frameworks Molecules Photocatalytic activity Surface reactions

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[ 1 ] [Tan, Li]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
[ 2 ] [Li, Yanru]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
[ 3 ] [Lv, Qian]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
[ 4 ] [Gan, Yuyan]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
[ 5 ] [Fang, Yuan]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
[ 6 ] [Tang, Yu]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
[ 7 ] [Wu, Lizhi]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China
[ 8 ] [Fang, Yuanxing]Institute of Molecular Catalysis and In Situ/Operando Studies, State Key Laboratory of Photocatalysis on Energy and Environment, College of Chemistry, Fuzhou University, Fuzhou; 350108, China

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Source ：

Catalysis Today

ISSN： 0920-5861

Year： 2023

Volume： 410

Page： 282-288

5 . 2

JCR@2023

5 . 2 0 0

JCR@2023

ESI HC Threshold：39

JCR Journal Grade：1

CAS Journal Grade：2

Cited Count：

WoS CC Cited Count： 0

SCOPUS Cited Count： 23

ESI Highly Cited Papers on the List： 0 Unfold All

WanFang Cited Count：

Chinese Cited Count：

30 Days PV： 7

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