• Complex
  • Title
  • Keyword
  • Abstract
  • Scholars
  • Journal
  • ISSN
  • Conference
成果搜索

author:

Liao, Wanru (Liao, Wanru.) [1] | Lu, Suwei (Lu, Suwei.) [2] | Chen, Weihang (Chen, Weihang.) [3] | Zhu, Shuying (Zhu, Shuying.) [4] | Xia, Yuzhou (Xia, Yuzhou.) [5] | Yang, Min-Quan (Yang, Min-Quan.) [6] | Liang, Shijing (Liang, Shijing.) [7]

Indexed by:

EI Scopus CSCD

Abstract:

Dye-sensitized photocatalysis has been extensively studied for photocatalytic solar energy conversion due to the advantage in capturing long-wavelength photons with a high absorption coefficient. The rational integration of photosensitizer with semiconductor and cocatalyst to collaboratively operate in one system is highly desired. Here, we fabricate a Ni(OH)2-loaded titanate nanosheet (Ni(OH)2/H2Ti6O13) composite for high-performance dye-sensitized photocatalytic CO2 reduction. The ultrathin H2Ti6O13 nanosheets with negative surface charge provide an excellent support to anchor the dye photosensitizer, while the loaded Ni(OH)2 serves as an adsorbent of CO2 and electron sink of photoelectrons. As such, the photoelectrons derived from the [Ru(bpy)3]Cl2 sensitizer can be targeted transfer to the Ni(OH)2 active sites via the H2Ti6O13 nanosheets linker. A high CO production rate of 1801 μmol g-1 h-1 is obtained over the optimal Ni(OH)2/H2Ti6O13, while the pure H2Ti6O13 shows significantly lower CO2 reduction performance. The work is anticipated to trigger more research attention on the rational design and synthesis of earth-abundant transition metal-based cocatalysts decorated on ultrathin 2D platforms for artificially photocatalytic CO2 reduction. © 2021 Institute of Process Engineering, Chinese Academy of Sciences.

Keyword:

Community:

  • [ 1 ] [Liao, Wanru]National Engineering Research Center of Chemical Fertilizer Catalyst, Fuzhou University, Fuzhou; 350002, China
  • [ 2 ] [Lu, Suwei]College of Environmental Science and Engineering, Fujian Key Laboratory of Pollution Control & Resource Reuse, Fujian Normal University, Fuzhou; 350007, China
  • [ 3 ] [Chen, Weihang]National Engineering Research Center of Chemical Fertilizer Catalyst, Fuzhou University, Fuzhou; 350002, China
  • [ 4 ] [Zhu, Shuying]College of Chemistry, Fuzhou University, Fuzhou; 350108, China
  • [ 5 ] [Xia, Yuzhou]Province University Key Laboratory of Green Energy and Environment Catalysis, Ningde Normal University, Ningde; 352100, China
  • [ 6 ] [Yang, Min-Quan]College of Environmental Science and Engineering, Fujian Key Laboratory of Pollution Control & Resource Reuse, Fujian Normal University, Fuzhou; 350007, China
  • [ 7 ] [Liang, Shijing]National Engineering Research Center of Chemical Fertilizer Catalyst, Fuzhou University, Fuzhou; 350002, China

Reprint 's Address:

Email:

Show more details

Related Keywords:

Related Article:

Source :

Green Chemical Engineering

ISSN: 2096-9147

Year: 2022

Issue: 3

Volume: 3

Page: 240-249

9 . 1 0 0

JCR@2023

Cited Count:

WoS CC Cited Count: 0

SCOPUS Cited Count: 15

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

Affiliated Colleges:

Online/Total:38/10101028
Address:FZU Library(No.2 Xuyuan Road, Fuzhou, Fujian, PRC Post Code:350116) Contact Us:0591-22865326
Copyright:FZU Library Technical Support:Beijing Aegean Software Co., Ltd. 闽ICP备05005463号-1