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Abstract:
Solid oxide electrolysis cells (SOECs) are regarded as promising candidates for the next generation of energy conversion device due to their extremely high conversion efficiency. However, the electrolysis current density should be further increased to meet the demands of large-scale industrial application in the future. Here, a novel anode configuration for SOEC is reported that achieves an ultra-high current density of 5.73 A cm(-2) for at least 4 h. To the best of the authors' knowledge, such current density surpasses the record of present state-of-the-art research. The unique stability under such high current density is attributed to the novel SOEC constructed with a La0.6Sr0.4CoO3-delta anode catalyst nano-layer to promote oxygen generation, vertically aligned micro channel anode scaffold to accelerate oxygen release, and integrated anode-electrolyte interface to improve the interfacial strength. The novel SOEC successfully demonstrates stable steam electrolysis under an ultra-high current density of 5.96 A cm(-2) at 800 degrees C under the constant operating voltage of 1.3 V, corresponding to a hydrogen production rate of 2.5 L h(-1) cm(-2).
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Source :
ADVANCED ENERGY MATERIALS
ISSN: 1614-6832
Year: 2022
Issue: 28
Volume: 12
2 7 . 8
JCR@2022
2 4 . 4 0 0
JCR@2023
ESI Discipline: MATERIALS SCIENCE;
ESI HC Threshold:91
JCR Journal Grade:1
CAS Journal Grade:1
Cited Count:
SCOPUS Cited Count: 30
ESI Highly Cited Papers on the List: 0 Unfold All
WanFang Cited Count:
Chinese Cited Count:
30 Days PV: 0
Affiliated Colleges: