Ultrasonic　rolling　processing　(URP)　can　strengthen　the　material　surface　layer　and　enhance　the　material　properties.　However,　the　surface　layer　of　work　hardening　induced　by　URP　behaves　like　a　hard　shell　that　can　restrict　further　strengthening　of　deeper　material.　The　URP　of　Ti　alloy　Ti5Al4Mo6V2Nb1Fe　strengthened　its　surface　layer　properties,　but　the　material　performance　did　not　improve　to　a　greater　extent.　In　this　study,　electric　pulse　aided　ultrasonic　rolling　processing　(EPAURP)　was　utilized　for　the　nanocrystallization　of　the　surface　layer　and　further　improvement　of　the　Ti5Al4Mo6V2Nb1Fe　properties　such　as　wear　resistance,　mechanical　properties,　and　fatigue　properties.　The　experimental　results　revealed　the　nanocrystallization　of　the　surface　layer　through　the　introduction　of　electric　pulse.　The　nanocrystallized　surface　layer　was　approximately　300　nm　thick,　and　the　size　of　the　nanocrystalline　was　about　30　nm.　In　addition,　the　EPAURP　induced　the　formation　of　a　serious　plastic　deformation　(SPD)　surface　layer,　with　thickness　greater　than　that　induced　by　the　URP.　The　EPAURP　reduced　the　defects　and　cracks　in　the　surface　and　improved　the　fretting　wear　resistance,　attributing　to　work-hardening　and　nanocrystallization.　The　tensile　properties　and　fatigue　properties　improved　after　EPAURP　owing　to　the　smooth　surface,　higher　compressive　residual　stress,　and　the　nanocrystallization.