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author:

Wan, Chao (Wan, Chao.) [1] | Zhou, Liu (Zhou, Liu.) [2] | Xu, Shuman (Xu, Shuman.) [3] | Jin, Biyu (Jin, Biyu.) [4] | Ge, Xin (Ge, Xin.) [5] | Qian, Xing (Qian, Xing.) [6] (Scholars:钱兴) | Xu, Lixin (Xu, Lixin.) [7] | Chen, Fengqiu (Chen, Fengqiu.) [8] | Zhan, Xiaoli (Zhan, Xiaoli.) [9] | Yang, Yongrong (Yang, Yongrong.) [10] | Cheng, Dang-guo (Cheng, Dang-guo.) [11]

Indexed by:

EI SCIE

Abstract:

Hydrogen energy, as an ideal renewable resource and green energy replacement, has attracted growing attention. However, constructing highly active and stable catalysts for hydrogen evolution from Formic acid (FA) is still a challenging issue for development of renewable hydrogen energy. Herein, we develop a facile defect engineering strategy to construct N-deficient ordered mesoporous graphitic carbon nitride coupled with AgPd nanoparticles (denoted as AgPd/N-ompg-C3N4). Impressively, the as-prepared Ag0.1Pd0.9/N-ompg-C3N4 catalyst exhibits remarkable activity with the Turnover frequency (TOF) value of 1588.2 h-1 and robust stability with only a slight decrease in activity after ten cycles. Such markedly enhanced catalytic performance of Ag0.1Pd0.9/N-ompgC3N4 is mainly attributed to the unique structure of N-ompg-C3N4 with higher surface area and abundant surface defects, the strong metal - support interaction between AgPd and N-ompg-C3N4, and charge transfer from Pd to Ag. This study provides a novel and efficient strategy for designing efficient catalysts to drive the hydrogen evolution from FA.

Keyword:

Defect engineering Formic acid Hydrogen evolution N-ompg-C3N4 Synergistic effect

Community:

  • [ 1 ] [Wan, Chao]Anhui Univ Technol, Anhui Prov Key Lab Coal Clean Convers & High Valu, Sch Chem & Chem Engn, Maanshan 243002, Peoples R China
  • [ 2 ] [Zhou, Liu]Anhui Univ Technol, Anhui Prov Key Lab Coal Clean Convers & High Valu, Sch Chem & Chem Engn, Maanshan 243002, Peoples R China
  • [ 3 ] [Jin, Biyu]Anhui Univ Technol, Anhui Prov Key Lab Coal Clean Convers & High Valu, Sch Chem & Chem Engn, Maanshan 243002, Peoples R China
  • [ 4 ] [Xu, Lixin]Anhui Univ Technol, Anhui Prov Key Lab Coal Clean Convers & High Valu, Sch Chem & Chem Engn, Maanshan 243002, Peoples R China
  • [ 5 ] [Wan, Chao]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China
  • [ 6 ] [Xu, Shuman]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China
  • [ 7 ] [Chen, Fengqiu]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China
  • [ 8 ] [Zhan, Xiaoli]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China
  • [ 9 ] [Yang, Yongrong]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China
  • [ 10 ] [Cheng, Dang-guo]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China
  • [ 11 ] [Wan, Chao]Inst Zhejiang Univ Quzhou, 78 Jiuhua Blvd North, Quzhou 324000, Peoples R China
  • [ 12 ] [Xu, Shuman]Inst Zhejiang Univ Quzhou, 78 Jiuhua Blvd North, Quzhou 324000, Peoples R China
  • [ 13 ] [Chen, Fengqiu]Inst Zhejiang Univ Quzhou, 78 Jiuhua Blvd North, Quzhou 324000, Peoples R China
  • [ 14 ] [Zhan, Xiaoli]Inst Zhejiang Univ Quzhou, 78 Jiuhua Blvd North, Quzhou 324000, Peoples R China
  • [ 15 ] [Yang, Yongrong]Inst Zhejiang Univ Quzhou, 78 Jiuhua Blvd North, Quzhou 324000, Peoples R China
  • [ 16 ] [Cheng, Dang-guo]Inst Zhejiang Univ Quzhou, 78 Jiuhua Blvd North, Quzhou 324000, Peoples R China
  • [ 17 ] [Ge, Xin]Jiangnan Univ, Sch Chem & Mat Engn, Wuxi 214122, Jiangsu, Peoples R China
  • [ 18 ] [Qian, Xing]Fuzhou Univ, Coll Chem Engn, Xueyuan Rd 2, Fuzhou 350116, Peoples R China

Reprint 's Address:

  • [Ge, Xin]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China;;[Cheng, Dang-guo]Zhejiang Univ, Coll Chem & Biol Engn, Zhejiang Prov Key Lab Adv Chem Engn Manufacture T, 38 Zheda Rd, Hangzhou 310027, Peoples R China

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Source :

CHEMICAL ENGINEERING JOURNAL

ISSN: 1385-8947

Year: 2022

Volume: 429

1 5 . 1

JCR@2022

1 3 . 4 0 0

JCR@2023

ESI Discipline: ENGINEERING;

ESI HC Threshold:66

JCR Journal Grade:1

CAS Journal Grade:1

Cited Count:

WoS CC Cited Count: 63

SCOPUS Cited Count: 84

ESI Highly Cited Papers on the List: 0 Unfold All

WanFang Cited Count:

Chinese Cited Count:

30 Days PV: 0

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